146 research outputs found
Theory of selective excitation in Stimulated Raman Scattering
A semiclassical model is used to investigate the possibility of selectively
exciting one of two closely spaced, uncoupled Raman transitions. The duration
of the intense pump pulse that creates the Raman coherence is shorter than the
vibrational period of a molecule (impulsive regime of interaction). Pulse
shapes are found that provide either enhancement or suppression of particular
vibrational excitations.Comment: RevTeX4,10 pages, 5 figures, submitted to Phys.Rev.
Coherent control using adaptive learning algorithms
We have constructed an automated learning apparatus to control quantum
systems. By directing intense shaped ultrafast laser pulses into a variety of
samples and using a measurement of the system as a feedback signal, we are able
to reshape the laser pulses to direct the system into a desired state. The
feedback signal is the input to an adaptive learning algorithm. This algorithm
programs a computer-controlled, acousto-optic modulator pulse shaper. The
learning algorithm generates new shaped laser pulses based on the success of
previous pulses in achieving a predetermined goal.Comment: 19 pages (including 14 figures), REVTeX 3.1, updated conten
Nonresonant control of multimode molecular wave packets at room temperature
Includes bibliographical references (pages 033001-4).We demonstrate the creation and measurement of shaped multimode vibrational wave packets with overtone and combination mode excitation in CCl4. Excitation of wave packets through nonresonant impulsive stimulated Raman scattering allows for coherent control of molecular vibrations without passing through an electronic resonance. This technique is therefore very general and can be implemented in a large class of molecular gases and liquids at STP, which were previously inaccessible because their resonances are in the VUV
Recommended from our members
Using spallation neutron sources for defense research
Advanced characterization techniques and accelerated simulation are the cornerstones of the Energy Department`s science-based program to maintain confidence in the safety, reliability, and performance of the US nuclear deterrent in an era of no nuclear testing. Neutrons and protons provided by an accelerator-based facility have an important role to play in this program, impacting several of the key stockpile stewardship and management issues identified by the Department of Defense. Many of the techniques used for defense research at a spallation source have been used for many years for the basic research community, and to a lesser extent by industrial scientists. By providing access to a broad spectrum of researchers with different backgrounds, a spallation source such as the Los Alamos Neutron Science Center is able to promote synergistic interaction between defense, basic and industrial researchers. This broadens the scientific basis of the stockpile stewardship program in the short term and will provide spin-off to industrial and basic research in the longer term
Beable trajectories for revealing quantum control mechanisms
The dynamics induced while controlling quantum systems by optimally shaped
laser pulses have often been difficult to understand in detail. A method is
presented for quantifying the importance of specific sequences of quantum
transitions involved in the control process. The method is based on a
``beable'' formulation of quantum mechanics due to John Bell that rigorously
maps the quantum evolution onto an ensemble of stochastic trajectories over a
classical state space. Detailed mechanism identification is illustrated with a
model 7-level system. A general procedure is presented to extract mechanism
information directly from closed-loop control experiments. Application to
simulated experimental data for the model system proves robust with up to 25%
noise.Comment: Latex, 20 pages, 13 figure
An optically driven quantum dot quantum computer
We propose a quantum computer structure based on coupled asymmetric
single-electron quantum dots. Adjacent dots are strongly coupled by means of
electric dipole-dipole interactions enabling rapid computation rates. Further,
the asymmetric structures can be tailored for a long coherence time. The result
maximizes the number of computation cycles prior to loss of coherence.Comment: 4 figure
Momentum state engineering and control in Bose-Einstein condensates
We demonstrate theoretically the use of genetic learning algorithms to
coherently control the dynamics of a Bose-Einstein condensate. We consider
specifically the situation of a condensate in an optical lattice formed by two
counterpropagating laser beams. The frequency detuning between the lasers acts
as a control parameter that can be used to precisely manipulate the condensate
even in the presence of a significant mean-field energy. We illustrate this
procedure in the coherent acceleration of a condensate and in the preparation
of a superposition of prescribed relative phase.Comment: 9 pages incl. 6 PostScript figures (.eps), LaTeX using RevTeX,
submitted to Phys. Rev. A, incl. small modifications, some references adde
Quantum Holographic Encoding in a Two-dimensional Electron Gas
The advent of bottom-up atomic manipulation heralded a new horizon for
attainable information density, as it allowed a bit of information to be
represented by a single atom. The discrete spacing between atoms in condensed
matter has thus set a rigid limit on the maximum possible information density.
While modern technologies are still far from this scale, all theoretical
downscaling of devices terminates at this spatial limit. Here, however, we
break this barrier with electronic quantum encoding scaled to subatomic
densities. We use atomic manipulation to first construct open
nanostructures--"molecular holograms"--which in turn concentrate information
into a medium free of lattice constraints: the quantum states of a
two-dimensional degenerate Fermi gas of electrons. The information embedded in
the holograms is transcoded at even smaller length scales into an atomically
uniform area of a copper surface, where it is densely projected into both two
spatial degrees of freedom and a third holographic dimension mapped to energy.
In analogy to optical volume holography, this requires precise amplitude and
phase engineering of electron wavefunctions to assemble pages of information
volumetrically. This data is read out by mapping the energy-resolved electron
density of states with a scanning tunnelling microscope. As the projection and
readout are both extremely near-field, and because we use native quantum states
rather than an external beam, we are not limited by lensing or collimation and
can create electronically projected objects with features as small as ~0.3 nm.
These techniques reach unprecedented densities exceeding 20 bits/nm2 and place
tens of bits into a single fermionic state.Comment: Published online 25 January 2009 in Nature Nanotechnology; 12 page
manuscript (including 4 figures) + 2 page supplement (including 1 figure);
supplementary movie available at http://mota.stanford.ed
Recommended from our members
Overview of progress on the improvement projects for the LANSCE accelerator and target facilities
Three projects have been initiated since 1994 to improve the performance of the accelerator and target facilities for the Los Alamos Neutron Science Center (LANSCE). The LANSCE Reliability Improvement Project (LRIP) was separated into two phases. Phase 1, completed in 1995, targeted near-term improvements to beam reliability and availability that could be completed in one-year`s time. Phase 2, now underway and scheduled for completion in May 1998, consists of two projects: (a) implementation of direct H-injection for the Proton Storage Ring (PSR) and (b) an upgrade of the target/moderator system for the short pulse spallation neutron (SPSS) source. The latter will reduce the target change-out time from about 10 months to about three weeks. The third project, the SPSS Enhancement Project, is aimed at increasing the PSR output beam current to 200 {micro}A at 30 Hz and providing up to seven new neutron scattering instruments
Optimized Dynamical Decoupling in a Model Quantum Memory
We present experimental measurements on a model quantum system that
demonstrate our ability to dramatically suppress qubit error rates by the
application of optimized dynamical decoupling pulse sequences in a variety of
experimentally relevant noise environments. We provide the first demonstration
of an analytically derived pulse sequence developed by Uhrig, and find novel
sequences through active, real-time experimental feedback. These new sequences
are specially tailored to maximize error suppression without the need for a
priori knowledge of the ambient noise environment. We compare these sequences
against the Uhrig sequence, and the well established CPMG-style spin echo,
demonstrating that our locally optimized pulse sequences outperform all others
under test. Numerical simulations show that our locally optimized pulse
sequences are capable of suppressing errors by orders of magnitude over other
existing sequences. Our work includes the extension of a treatment to predict
qubit decoherence under realistic conditions, including the use of
finite-duration, square pulses, yielding strong agreement between
experimental data and theory for arbitrary pulse sequences. These results
demonstrate the robustness of qubit memory error suppression through dynamical
decoupling techniques across a variety of qubit technologies.Comment: Subject to press embarg
- …