811 research outputs found
Spin Dynamics in the Magnetic Chains Arrays of Sr14Cu24O41: a Neutron Inelastic scattering Investigation
Below about 150 K, the spin arrangement in the chain arrays of Sr14Cu24O41 is
shown to develop in two dimensions (2D). Both the correlations and the
dispersion of the observed elementary excitations agree well with a model of
interacting dimers. Along the chains, the intra- and inter-dimer distances are
equal to 2 and about 3 times the distance (c) between neighboring Cu ions.
While the intra-dimer coupling is J about 10 meV, the inter-dimer couplings
along and between the chains are of comparable strenght, J// about -1.1 meV and
Jperp about 1.7 meV, respectively. This remarkable 2D arrangement satisfies the
formal Cu valence of the undoped compound. Our data suggest also that it is
associated with a relative sliding of one chain with respect to the next one,
which, as T decreases, develops in the chain direction. A qualitative analysis
shows that nearest inter-dimer spin correlations are ferromagnetic, which, in
such a 2D structure, could well result from frustration effects.Comment: 4 pages, 5 figures, submitted to Phys.Rev.B, date of receipt 29 June
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Single-crystal growth and dependences on the hole concentration and magnetic field of the magnetic ground state in the edge-sharing CuO chain system CaYCuO
We have succeeded in growing large-size single-crystals of
CaYCuO with and measured the
magnetic susceptibility, specific heat and magnetization curve, in order to
study the magnetic ground state in the edge-sharing CuO chain as a function
of hole concentration and magnetic field. In , it has been
found that an antiferromagnetically ordered phase with the magnetic easy axis
along the b-axis is stabilized and that a spin-flop transition occurs by the
application of magnetic fields parallel to the b-axis. The antiferromagnetic
transition temperature decreases with increasing and disappears around 1.4. Alternatively, a spin-glass phase appears around . At where the hole concentration is 1/3 per Cu, it appears that a
spin-gap state is formed owing to the formation of spin-singlet pairs. No sign
of the coexistence of an antiferromagnetically ordered state and a spin-gap one
suggested in CaCuO has been found in
CaYCuO.Comment: 13 pages, 12 figures, 1 tabl
Magnetic excitations and structural change in the S=1/2 quasi-one-dimensional magnet Sr_{14-x}Y_{x}Cu_{24}O_{41} (0<x<1)
Neutron scattering measurements have been performed on the S=1/2
quasi-one-dimensional system Sr_{14-x}Y_{x}Cu_{24}O_{41}, which has both simple
chains and two-leg ladders of copper ions. We observed that when a small amount
of yttrium is substituted for strontium, which is expected to reduce the number
of holes, the dimerized state and the structure in the chain are changed
drastically. The inelastic peaks originating from the dimerized state of the
chain becomes broader in energy but not in momentum space. This implies that
the dimerized state becomes unstable but the spin correlations are unchanged
with yttrium substitution. Furthermore, it was observed that nuclear Bragg peak
intensities originating from the chain show strong temperature and x
dependence, which suggests that the chains slide along the c axis as
temperature and x are varied.Comment: 5 pages, 6 figures, to appear in Phys. Rev.
Dynamic Spin Response for Heisenberg Ladders
We employ the recently proposed plaquette basis to investigate static and
dynamic properties of isotropic 2-leg Heisenberg spin ladders. Simple
non-interacting multi-plaquette states provide a remarkably accurate picture of
the energy/site and dynamic spin response of these systems. Insights afforded
by this simple picture suggest a very efficient truncation scheme for more
precise calculations. When the small truncation errors are accounted for using
recently developed Contractor Renormalization techniques, very accurate results
requiring a small fraction of the computational effort of exact calculations
are obtained. These methods allow us to determine the energy/site, gap, and
spin response of 2x16 ladders. The former two values are in good agreement with
density matrix renormalization group results. The spin response calculations
show that nearly all the strength is concentrated in the lowest triplet level
and that coherent many-body effects enhance the response/site by nearly a
factor of 1.6 over that found for 2x2 systems.Comment: 9 pages with two enclosed postscript figure
Effects of interladder couplings in the trellis lattice
Strongly correlated models on coupled ladders in the presence of frustration,
in particular the trellis lattice, are studied by numerical techniques. For the
undoped case, the possibility of incommensurate peaks in the magnetic structure
factor at low temperatures is suggested. In the doped case, our main conclusion
for the trellis lattice is that by increasing the interladder coupling, the
balance between the magnetic energy in the ladders and the kinetic energy in
the zig-zag chains is altered leading eventually to the destruction of the hole
pairs initially formed and localized in the ladders.Comment: final version, to appear in Physical Review
Dynamical Spin Response Functions for Heisenberg Ladders
We present the results of a numerical study of the 2 by L spin 1/2 Heisenberg
ladder. Ground state energies and the singlet-triplet energy gaps for L =
(4-14) and equal rung and leg interaction strengths were obtained in a Lanczos
calculation and checked against earlier calculations by Barnes et al. (even L
up to 12). A related moments technique is then employed to evaluate the
dynamical spin response for L=12 and a range of rung to leg interaction
strength ratios (0 - 5). We comment on two issues, the need for
reorthogonalization and the rate of convergence, that affect the numerical
utility of the moments treatment of response functions.Comment: Revtex, 3 figure
Quasi-two-dimensional hole ordering and dimerized state in the CuO2-chain layers in Sr14Cu24O41
Neutron scattering experiments have been performed on
SrCuO which consists of both chains and ladders of copper
ions. We observed that the magnetic excitations from the CuO chain have two
branches and that both branches are weakly dispersive along the and
axes. The - dispersion relation as well as the intensities can be
reasonably described by a random phase approximation with intradimer coupling
between next-nearest-neighbor copper spins =11 meV, interdimer coupling
along the c axis =0.75 meV, and interdimer coupling along the a axis
=0.75 meV. The dimer configuration indicates a quasi-two-dimensional hole
ordering, resulting in an ordering of magnetic Cu with spin-1/2 and
nonmagnetic Cu, which forms the Zhang-Rice singlet. We have also studied the
effect of Ca substitution for Sr on the dimer and the hole ordering.Comment: 7 pages, Revtex, 10 figures, Submitted to Phys. Rev.
Phases of two coupled Luttinger liquids
A model of two interacting one--dimensional fermion systems (``Luttinger
liquids'') coupled by single--particle hopping is investigated. Bosonization
allows a number of exact statements to be made. In particular, for forward
scattering only, the model contains two massless boson sectors and an Ising
type critical sector. For general interactions, there is a spin excitation gap
and either s-- or d--type pairing fluctuations dominate. It is shown that the
same behavior is also found for strong interactions. A possible scenario for
the crossover to a Fermi liquid in a many chain system is discussed.Comment: revised version, some changes, 11 pages, no figures, RexTeX3.
Nuclear Spin Relaxation in Hole Doped Two-Leg Ladders
The nuclear spin-lattice relaxation rate () has been measured in the
single crystals of hole doped two-leg ladder compounds
SrCaCuO and in the undoped parent material
LaCaCuO. Comparison of at the Cu and the two
distinct oxygen sites revealed that the major spectral weight of low frequency
spin fluctuations is located near for most of the
temperature and doping ranges investigated. Remarkable difference in the
temperature dependence of for the two oxygen sites in the heavily doped
=12 sample revealed reduction of singlet correlations between two legs in
place of growing antiferromagnetic correlations along the leg direction with
increasing temperature. Such behavior is most likely caused by the dissociation
of bound hole pairs.Comment: 4 pages. to appear in J. Phys. Soc. Jpn. Vol. 6
Role of low-frequency vibrations on sound propagation in glasses at intermediate temperature
We report measurements of the temperature dependence of the sound attenuation and the fractional change in sound velocity for the glass (G) and orientational-glass (OG) phases of polymorphic ethanol. Strikingly similar behaviors are found for both phases despite the OG's underlying crystal (bcc) lattice. Such similarity, which is also revealed in dielectric spectroscopy and inelastic neutron scattering measurements, suggests whole molecule small-angle librations as a common microscopic origin for a wide variety of "glassy" phenomena.Dirección General de Investigación Científica y Técnica PB95-0075-C03-0
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