864 research outputs found
Optical control of magnetization of micron-size domains in antiferromagnetic NiO single crystals
We propose Raman-induced collinear difference-frequency generation (DFG) as a
method to manipulate dynamical magnetization. When a fundamental beam
propagates along a threefold rotational axis, this coherent second-order
optical process is permitted by angular momentum conservation through the
rotational analogue of the Umklapp process. As a demonstration, we
experimentally obtained polarization properties of collinear magnetic DFG along
a [111] axis of a single crystal of antiferromagnetic NiO with micro
multidomain structure, which excellently agreed with the theoretical
prediction.Comment: 11 pages, 3 figures, submitted to Physical Review Letter
The Yellow Excitonic Series of Cu2O Revisited by Lyman Spectroscopy
We report on the observation of the yellow exciton Lyman series up to the
fourth term in Cu2O by time-resolved mid-infrared spectroscopy. The dependence
of the oscillator strength on the principal quantum number n can be well
reproduced using the hydrogenic model including an AC dielectric constant, and
precise information on the electronic structure of the 1s exciton state can be
obtained. A Bohr radius a_{1s}=7.9 A and a 1s-2p transition dipole moment
\mu_{1s-2p}= 4.2 eA were found
Study of ortho-to-paraexciton conversion in CuO by excitonic Lyman spectroscopy
Using time-resolved - excitonic Lyman spectroscopy, we study the
orthoexciton-to-paraexcitons transfer, following the creation of a high density
population of ultracold orthoexcitons by resonant two-photon excitation
with femtosecond pulses.
An observed fast exciton-density dependent conversion rate is attributed to
spin exchange between pairs of orthoexcitons.
Implication of these results on the feasibility of BEC of paraexcitons in
CuO is discussed
Formation and decay of electron-hole droplets in diamond
We study the formation and decay of electron-hole droplets in diamonds at
both low and high temperatures under different excitations by master equations.
The calculation reveals that at low temperature the kinetics of the system
behaves as in direct-gap semiconductors, whereas at high temperature it shows
metastability as in traditional indirect-gap semiconductors. Our results at low
temperature are consistent with the experimental findings by Nagai {\em et al.}
[Phys. Rev. B {\bf 68}, 081202 (R) (2003)]. The kinetics of the e-h system in
diamonds at high temperature under both low and high excitations is also
predicted.Comment: 7 pages, 8 figures, revised with some modifications in physics
discussion, to be published in PR
Dimensionality dependence of optical nonlinearity and relaxation dynamics in cuprates
Femtosecond pump-probe measurements find pronounced dimensionality dependence
of the optical nonlinearity in cuprates. Although the coherent two-photon
absorption (TPA) and linear absorption bands nearly overlap in both quasi-one
and two-dimensional (1D and 2D) cuprates, the TPA coefficient is one order of
magnitude smaller in 2D than in 1D. Furthermore, picosecond recovery of optical
transparency is observed in 1D cuprates, while the recovery in 2D involves
relaxation channels with a time scales of tens of picoseconds. The experimental
results are interpreted within the two-band extended Hubbard model.Comment: 10 pages, 4 figure
The Persistence and Memory of Polar Nano-Regions in a Ferroelectric Relaxor Under an Electric Field
The response of polar nanoregions (PNR) in the relaxor compound
Pb[(ZnNb)Ti]O subject to a [111]-oriented
electric field has been studied by neutron diffuse scattering. Contrary to
classical expectations, the diffuse scattering associated with the PNR
persists, and is even partially enhanced by field cooling. The effect of the
external electric field is retained by the PNR after the field is removed. The
``memory'' of the applied field reappears even after heating the system above
, and cooling in zero field
Quasi-degenerate self-trapping in one-dimensional charge transfer exciton
The self-trapping by the nondiagonal particle-phonon interaction between two
quasi-degenerate energy levels of excitonic system, is studied. We propose this
is realized in charge transfer exciton, where the directions of the
polarization give the quasi-degeneracy. It is shown that this mechanism, unlike
the conventional diagonal one, allows a coexistence and resonance of the free
and self-trapped states even in one-dimensional systems and a quantitative
theory for the optical properties (light absorption and time-resolved
luminescence) of the resonating states is presented. This theory gives a
consistent resolution for the long-standing puzzles in quasi-one-dimensional
compound A-PMDA.Comment: accepted to Phys. Rev. Letter
Soft Phonon Anomalies in the Relaxor Ferroelectric Pb(Zn_1/3Nb_2/3)_0.92Ti_0.08O_3
Neutron inelastic scattering measurements of the polar TO phonon mode
dispersion in the cubic relaxor Pb(Zn_1/3Nb_2/3)_0.92Ti_0.08O_3 at 500K reveal
anomalous behavior in which the optic branch appears to drop precipitously into
the acoustic branch at a finite value of the momentum transfer q=0.2 inverse
Angstroms, measured from the zone center. We speculate this behavior is the
result of nanometer-sized polar regions in the crystal.Comment: 4 pages, 4 figure
Alternativity and reciprocity in the Cayley-Dickson algebra
We calculate the eigenvalue \rho of the multiplication mapping R on the
Cayley-Dickson algebra A_n. If the element in A_n is composed of a pair of
alternative elements in A_{n-1}, half the eigenvectors of R in A_n are still
eigenvectors in the subspace which is isomorphic to A_{n-1}.
The invariant under the reciprocal transformation A_n \times A_{n} \ni (x,y)
-> (-y,x) plays a fundamental role in simplifying the functional form of \rho.
If some physical field can be identified with the eigenspace of R, with an
injective map from the field to a scalar quantity (such as a mass) m, then
there is a one-to-one map \pi: m \mapsto \rho. As an example, the electro-weak
gauge field can be regarded as the eigenspace of R, where \pi implies that the
W-boson mass is less than the Z-boson mass, as in the standard model.Comment: To be published in J. Phys. A: Mathematical and Genera
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