81 research outputs found
Field-induced carrier delocalization in the strain-induced Mott insulating state of an organic superconductor
We report the influence of the field effect on the dc resistance and Hall
coefficient in the strain-induced Mott insulating state of an organic
superconductor -(BEDT-TTF)Cu[N(CN)]Br. Conductivity obeys
the formula for activated transport , where is a constant and depends on
the gate voltage. The gate voltage dependence of the Hall coefficient shows
that, unlike in conventional FETs, the effective mobility of dense hole
carriers ( cm) is enhanced by a positive gate
voltage. This implies that carrier doping involves delocalization of intrinsic
carriers that were initially localized due to electron correlation.Comment: 5 pages, 3 figure
Magnetic oscillations in a two-dimensional network of compensated electron and hole orbits
The FS of (ET)8Hg4Cl12(C6H5Br)2 can be regarded as a 2D network of
compensated electron and hole orbits coupled by magnetic breakthrough.
Simultaneous measurements of the interlayer magnetoresistance and magnetic
torque have been performed up to 28 T. Magnetoresistance and de dHvA
oscillations spectra exhibit frequency combinations typical of such a network.
Even though some of the observed magnetoresistance oscillations cannot be
interpreted on the basis of neither conventional SdH oscillations nor quantum
interference, the temperature and magnetic field (both orientation and
magnitude) dependence of all the Fourier components of the dHvA spectra can be
consistently accounted for by the LK formula. This behaviour is at variance
with that currently reported for compounds illustrating the linear chain of
coupled orbits model.Comment: accepted for publication in europhysics Letter
Competing types of quantum oscillations in the 2D organic conductor (BEDT-TTF)8Hg4Cl12(C6H5Cl)2
Interlayer magnetoconductance of the quasi-two dimensional organic metal
(BEDT-TTF)8Hg4Cl12(C6H5Cl)2 has been investigated in pulsed magnetic fields
extending up to 36 T and in the temperature range from 1.6 to 15 K. A complex
oscillatory spectrum, built on linear combinations of three basic frequencies
only is observed. These basic frequencies arise from the compensated closed
hole and electron orbits and from the two orbits located in between. The field
and temperature dependencies of the amplitude of the various oscillation series
are studied within the framework of the coupled orbits model of Falicov and
Stachowiak. This analysis reveals that these series result from the
contribution of either conventional Shubnikov-de Haas effect (SdH) or quantum
interference (QI), both of them being induced by magnetic breakthrough.
Nevertheless, discrepancies between experimental and calculated parameters
indicate that these phenomena alone cannot account for all of the data. Due to
its low effective mass, one of the QI oscillation series - which corresponds to
the whole first Brillouin zone area - is clearly observed up to 13 K.Comment: 8 pages, 8 figures. To be published in Phys. Rev.
High frequency magnetic oscillations of the organic metal -(ET)ZnBr(CHCl) in pulsed magnetic field of up to 81 T
De Haas-van Alphen oscillations of the organic metal
-(ET)ZnBr(CHCl) are studied in pulsed magnetic
fields up to 81 T. The long decay time of the pulse allows determining reliable
field-dependent amplitudes of Fourier components with frequencies up to several
kiloteslas. The Fourier spectrum is in agreement with the model of a linear
chain of coupled orbits. In this model, all the observed frequencies are linear
combinations of the frequency linked to the basic orbit and to the
magnetic-breakdown orbit .Comment: 6 pages, 4 figure
Quantum oscillations in the linear chain of coupled orbits: the organic metal with two cation layers theta-(ET)(4)CoBr(4)(C(6)H(4)Cl(2))
Analytical formulae for de Haas-van Alphen (dHvA) oscillations in linear
chain of coupled two-dimensional (2D) orbits (Pippard's model) are derived
systematically taking into account the chemical potential oscillations in
magnetic field. Although corrective terms are observed, basic (alpha) and
magnetic breakdown-induced (beta and 2beta - alpha) orbits can be accounted for
by the Lifshits-Kosevich (LK) and Falicov-Stachowiak semiclassical models in
the explored field and temperature ranges. In contrast, the 'forbidden orbit'
beta - alpha amplitude is described by a non-LK equation involving a product of
two classical orbit amplitudes. Furthermore, strongly non-monotonic field and
temperature dependence may be observed for the second harmonics of basic
frequencies such as 2alpha and the magnetic breakdown orbit beta + alpha,
depending on the value of the spin damping factors. These features are in
agreement with the dHvA oscillation spectra of the strongly 2D organic metal
theta- theta-(ET)(4)CoBr(4)(C(6)H(4)Cl(2)).Comment: to be published in Europhysics Letters (2012
Structure of the Fulde-Ferrell-Larkin-Ovchinnikov state in two-dimensional superconductors
Nonuniform superconducting state due to strong spin magnetism is studied in
two-dimensional type-II superconductors near the second order phase transition
line between the normal and the superconducting states. The optimum spatial
structure of the orderparameter is examined in systems with cylindrical
symmetric Fermi surfaces. It is found that states with two-dimensional
structures have lower free energies than the traditional one-dimensional
solutions, at low temperatures and high magnetic fields. For s-wave pairing,
triangular, square, hexagonal states are favored depending on the temperature,
while square states are favored at low temperatures for d-wave pairing. In
these states, orderparameters have two-dimensional structures such as square
and triangular lattices.Comment: 11 pages (LaTeX, revtex.sty), 3 figures; added reference
Different Types of Electron-Vibrational Interaction in BEDT-TTF Salts with Halide-Mercurate Anions Studied by IR Spectroscopy
Infrared optical properties of a large family of BEDT-TTF salts with mercury-halide anions are studied which exhibit different types of electron-vibrational spectra
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