432 research outputs found

    The Jamming Transition in Granular Systems

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    Recent simulations have predicted that near jamming for collections of spherical particles, there will be a discontinuous increase in the mean contact number, Z, at a critical volume fraction, phi_c. Above phi_c, Z and the pressure, P are predicted to increase as power laws in phi-phi_c. In experiments using photoelastic disks we corroborate a rapid increase in Z at phi_c and power-law behavior above phi_c for Z and P. Specifically we find power-law increase as a function of phi-phi_c for Z-Z_c with an exponent beta around 0.5, and for P with an exponent psi around 1.1. These exponents are in good agreement with simulations. We also find reasonable agreement with a recent mean-field theory for frictionless particles.Comment: 4 pages, 4 figures, 2 pages supplement; minor changes and clarifications, 2 addtl. refs., accepted for publication in Phys. Rev. Let

    Critical Decay at Higher-Order Glass-Transition Singularities

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    Within the mode-coupling theory for the evolution of structural relaxation in glass-forming systems, it is shown that the correlation functions for density fluctuations for states at A_3- and A_4-glass-transition singularities can be presented as an asymptotic series in increasing inverse powers of the logarithm of the time t: ϕ(t)−f∝∑igi(x)\phi(t)-f\propto \sum_i g_i(x), where gn(x)=pn(ln⁥x)/xng_n(x)=p_n(\ln x)/x^n with p_n denoting some polynomial and x=ln (t/t_0). The results are demonstrated for schematic models describing the system by solely one or two correlators and also for a colloid model with a square-well-interaction potential.Comment: 26 pages, 7 figures, Proceedings of "Structural Arrest Transitions in Colloidal Systems with Short-Range Attractions", Messina, Italy, December 2003 (submitted

    Evolution of unoccupied resonance during the synthesis of a silver dimer on Ag(111)

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    Silver dimers were fabricated on Ag(111) by single-atom manipulation using the tip of a cryogenic scanning tunnelling microscope. An unoccupied electronic resonance was observed to shift toward the Fermi level with decreasing atom-atom distance as monitored by spatially resolved scanning tunnelling spectroscopy. Density functional calculations were used to analyse the experimental observations and revealed that the coupling between the adsorbed atoms is predominantly direct rather than indirect via the Ag(111) substrate.Comment: 9 pages, 3 figure

    Unoccupied states of individual silver clusters and chains on Ag(111)

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    Size-selected silver clusters on Ag(111) were fabricated with the tip of a scanning tunneling microscope. Unoccupied electron resonances give rise to image contrast and spectral features which shift toward the Fermi level with increasing cluster size. Linear assemblies exhibit higher resonance energies than equally sized compact assemblies. Density functional theory calculations reproduce the observed energies and enable an assignment of the resonances to hybridized atomic 5s and 5p orbitals with silver substrate states.Comment: 9 pages, 8 figure

    EEG Microstates in Social and Affective Neuroscience.

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    Social interactions require both the rapid processing of multifaceted socio-affective signals (e.g., eye gaze, facial expressions, gestures) and their integration with evaluations, social knowledge, and expectations. Researchers interested in understanding complex social cognition and behavior face a "black box" problem: What are the underlying mental processes rapidly occurring between perception and action and why are there such vast individual differences? In this review, we promote electroencephalography (EEG) microstates as a powerful tool for both examining socio-affective states (e.g., processing whether someone is in need in a given situation) and identifying the sources of heterogeneity in socio-affective traits (e.g., general willingness to help others). EEG microstates are identified by analyzing scalp field maps (i.e., the distribution of the electrical field on the scalp) over time. This data-driven, reference-independent approach allows for identifying, timing, sequencing, and quantifying the activation of large-scale brain networks relevant to our socio-affective mind. In light of these benefits, EEG microstates should become an indispensable part of the methodological toolkit of laboratories working in the field of social and affective neuroscience

    Dynamic Glass Transition in Two Dimensions

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    The question about the existence of a structural glass transition in two dimensions is studied using mode coupling theory (MCT). We determine the explicit d-dependence of the memory functional of mode coupling for one-component systems. Applied to two dimensions we solve the MCT equations numerically for monodisperse hard discs. A dynamic glass transition is found at a critical packing fraction phi_c^{d=2} = 0.697 which is above phi_c^{d=3} = 0.516 by about 35%. phi^d_c scales approximately with phi^d_{\rm rcp} the value for random close packing, at least for d=2, 3. Quantities characterizing the local, cooperative 'cage motion' do not differ much for d=2 and d=3, and we e.g. find the Lindemann criterion for the localization length at the glass transition. The final relaxation obeys the superposition principle, collapsing remarkably well onto a Kohlrausch law. The d=2 MCT results are in qualitative agreement with existing results from MC and MD simulations. The mean squared displacements measured experimentally for a quasi-two-dimensional binary system of dipolar hard spheres can be described satisfactorily by MCT for monodisperse hard discs over four decades in time provided the experimental control parameter Gamma (which measures the strength of dipolar interactions) and the packing fraction phi are properly related to each other.Comment: 14 pages, 15 figure

    EAC-1A: A novel large-volume lunar regolith simulant

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    The European Astronaut Centre (EAC) is currently constructing the European Lunar Exploration Laboratory (LUNA), a large training and operations facility to be located adjacent to EAC at the DLR (German Aerospace Centre) campus in Cologne, Germany. With an estimated representative lunar testbed area of approximately 660 m(2), a large volume of lunar regolith simulant material is needed for this purpose. In this study, a basanitic sandy silt from a quarry located in the Siebengebirge Volcanic Field is evaluated as a large-volume source of material. The focus of this project has been to conduct a physical and chemical characterisation of the fine-grained material to be used in LUNA;the European Astronaut Centre lunar regolith simulant 1 (EAC-1A). The physical characterisation tests undertaken include sphericity, density measurements, cohesion and static angle of repose, with mineralogical investigations via petrographical analysis with optical microscope and SEM, XRF, XRD and DSC measurements. The results of the EAC-1A tests are compared to published data on existing widely used lunar regolith simulants, namely JSC-1A, JSC-2A, NU-LHT-3M, DNA and FJS-1

    Probing calculated O-2(+) potential-energy curves with an XUV-IR pump-probe experiment

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    Citation: Corlin, P., Fischer, A., Schonwald, M., Sperl, A., Mizuno, T., Thumm, U., . . . Moshammer, R. (2015). Probing calculated O-2(+) potential-energy curves with an XUV-IR pump-probe experiment. Physical Review A, 91(4), 8. doi:10.1103/PhysRevA.91.043415We study dissociative photoionization of molecular oxygen in a kinematically complete XUV-IR pump-probe experiment. Detecting charged fragments and photoelectrons in coincidence using a reaction microscope, we observe a pump-probe delay-dependent yield of very low energetic O+ ions which oscillates with a period of 40 fs. This feature is caused by a time-dependent vibrational wave packet in the potential of the binding O-2(+)(a(4)Pi(u))state, which is probed by resonant absorption of a single infrared photon to the weakly repulsive O-2(+)(f(4)Pi(g)) state. By quantitative comparison of the experimental kinetic-energy-release (KER) and quantum-beat (QB) spectra with the results of a coupled-channel simulation, we are able to discriminate between the calculated adiabatic O-2(+) potential-energy curves (PECs) of Marian et al. [Marian, Marian, Peyerimhoff, Hess, Buenker, and Seger, Mol. Phys. 46, 779 (1982)] and Magrakvelidze et al. [Magrakvelidze, Aikens, and Thumm, Phys. Rev. A 86, 023402 (2012)]. In general, we find a good agreement between experimental and simulated KER and QB spectra. However, we could not reproduce all features of the experimental data with these PECs. In contrast, adjusting a Morse potential to the experimental data, most features of the experimental spectra are well reproduced by our simulation. By comparing this Morse potential to theoretically predicted PECs, we demonstrate the sensitivity of our experimental method to small changes in the shape of the binding potential
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