Measurement of spin memory lengths in PdNi and PdFe ferromagnetic alloys

Weakly ferromagnetic alloys are being used by several groups in the study of superconducting/ferromagnetic hybrid systems. Because spin-flip and spin-orbit scattering in such alloys disrupt the penetration of pair correlations into the ferromagnetic material, it is desirable to have a direct measurement of the spin memory length in such alloys. We have measured the spin memory length at 4.2 K in sputtered Pd0.88Ni0.12 and Pd0.987Fe0.013 alloys using methods based on current-perpendicular-to-plane giant magnetoresistance. The alloys are incorporated into hybrid spin valves of various types, and the spin memory length is determined by fits of the Valet-Fert spin-transport equations to data of magnetoresistance vs. alloy thickness. For the case of PdNi alloy, the resulting values of the spin memory length are lsf(PdNi) = 2.8 +/- 0.5 nm and 5.4 +/- 0.6 nm, depending on whether or not the PdNi is exchange biased by an adjacent Permalloy layer. For PdFe, the spin memory length is somewhat longer, lsf(PdFe) = 9.6 +/- 2 nm, consistent with earlier measurements indicating lower spin-orbit scattering in that material. Unfortunately, even the longer spin memory length in PdFe may not be long enough to facilitate observation of spin-triplet superconducting correlations predicted to occur in superconducting/ferromagnetic hybrid systems in the presence of magnetic inhomogeneity.Comment: 7 pages, 8 figure

Conductance fluctuations in the presence of spin scattering

Electron transport through disordered systems that include spin scatterers is studied numerically. We consider three kinds of magnetic impurities: the Ising, the XY and the Heisenberg. By extending the transfer matrix method to include the spin degree of freedom, the two terminal conductance is calculated. The variance of conductance is halved as the number of spin components of the magnetic impurities increases. Application of the Zeeman field in the lead causes a further halving of the variance under certain conditions.Comment: to be published in Phys. Rev.

Shifting a Quantum Wire through a Disordered Crystal: Observation of Conductance Fluctuations in Real Space

A quantum wire is spatially displaced by suitable electric fields with respect to the scatterers inside a semiconductor crystal. As a function of the wire position, the low-temperature resistance shows reproducible fluctuations. Their characteristic temperature scale is a few hundred millikelvin, indicating a phase-coherent effect. Each fluctuation corresponds to a single scatterer entering or leaving the wire. This way, scattering centers can be counted one by one.Comment: 4 pages, 3 figure

Observation of Fluctuation-Dissipation-Theorem Violations in a Structural Glass

The fluctuation-dissipation theorem (FDT), connecting dielectric susceptibility and polarization noise was studied in glycerol below its glass transition temperature Tg. Weak FDT violations were observed after a quench from just above to just below Tg, for frequencies above the alpha peak. Violations persisted up to 10^5 times the thermal equilibration time of the configurational degrees of freedom under study, but comparable to the average relaxation time of the material. These results suggest that excess energy flows from slower to faster relaxing modes.Comment: Improved discussion; final version to appear in Phys. Rev. Lett. 4 pages, 5 PS figures, RevTe

Spin-boson models for quantum decoherence of electronic excitations of biomolecules and quantum dots in a solvent

We give a theoretical treatment of the interaction of electronic excitations (excitons) in biomolecules and quantum dots with the surrounding polar solvent. Significant quantum decoherence occurs due to the interaction of the electric dipole moment of the solute with the fluctuating electric dipole moments of the individual molecules in the solvent. We introduce spin boson models which could be used to describe the effects of decoherence on the quantum dynamics of biomolecules which undergo light-induced conformational change and on biomolecules or quantum dots which are coupled by Forster resonant energy transfer.Comment: More extended version, to appear in Journal of Physics: Condensed Matter. 13 pages, 3 figure

Frequency dependent specific heat of viscous silica

We apply the Mori-Zwanzig projection operator formalism to obtain an expression for the frequency dependent specific heat c(z) of a liquid. By using an exact transformation formula due to Lebowitz et al., we derive a relation between c(z) and K(t), the autocorrelation function of temperature fluctuations in the microcanonical ensemble. This connection thus allows to determine c(z) from computer simulations in equilibrium, i.e. without an external perturbation. By considering the generalization of K(t) to finite wave-vectors, we derive an expression to determine the thermal conductivity \lambda from such simulations. We present the results of extensive computer simulations in which we use the derived relations to determine c(z) over eight decades in frequency, as well as \lambda. The system investigated is a simple but realistic model for amorphous silica. We find that at high frequencies the real part of c(z) has the value of an ideal gas. c'(\omega) increases quickly at those frequencies which correspond to the vibrational excitations of the system. At low temperatures c'(\omega) shows a second step. The frequency at which this step is observed is comparable to the one at which the \alpha-relaxation peak is observed in the intermediate scattering function. Also the temperature dependence of the location of this second step is the same as the one of the $\alpha-$peak, thus showing that these quantities are intimately connected to each other. From c'(\omega) we estimate the temperature dependence of the vibrational and configurational part of the specific heat. We find that the static value of c(z) as well as \lambda are in good agreement with experimental data.Comment: 27 pages of Latex, 8 figure

Slow dynamics and aging in a non-randomly frustrated spin system

A simple, non-disordered spin model has been studied in an effort to understand the origin of the precipitous slowing down of dynamics observed in supercooled liquids approaching the glass transition. A combination of Monte Carlo simulations and exact calculations indicates that this model exhibits an entropy vanishing transition accompanied by a rapid divergence of time scales. Measurements of various correlation functions show that the system displays a hierarchy of time scales associated with different degrees of freedom. Extended structures, arising from the frustration in the system, are identified as the source of the slow dynamics. In the simulations, the system falls out of equilibrium at a temperature $T_{g}$ higher than the entropy-vanishing transition temperature and the dynamics below $T_{g}$ exhibits aging as distinct from coarsening. The cooling rate dependence of the energy is also consistent with the usual glass formation scenario.Comment: 41 pages, 16 figures. Bibliography file is correcte