Deuterium site occupancy and phase boundaries in ZrNiDx (0.87<=x<=3.0)

ZrNiDx samples with compositions between x=0.87 and x=3.0 were investigated by 2H magic-angle spinning nuclear magnetic resonance spectroscopy (MAS-NMR), powder x-ray diffraction (XRD), neutron vibrational spectroscopy (NVS), and neutron powder diffraction (NPD). The rigid-lattice MAS-NMR spectrum for a ZrNiD0.88 sample in the triclinic beta phase shows a single phase with two well-resolved resonances at +11.5 and −1.7 ppm, indicating that two inequivalent D sites are occupied, as was observed previously in ZrNiD1.0. For ZrNiD0.88, the ratio of spectral intensities of the two lines is 1:0.76, indicating that the D site corresponding to the +11.5 ppm line has the lower site energy and is fully occupied. Similarly, the neutron vibrational spectra for ZrNiD0.88 clearly confirm that at least two sites are occupied. For ZrNiD1.0, XRD indicates that ~5% of the metal atoms are in the gamma phase, corresponding to an upper composition for the beta phase of x=0.90±0.04, consistent with the MAS-NMR and neutron vibrational spectra indicating that x=0.88 is single phase. The MAS-NMR and NVS of ZrNiD1.87 indicate a mixed-phase sample (beta+gamma) and clearly show that the two inequivalent sites observed at x=0.88 cannot be attributed to the sites normally occupied in the gamma phase. For ZrNiD2.75, NPD results indicate a gamma-phase boundary of x=2.86±0.03 at 300 K, increasing to 2.93±0.02 at 180 K and below, in general agreement with the phase boundary estimated from the NVS and MAS-NMR spectra of ZrNiD1.87. Rigid-lattice 2H MAS-NMR spectra of ZrNiD2.75 and ZrNiD2.99 show a ratio of spectral intensities of 1.8±0.1:1 and 2.1±0.1:1 (Zr3Ni:Zr3Ni2), respectively, indicating complete occupancy of the lower-energy Zr3Ni2 site, consistent with the NPD results. For each composition, the correlation time for deuterium hopping was determined at the temperature where resolved peaks in the MAS-NMR spectrum coalesce due to motion between inequivalent D sites. The measured correlation times are consistent with previously determined motional parameters for ZrNiHx

Island Size and Environment Dependence of Adatom Capture: CuyCo Islands on Ru(0001)

We quantify the rate of capture by Co islands on Ru(0001) of additionally deposited Cu atoms, using scanning tunneling microscopy. The dependence of the capture rates on Co-island size is shown to reflect larger island-free areas surrounding bigger islands, a feature neglected in mean-field treatments. We also find a strong direction dependence in Cu adatom capture, reflecting the local environment of individual islands. These features are elucidated by simulations and diffusion equation analyses

Effect of the length of inflation on angular TT and TE power spectra in power-law inflation

The effect of the length of inflation on the power spectra of scalar and tensor perturbations is estimated using the power-law inflation model with a scale factor of a(t) = t^q. Considering various pre-inflation models with radiation-dominated or scalar matter-dominated periods before inflation in combination with two matching conditions, the temperature angular power spectrum (TT) and temperature-polarization cross-power spectrum (TE) are calculated and a likelihood analysis is performed. It is shown that the discrepancies between the Wilkinson Microwave Anisotropy Probe (WMAP) data and the LCDM model, such as suppression of the spectrum at l = 2,3 and oscillatory behavior, may be explained by the finite length of inflation model if the length of inflation is near 60 e-folds and q > 300. The proposed models retain similar values of chi^2 to that achieved by the LCDM model with respect to fit to the WMAP data, but display different characteristics of the angular TE power spectra at l < 20.Comment: 41 pages, 11 figure

Quasiparticle properties of a coupled quantum wire electron-phonon system

We study leading-order many-body effects of longitudinal optical (LO) phonons on electronic properties of one-dimensional quantum wire systems. We calculate the quasiparticle properties of a weakly polar one dimensional electron gas in the presence of both electron-phonon and electron-electron interactions. The leading-order dynamical screening approximation (GW approximation) is used to obtain the electron self-energy, the quasiparticle spectral function, and the quasiparticle damping rate in our calculation by treating electrons and phonons on an equal footing. Our theory includes effects (within the random phase approximation) of Fermi statistics, Landau damping, plasmon-phonon mode coupling, phonon renormalization, dynamical screening, and impurity scattering. In general, electron-electron and electron-phonon many-body renormalization effects are found to be nonmultiplicative and nonadditive in our theoretical results for quasiparticle properties.Comment: 21 pages, Revtex, 12 figures enclose

Tunneling effects on impurity spectral function in coupled asymmetric quantum wires

The impurity spectral function is studied in coupled double quantum wires at finite temperatures. Simple anisotropy in the confinement direction of the wires leads to finite non-diagonal elements of the impurity spectral function matrix. These non-diagonal elements are responsible for tunneling effects and result in pronounced extra peak in the impurity spectral function up to temperatures as high as 20 K.Comment: Accepted in Phys. Rev.

Inelastic Coulomb scattering rates due to acoustic and optical plasmon modes in coupled quantum wires

We report a theoretical study on the inelastic Coulomb scattering rate of an injected electron in two coupled quantum wires in quasi-one-dimensional doped semiconductors. Two peaks appear in the scattering spectrum due to the optical and the acoustic plasmon scattering in the system. We find that the scattering rate due to the optical plasmon mode is similar to that in a single wire but the acoustic plasmon scattering depends crucially on its dispersion relation at small $q$. Furthermore, the effects of tunneling between the two wires are studied on the inelastic Coulomb scattering rate. We show that a weak tunneling can strongly affect the acoustic plasmon scattering.Comment: 6 Postscript figure

Heavy quarkonium 2S states in light-front quark model

We study the charmonium 2S states $\psi'$ and $\eta_c'$, and the bottomonium 2S states $\Upsilon'$ and $\eta_b'$, using the light-front quark model and the 2S state wave function of harmonic oscillator as the approximation of the 2S quarkonium wave function. The decay constants, transition form factors and masses of these mesons are calculated and compared with experimental data. Predictions of quantities such as Br$(\psi' \to \gamma \eta_c')$ are made. The 2S wave function may help us learn more about the structure of these heavy quarkonia.Comment: 5 latex pages, final version for journal publicatio

Large corrections to asymptotic FηcγF_{\eta_c \gamma} and FηbγF_{\eta_b \gamma} in the light-cone perturbative QCD

The large-$Q^2$ behavior of $\eta_c$-$\gamma$ and $\eta_b$-$\gamma$ transition form factors, $F_{\eta_c\gamma}(Q^2)$ and $F_{\eta_b\gamma}(Q^2)$ are analyzed in the framework of light-cone perturbative QCD with the heavy quark ($c$ and $b$) mass effect, the parton's transverse momentum dependence and the higher helicity components in the light-cone wave function are respected. It is pointed out that the quark mass effect brings significant modifications to the asymptotic predictions of the transition form factors in a rather broad energy region, and this modification is much severer for $F_{\eta_b\gamma}(Q^2)$ than that for $F_{\eta_c\gamma}(Q^2)$ due to the $b$-quark being heavier than the $c$-quark. The parton's transverse momentum and the higher helicity components are another two factors which decrease the perturbative predictions. For the transition form factor $F_{\eta_c\gamma}(Q^2)$, they bring sizable corrections in the present experimentally accessible energy region ($Q^2 \leq 10 GeV^2$). For the transition form factor $F_{\eta_b\gamma}(Q^2)$, the corrections coming from these two factors are negligible since the $b$-quark mass is much larger than the parton's average transverse momentum. The coming $e^+ e^-$ collider (LEP2) will provide the opportunity to examine these theoretical predictions.Comment: 8 pages, RevTex, 5 PostScript figure