60 research outputs found
Evidence of polariton induced transparency in a single organic quantum wire
The resonant interaction between quasi-one dimensional excitons and photons
is investigated. For a single isolated organic quantum wire, embedded in its
single crystal monomer matrix, the strong exciton-photon coupling regime is
reached. This is evidenced by the suppression of the resonant excitonic
absorption arising when the system eigenstate is a polariton. These
observations demonstrate that the resonant excitonic absorption in a
semiconductor can be understood in terms of a balance between the exciton
coherence time and the Rabi period between exciton-like and photon-like states
of the polariton.Comment: 9 pages and 4 figure
Langevin dynamics of the Coulomb frustrated ferromagnet: a mode-coupling analysis
We study the Langevin dynamics of the soft-spin, continuum version of the
Coulomb frustrated Ising ferromagnet. By using the dynamical mode-coupling
approximation, supplemented by reasonable approximations for describing the
equilibrium static correlation function, and the somewhat improved dynamical
self-consistent screening approximation, we find that the system displays a
transition from an ergodic to a non-ergodic behavior. This transition is
similar to that obtained in the idealized mode-coupling theory of glassforming
liquids and in the mean-field generalized spin glasses with one-step replica
symmetry breaking. The significance of this result and the relation to the
appearance of a complex free-energy landscape are also discussed.Comment: 13 pages, 11 figures, submitted to Phys. Rev.
Locally Preferred Structure and Frustration in Glassforming Liquids: A Clue to Polyamorphism?
We propose that the concept of liquids characterized by a given locally
preferred structure (LPS) could help in understanding the observed phenomenon
of polyamorphism. ``True polyamorphism'' would involve the competition between
two (or more) distinct LPS, one favored at low pressure because of its low
energy and one favored at high pressure because of its small specific volume,
as in tetrahedrally coordinated systems. ``Apparent polyamorphism'' could be
associated with the existence of a poorly crystallized defect-ordered phase
with a large unit cell and small crystallites, which may be illustrated by the
metastable glacial phase of the fragile glassformer triphenylphosphite; the
apparent polyamorphism might result from structural frustration, i. e., a
competition between the tendency to extend the LPS and a global constraint that
prevents tiling of the whole space by the LPS.Comment: 11, 6 figures, Proceedings of the Conference "Horizons in Complex
Systems", Messina; in honor of the 60th birthday of H.E. Stanle
Resonant excitonic emission of a single quantum dot in the Rabi regime
We report on coherent resonant emission of the fundamental exciton state in a
single semiconductor GaAs quantum dot. Resonant regime with picoseconde laser
excitation is realized by embedding the quantum dots in a waveguiding
structure. As the pulse intensity is increased, Rabi oscillation is observed up
to three periods. The Rabi regime is achieved owing to an enhanced light-matter
coupling in the waveguide. This is due to a \emph{slow light effect}
(), occuring when an intense resonant pulse propagates in a
medium. The resonant control of the quantum dot fundamental transition opens
new possibilities in quantum state manipulation and quantum optics experiments
in condensed matter physics.Comment: Submitted to Phys. Rev. Let
Influence of exciton spin relaxation on the photoluminescence spectra of semimagnetic quantum dots
We present a comprehensive experimental and theoretical studies of
photoluminescence of single CdMnTe quantum dots with Mn content x ranging from
0.01 to 0.2. We distinguish three stages of the equilibration of the exciton-Mn
ion spin system and show that the intermediate stage, in which the exciton spin
is relaxed, while the total equilibrium is not attained, gives rise to a
specific asymmetric shape of the photoluminescence spectrum. From an excellent
agreement between the measured and calculated spectra we are able to evaluate
the exciton localization volume, number of paramagnetic Mn ions, and their
temperature for each particular dot. We discuss the values of these parameters
and compare them with results of other experiments. Furthermore, we analyze the
dependence of average Zeeman shifts and transition linewidths on the Mn content
and point out specific processes, which control these values at particular Mn
concentrations.Comment: submitted to Phys. Rev.
The nature of slow dynamics in a minimal model of frustration-limited domains
We present simulation results for the dynamics of a schematic model based on
the frustration-limited domain picture of glass-forming liquids. These results
are compared with approximate theoretical predictions analogous to those
commonly used for supercooled liquid dynamics. Although model relaxation times
increase by several orders of magnitude in a non-Arrhenius manner as a
microphase separation transition is approached, the slow relaxation is in many
ways dissimilar to that of a liquid. In particular, structural relaxation is
nearly exponential in time at each wave vector, indicating that the mode
coupling effects dominating liquid relaxation are comparatively weak within
this model. Relaxation properties of the model are instead well reproduced by
the simplest dynamical extension of a static Hartree approximation. This
approach is qualitatively accurate even for temperatures at which the mode
coupling approximation predicts loss of ergodicity. These results suggest that
the thermodynamically disordered phase of such a minimal model poorly
caricatures the slow dynamics of a liquid near its glass transition
Macroscopic coherence of a single exciton state in a polydiacetylene organic quantum wire
We show that a single exciton state in an individual ordered conjugated
polymer chain exhibits macroscopic quantum spatial coherence reaching tens of
microns, limited by the chain length. The spatial coherence of the k=0 exciton
state is demonstrated by selecting two spatially separated emitting regions of
the chain and observing their interference.Comment: 12 pages with 2 figure
Dynamics of systems with isotropic competing interactions in an external field: a Langevin approach
We study the Langevin dynamics of a ferromagnetic Ginzburg-Landau Hamiltonian
with a competing long-range repulsive term in the presence of an external
magnetic field. The model is analytically solved within the self consistent
Hartree approximation for two different initial conditions: disordered or zero
field cooled (ZFC), and fully magnetized or field cooled (FC). To test the
predictions of the approximation we develop a suitable numerical scheme to
ensure the isotropic nature of the interactions. Both the analytical approach
and the numerical simulations of two-dimensional finite systems confirm a
simple aging scenario at zero temperature and zero field. At zero temperature a
critical field is found below which the initial conditions are relevant
for the long time dynamics of the system. For a logarithmic growth of
modulated domains is found in the numerical simulations but this behavior is
not captured by the analytical approach which predicts a growth law at
A Monte Carlo study of the three-dimensional Coulomb frustrated Ising ferromagnet
We have investigated by Monte-Carlo simulation the phase diagram of a
three-dimensional Ising model with nearest-neighbor ferromagnetic interactions
and small, but long-range (Coulombic) antiferromagnetic interactions. We have
developed an efficient cluster algorithm and used different lattice sizes and
geometries, which allows us to obtain the main characteristics of the
temperature-frustration phase diagram. Our finite-size scaling analysis
confirms that the melting of the lamellar phases into the paramgnetic phase is
driven first-order by the fluctuations. Transitions between ordered phases with
different modulation patterns is observed in some regions of the diagram, in
agreement with a recent mean-field analysis.Comment: 14 pages, 10 figures, submitted to Phys. Rev.
Local disorder and optical properties in V-shaped quantum wires : towards one-dimensional exciton systems
The exciton localization is studied in GaAs/GaAlAs V-shaped quantum wires
(QWRs) by high spatial resolution spectroscopy. Scanning optical imaging of
different generations of samples shows that the localization length has been
enhanced as the growth techniques were improved. In the best samples, excitons
are delocalized in islands of length of the order of 1 micron, and form a
continuum of 1D states in each of them, as evidenced by the sqrt(T) dependence
of the radiative lifetime. On the opposite, in the previous generation of QWRs,
the localization length is typically 50 nm and the QWR behaves as a collection
of quantum boxes. These localization properties are compared to structural
properties and related to the progresses of the growth techniques. The presence
of residual disorder is evidenced in the best samples and explained by the
separation of electrons and holes due to the large in-built piezo-electric
field present in the structure.Comment: 8 figure
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