359 research outputs found
Superconductivity and magnetism in platinum-substituted SrFe2As2 single crystals
Single crystals of SrFe2-xPtxAs2 (0 < x < 0.36) were grown using the self
flux solution method and characterized using x-ray crystallography, electrical
transport, magnetic susceptibility, and specific heat measurements. The
magnetic/structural transition is suppressed with increasing Pt concentration,
with superconductivity seen over the range 0.08 < x < 0.36 with a maximum
transition temperature Tc of 16 K at x = 0.16. The shape of the phase diagram
and the changes to the lattice parameters are similar to the effects of other
group VIII elements Ni and Pd, however the higher transition temperature and
extended range of superconductivity suggest some complexity beyond the simple
electron counting picture that has been discussed thus far.Comment: 6 pages, 6 figure
Superconducting and ferromagnetic phases induced by lattice distortions in SrFe2As2
Single crystals of SrFe2As2 grown using a self-flux solution method were
characterized via x-ray, transport and magnetization studies, revealing a
superconducting phase below T_c = 21 K characterized by a full electrical
resistivity transition and partial diamagnetic screening. The reversible
destruction and reinstatement of this phase by heat treatment and mechanical
deformation studies, along with single-crystal X-ray diffraction measurements,
indicate that internal crystallographic strain originating from c-axis-oriented
planar defects plays a central role in promoting the appearance of
superconductivity under ambient pressure conditions in ~90% of as-grown
crystals. The appearance of a ferromagnetic moment with magnitude proportional
to the tunable superconducting volume fraction suggests that these phenomena
are both stabilized by lattice distortion.Comment: 4 pages, 4 figure
The suppression of magnetism and the development of superconductivity within the collapsed tetragonal phase of Ca0.67Sr0.33Fe2As2 at high pressure
Structural and electronic characterization of (Ca0.67Sr0.33)Fe2As2 has been
performed as a func- tion of pressure up to 12 GPa using conventional and
designer diamond anvil cells. The compound (Ca0.67Sr0.33)Fe2As2 behaves
intermediate between its end members-CaFe2As2 and SrFe2As2- displaying a
suppression of magnetism and the onset of superconductivity. Like other members
of the AEFe2As2 family, (Ca0.67Sr0.33)Fe2As2 undergoes a pressure-induced
isostructural volume collapse, which we associate with the development of As-As
bonding across the mirror plane of the structure. This collapsed tetragonal
phase abruptly cuts off the magnetic state, giving rise to superconductivity
with a maximum Tc=22.2 K. The maximum Tc of the superconducting phase is not
strongly correlated with any structural parameter, but its proximity to the
abrupt suppression of magnetism as well as the volume collapse transition
suggests that magnetic interactions and structural inhomogeneity may play a
role in its development. The pressure-dependent evolution of the ordered states
and crystal structures in (Ca,Sr)Fe2As2 provides an avenue to understand the
generic behavior of the other members of the AEFe2As2 family.Comment: 9 pages, 9 figure
Universal pair-breaking in transition metal-substituted iron-pnictide superconductors
The experimental transport scattering rate was determined for a wide range of
optimally doped transition metal-substituted FeAs-based compounds with the
ThCr2Si2 (122) crystal structure. The maximum transition temperature Tc for
several Ba-, Sr-, and Ca-based 122 systems follows a universal rate of
suppression with increasing scattering rate indicative of a common
pair-breaking mechanism. Extraction of standard pair-breaking parameters puts a
limit of \sim26 K on the maximum Tc for all transition metal-substituted 122
systems, in agreement with experimental observations, and sets a critical
scattering rate of 1.5x10^14 s^-1 for the suppression of the superconducting
phase. The observed critical scattering rate is much weaker than that expected
for a sign-changing order parameter, providing important constraints on the
nature of the superconducting gap in the 122 family of iron-based
superconductors.Comment: 4 pages, 3 figure
On the resistivity at low temperatures in electron-doped cuprate superconductors
We measured the magnetoresistance as a function of temperature down to 20mK
and magnetic field for a set of underdoped PrCeCuO (x=0.12) thin films with
controlled oxygen content. This allows us to access the edge of the
superconducting dome on the underdoped side. The sheet resistance increases
with increasing oxygen content whereas the superconducting transition
temperature is steadily decreasing down to zero. Upon applying various magnetic
fields to suppress superconductivity we found that the sheet resistance
increases when the temperature is lowered. It saturates at very low
temperatures. These results, along with the magnetoresistance, cannot be
described in the context of zero temperature two dimensional
superconductor-to-insulator transition nor as a simple Kondo effect due to
scattering off spins in the copper-oxide planes. We conjecture that due to the
proximity to an antiferromagnetic phase magnetic droplets are induced. This
results in negative magnetoresistance and in an upturn in the resistivity.Comment: Accepted in Phys. Rev.
- …