15,176 research outputs found

    Fe-doping induced superconductivity in charge-density-wave system 1T-TaS2

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    We report the interplay between charge-density-wave (CDW) and superconductivity of 1TT-Fex_{x}Ta1−x_{1-x}S2_{2} (0≤x≤0.050\leq x \leq 0.05) single crystals. The CDW order is gradually suppressed by Fe-doping, accompanied by the disappearance of pseudogap/Mott-gap as shown by the density functional theory (DFT) calculations. The superconducting state develops at low temperatures within the CDW state for the samples with the moderate doping levels. The superconductivity strongly depends on xx within a narrow range, and the maximum superconducting transition temperature is 2.8 K as x=0.02x=0.02. We propose that the induced superconductivity and CDW phases are separated in real space. For high doping level (x>0.04x>0.04), the Anderson localization (AL) state appears, resulting in a large increase of resistivity. We present a complete electronic phase diagram of 1TT-Fex_{x}Ta1−x_{1-x}S2_{2} system that shows a dome-like Tc(x)T_{c}(x)

    Anomalous thermoelectric effects of ZrTe5_{5} in and beyond the quantum limit

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    Thermoelectric effects are more sensitive and promising probes to topological properties of emergent materials, but much less addressed compared to other physical properties. Zirconium pentatelluride (ZrTe5_{5}) has inspired active investigations recently because of its multiple topological nature. We study the thermoelectric effects of ZrTe5_{5} in a magnetic field and find several anomalous behaviors. The Nernst response has a steplike profile near zero field when the charge carriers are electrons only, suggesting the anomalous Nernst effect arising from a nontrivial profile of Berry curvature. Both the thermopower and Nernst signal exhibit exotic peaks in the strong-field quantum limit. At higher magnetic fields, the Nernst signal has a sign reversal at a critical field where the thermopower approaches to zero. We propose that these anomalous behaviors can be attributed to the Landau index inversion, which is resulted from the competition of the B\sqrt{B} dependence of the Dirac-type Landau bands and linear-BB dependence of the Zeeman energy (BB is the magnetic field). Our understanding to the anomalous thermoelectric properties in ZrTe5_{5} opens a new avenue for exploring Dirac physics in topological materials.Comment: 6 pages, 4 figure
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