Superconductivity and magnetism in platinum-substituted SrFe2As2 single crystals

Single crystals of SrFe2-xPtxAs2 (0 < x < 0.36) were grown using the self flux solution method and characterized using x-ray crystallography, electrical transport, magnetic susceptibility, and specific heat measurements. The magnetic/structural transition is suppressed with increasing Pt concentration, with superconductivity seen over the range 0.08 < x < 0.36 with a maximum transition temperature Tc of 16 K at x = 0.16. The shape of the phase diagram and the changes to the lattice parameters are similar to the effects of other group VIII elements Ni and Pd, however the higher transition temperature and extended range of superconductivity suggest some complexity beyond the simple electron counting picture that has been discussed thus far.Comment: 6 pages, 6 figure

Superconducting and ferromagnetic phases induced by lattice distortions in SrFe2As2

Single crystals of SrFe2As2 grown using a self-flux solution method were characterized via x-ray, transport and magnetization studies, revealing a superconducting phase below T_c = 21 K characterized by a full electrical resistivity transition and partial diamagnetic screening. The reversible destruction and reinstatement of this phase by heat treatment and mechanical deformation studies, along with single-crystal X-ray diffraction measurements, indicate that internal crystallographic strain originating from c-axis-oriented planar defects plays a central role in promoting the appearance of superconductivity under ambient pressure conditions in ~90% of as-grown crystals. The appearance of a ferromagnetic moment with magnitude proportional to the tunable superconducting volume fraction suggests that these phenomena are both stabilized by lattice distortion.Comment: 4 pages, 4 figure

The suppression of magnetism and the development of superconductivity within the collapsed tetragonal phase of Ca0.67Sr0.33Fe2As2 at high pressure

Structural and electronic characterization of (Ca0.67Sr0.33)Fe2As2 has been performed as a func- tion of pressure up to 12 GPa using conventional and designer diamond anvil cells. The compound (Ca0.67Sr0.33)Fe2As2 behaves intermediate between its end members-CaFe2As2 and SrFe2As2- displaying a suppression of magnetism and the onset of superconductivity. Like other members of the AEFe2As2 family, (Ca0.67Sr0.33)Fe2As2 undergoes a pressure-induced isostructural volume collapse, which we associate with the development of As-As bonding across the mirror plane of the structure. This collapsed tetragonal phase abruptly cuts off the magnetic state, giving rise to superconductivity with a maximum Tc=22.2 K. The maximum Tc of the superconducting phase is not strongly correlated with any structural parameter, but its proximity to the abrupt suppression of magnetism as well as the volume collapse transition suggests that magnetic interactions and structural inhomogeneity may play a role in its development. The pressure-dependent evolution of the ordered states and crystal structures in (Ca,Sr)Fe2As2 provides an avenue to understand the generic behavior of the other members of the AEFe2As2 family.Comment: 9 pages, 9 figure

Universal pair-breaking in transition metal-substituted iron-pnictide superconductors

The experimental transport scattering rate was determined for a wide range of optimally doped transition metal-substituted FeAs-based compounds with the ThCr2Si2 (122) crystal structure. The maximum transition temperature Tc for several Ba-, Sr-, and Ca-based 122 systems follows a universal rate of suppression with increasing scattering rate indicative of a common pair-breaking mechanism. Extraction of standard pair-breaking parameters puts a limit of \sim26 K on the maximum Tc for all transition metal-substituted 122 systems, in agreement with experimental observations, and sets a critical scattering rate of 1.5x10^14 s^-1 for the suppression of the superconducting phase. The observed critical scattering rate is much weaker than that expected for a sign-changing order parameter, providing important constraints on the nature of the superconducting gap in the 122 family of iron-based superconductors.Comment: 4 pages, 3 figure

On the resistivity at low temperatures in electron-doped cuprate superconductors

We measured the magnetoresistance as a function of temperature down to 20mK and magnetic field for a set of underdoped PrCeCuO (x=0.12) thin films with controlled oxygen content. This allows us to access the edge of the superconducting dome on the underdoped side. The sheet resistance increases with increasing oxygen content whereas the superconducting transition temperature is steadily decreasing down to zero. Upon applying various magnetic fields to suppress superconductivity we found that the sheet resistance increases when the temperature is lowered. It saturates at very low temperatures. These results, along with the magnetoresistance, cannot be described in the context of zero temperature two dimensional superconductor-to-insulator transition nor as a simple Kondo effect due to scattering off spins in the copper-oxide planes. We conjecture that due to the proximity to an antiferromagnetic phase magnetic droplets are induced. This results in negative magnetoresistance and in an upturn in the resistivity.Comment: Accepted in Phys. Rev.