80 research outputs found
Spin-resonance modes of the spin-gap magnet TlCuCl_3
Three kinds of magnetic resonance signals were detected in crystals of the
spin-gap magnet TlCuCl_3.
First, we have observed the microwave absorption due to the excitation of the
transitions between the singlet ground state and the excited triplet states.
This mode has the linear frequency-field dependence corresponding to the
previously known value of the zero-field spin-gap of 156 GHz and to the closing
of spin-gap at the magnetic field H_c of about 50 kOe.
Second, the thermally activated resonance absorption due to the transitions
between the spin sublevels of the triplet excitations was found. These
sublevels are split by the crystal field and external magnetic field.
Finally, we have observed antiferromagnetic resonance absorption in the
field-induced antiferromagnetic phase above the critical field H_c. This
resonance frequency is strongly anisotropic with respect to the direction of
the magnetic field.Comment: v.2: typo correction (one of the field directions was misprinted in
the v.1
Haldane-gap excitations in the low-H_c 1-dimensional quantum antiferromagnet NDMAP
Inelastic neutron scattering on deuterated single-crystal samples is used to
study Haldane-gap excitations in the new S=1 one-dimensional quantum
antiferromagnet NDMAP, that was recently recognized as an ideal model system
for high-field studies. The Haldane gap energies meV,
meV and meV, for excitations polarized along
the a, b, and c crystallographic axes, respectively, are directly measured. The
dispersion perpendicular to the chain axis c is studied, and extremely weak
inter-chain coupling constants meV and meV, along the a and b axes, respectively, are determined. The results
are discussed in the context of future experiments in high magnetic fields.Comment: 5 pages, 4 figures, submitted to Phys. Rev.
Hidden long range order in Heisenberg Kagome antiferromagnets
We give a physical picture of the low-energy sector of the spin 1/2
Heisenberg Kagome antiferromagnet (KAF). It is shown that Kagome lattice can be
presented as a set of stars which are arranged in a triangular lattice and
contain 12 spins. Each of these stars has two degenerate singlet ground states
which can be considered in terms of pseudospin. As a result of interaction
between stars we get Hamiltonian of the Ising ferromagnet in magnetic field. So
in contrast to the common view there is a long range order in KAF consisting of
definite singlet states of the stars.Comment: 4 pages, 3 figures, submitted to Physical Review Letter
Massive triplet excitations in a magnetized anisotropic Haldane spin chain
Inelastic neutron scattering experiments on the Haldane-gap quantum
antiferromagnet \nd are performed at mK temperatures in magnetic fields of
almost twice the critical field applied perpendicular to the spin cahins.
Above a re-opening of the spin gap is clearly observed. In the high-field
N\'eel-ordered state the spectrum is dominated by three distinct long-lived
excitation branches. Several field-theoretical models are tested in a
quantitative comparison with the experimental data.Comment: 4 pages, 3 figure
Further analysis of the quantum critical point of CeLaRuSi
New data on the spin dynamics and the magnetic order of
CeLaRuSi are presented. The importance of the Kondo
effect at the quantum critical point of this system is emphasized from the
behaviour of the relaxation rate at high temperature and from the variation of
the ordered moment with respect to the one of the N\'eel temperature for
various .Comment: Contribution for the Festschrift on the occasion of Hilbert von
Loehneysen 60 th birthday. To be published as a special issue in the Journal
of Low Temperature Physic
Dynamics of an anisotropic Haldane antiferromagnet in strong magnetic field
We report the results of elastic and inelastic neutron scattering experiments
on the Haldane gap quantum antiferromagnet Ni(C5D14N2)2N3(PF6) performed at mK
temperatures in a wide range of magnetic field applied parallel to the S = 1
spin chains. Even though this geometry is closest to an ideal axially symmetric
configuration, the Haldane gap closes at the critical field Hc~4T, but reopens
again at higher fields. The field dependence of the two lowest magnon modes is
experimentally studied and the results are compared with the predictions of
several theoretical models. We conclude that of several existing theories, only
the recently proposed model [Zheludev et al., cond-mat/0301424 ] is able to
reproduce all the features observed experimentally for different field
orientations.Comment: 11 pages 8 figures submitted to Phys. Rev.
Elementary Excitations in Dimerized and Frustrated Heisenberg Chains
We present a detailed numerical analysis of the low energy excitation
spectrum of a frustrated and dimerized spin Heisenberg chain. In
particular, we show that in the commensurate spin--Peierls phase the ratio of
the singlet and triplet excitation gap is a universal function which depends on
the frustration parameter only. We identify the conditions for which a second
elementary triplet branch in the excitation spectrum splits from the continuum.
We compare our results with predictions from the continuum limit field theory .
We discuss the relevance of our data in connection with recent experiments on
, , and .Comment: Corrections to the text + 1 new figure, will appear in PRB (august
98
Site-Dilution-Induced Antiferromagnetic Long-Range Order in Two-Dimensional Spin-Gapped Heisenberg Antiferromagnet
Effects of the site dilution on spin-gapped Heisenberg antiferromagnets with
and S=1 on a square lattice are investigated by means of the quantum
Monte Carlo method. It is found that effective magnetic moments induced around
the diluted sites exhibit the antiferromagnetic long-range order in the medium
of spin-singlet pairs. Their microscopic structure is examined in detail and
important roles of the higher dimensionality than one on the phenomenon are
discussed.Comment: RevTeX, 4 pages, 6 figure
The first-order phase transition between dimerized-antiferromagnetic and uniform-antiferromagnetic phases in Cu_(1-x)M_xGeO_3
We have performed detailed magnetic susceptibility measurements as well as
synchrotron x-ray diffraction studies to determine the temperature vs
concentration ( - ) phase diagram of CuMgGeO. We
observe clear double peaks in the magnetic susceptibility implying two
antiferromagnetic (AF) transition temperatures in samples with Mg
concentrations in the range 0.0237 0.0271. We also observe a
drastic change in the inverse correlation length in this concentration range by
x-ray diffraction. The drastic change of the AF transition temperature as well
as the disappearance of the spin-Peierls (SP) phase have been clarified; these
results are consistent with a first-order phase transition between dimerized AF
(D-AF) and uniform AF (U-AF) phases as reported by T. Masuda {\it et al.}
\lbrack Phys. Rev. Lett. {\bf 80}, 4566 (1998)\rbrack. The - phase
diagram of CuZnGeO is similar to that of
CuMgGeO, which suggests that the present phase transition
is universal for CuGeO.Comment: 7 pages, 5 figures. submitted to PR
Separation of the magnetic phases at the N\'{e}el point in the diluted spin-Peierls magnet CuGeO3
The impurity induced antiferromagnetic ordering of the doped spin-Peierls
magnet Cu(1-x)Mg(x)GeO(3) was studied by ESR technique. Crystals with the Mg
concentration x<4% demonstrate a coexistence of paramagnetic and
antiferromagnetic ESR modes. This coexistence indicates the separation of a
macroscopically uniform sample in the paramagnetic and antiferromagnetic
phases. In the presence of the long-range spin-Peierls order (in a sample with
x=1.71%) the volume of the antiferromagnetic phase immediately below the
N\'{e}el point T_N is much smaller than the volume of the paramagnetic phase.
In the presence of the short-range spin-Peierls order (in samples with x=2.88%,
x= 3.2%) there are comparable volumes of paramagnetic and antiferromagnetic
phases at T=T_N. The fraction of the antiferromagnetic phase increases with
lowering temperature. In the absence of the spin-Peierls dimerization (at
x=4.57%)the whole sample exhibits the transition into the antiferromagnetic
state and there is no phase separation. The phase separation is explained by
the consideration of clusters of staggered magnetization located near impurity
atoms. In this model the areas occupied by coherently correlated spins expand
with decreasing temperature and the percolation of the ordered area through a
macroscopic distance occurs.Comment: 7pages, 10 figure
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