3 research outputs found
Local modes, phonons, and mass transport in solid He
We propose a model to treat the local motion of atoms in solid He as a
local mode. In this model, the solid is assumed to be described by the Self
Consistent Harmonic approximation, combined with an array of local modes. We
show that in the bcc phase the atomic local motion is highly directional and
correlated, while in the hcp phase there is no such correlation. The correlated
motion in the bcc phase leads to a strong hybridization of the local modes with
the T phonon branch, which becomes much softer than that obtained
through a Self Consistent Harmonic calculation, in agreement with experiment.
In addition we predict a high energy excitation branch which is important for
self-diffusion. Both the hybridization and the presence of a high energy branch
are a consequence of the correlation, and appear only in the bcc phase. We
suggest that the local modes can play the role in mass transport usually
attributed to point defects (vacancies). Our approach offers a more overall
consistent picture than obtained using vacancies as the predominant point
defect. In particular, we show that our approach resolves the long standing
controversy regarding the contribution of point defects to the specific heat of
solid He.Comment: 10 pages, 10 figure