Experimental Determination of Thermal Entanglement in Spin Clusters using Magnetic Susceptibility Measurements

The present work reports an experimental observation of thermal entanglement in a clusterized spin chain formed in the compound Na$_2$Cu$_5$Si$_4$O$_{14}$. The presence of entanglement was investigated through two measured quantities, an Entanglement Witness and the Entanglement of Formation, both derived from the magnetic susceptibility. It was found that pairwise entanglement exists below $\sim 200$ K. Tripartite entanglement was also observed below $\sim 240$ K. A theoretical study of entanglement evolution as a function of applied field and temperature is also presented.Comment: Submited to Phys. Rev.

Experimental determination of the non-extensive entropic parameter qq

We show how to extract the $q$ parameter from experimental data, considering an inhomogeneous magnetic system composed by many Maxwell-Boltzmann homogeneous parts, which after integration over the whole system recover the Tsallis non-extensivity. Analyzing the cluster distribution of La$_{0.7}$Sr$_{0.3}$MnO$_{3}$ manganite, obtained through scanning tunnelling spectroscopy, we measure the $q$ parameter and predict the bulk magnetization with good accuracy. The connection between the Griffiths phase and non-extensivity is also considered. We conclude that the entropic parameter embodies information about the dynamics, the key role to describe complex systems.Comment: Submitted to Phys. Rev. Let

Non-Local Product Rules for Percolation

Despite original claims of a first-order transition in the product rule model proposed by Achlioptas et al. [Science 323, 1453 (2009)], recent studies indicate that this percolation model, in fact, displays a continuous transition. The distinctive scaling properties of the model at criticality, however, strongly suggest that it should belong to a different universality class than ordinary percolation. Here we introduce a generalization of the product rule that reveals the effect of non-locality on the critical behavior of the percolation process. Precisely, pairs of unoccupied bonds are chosen according to a probability that decays as a power-law of their Manhattan distance, and only that bond connecting clusters whose product of their sizes is the smallest, becomes occupied. Interestingly, our results for two-dimensional lattices at criticality shows that the power-law exponent of the product rule has a significant influence on the finite-size scaling exponents for the spanning cluster, the conducting backbone, and the cutting bonds of the system. In all three cases, we observe a continuous variation from ordinary to (non-local) explosive percolation exponents.Comment: 5 pages, 4 figure

How dense can one pack spheres of arbitrary size distribution?

We present the first systematic algorithm to estimate the maximum packing density of spheres when the grain sizes are drawn from an arbitrary size distribution. With an Apollonian filling rule, we implement our technique for disks in 2d and spheres in 3d. As expected, the densest packing is achieved with power-law size distributions. We also test the method on homogeneous and on empirical real distributions, and we propose a scheme to obtain experimentally accessible distributions of grain sizes with low porosity. Our method should be helpful in the development of ultra-strong ceramics and high performance concrete.Comment: 5 pages, 5 figure

Entanglement and Bell's inequality violation above room temperature in metal carboxylates

In the present work we show that a special family of materials, the metal carboxylates, may have entangled states up to very high temperatures. From magnetic susceptibility measurements, we have estimated the critical temperature below which entanglement exists in the cooper carboxylate \{Cu$_2$(O$_2$CH)$_4$\}\{Cu(O$_2$CH)$_2$(2-methylpyridine)$_2$\}, and we have found this to be above room temperature ($T_e \sim 630$ K). Furthermore, the results show that the system remains maximally entangled until close to $\sim 100$ K and the Bell's inequality is violated up to nearly room temperature ($\sim 290$ K)

Evidence for entanglement at high temperatures in an engineered molecular magnet

The molecular compound [Fe$_{2}$($\mu_{2}$-oxo)(C$_{3}$H$_{4}$N$_{2}$)$_{6}$(C$_{2}$O$_{4}$)$_{2}$] was designed and synthesized for the first time and its structure was determined using single-crystal X-ray diffraction. The magnetic susceptibility of this compound was measured from 2 to 300 K. The analysis of the susceptibility data using protocols developed for other spin singlet ground-state systems indicates that the quantum entanglement would remain at temperatures up to 732 K, significantly above the highest entanglement temperature reported to date. The large gap between the ground state and the first-excited state (282 K) suggests that the spin system may be somewhat immune to decohering mechanisms. Our measurements strongly suggest that molecular magnets are promising candidate platforms for quantum information processing