Shape coexistence from lifetime and branching-ratio measurements in 68,70Ni

© 2016 The Author(s) Shape coexistence near closed-shell nuclei, whereby states associated with deformed shapes appear at relatively low excitation energy alongside spherical ones, is indicative of the rapid change in structure that can occur with the addition or removal of a few protons or neutrons. Near 68Ni (Z=28, N=40), the identification of shape coexistence hinges on hitherto undetermined transition rates to and from low-energy 0+ states. In 68,70Ni, new lifetimes and branching ratios have been measured. These data enable quantitative descriptions of the 0+ states through the deduced transition rates and serve as sensitive probes for characterizing their nuclear wave functions. The results are compared to, and consistent with, large-scale shell-model calculations which predict shape coexistence. With the firm identification of this phenomenon near 68Ni, shape coexistence is now observed in all currently accessible regions of the nuclear chart with closed proton shells and mid-shell neutrons

β -decay half-lives of neutron-rich nuclides in the A=100-110 mass region

β-decay half-lives of neutron-rich nuclides in the A=100-110 mass region have been measured using an implantation station installed inside of the Summing NaI(Tl) (SuN) detector at the National Superconducting Cyclotron Laboratory. Accurate half-lives for these nuclides are important for nuclear astrophysics, nuclear structure, and nuclear technology. The half-lives from the present work are compared with previous measurements, showing overall good agreement

Total absorption spectroscopy of the β decay of Zr 101,102 and Tc 109

20 pags., 9 figs., 5 tabs.The β decay of Zr101,102 and Tc109 was studied using the technique of total absorption spectroscopy. The experiment was performed at the National Superconducting Cyclotron Laboratory using the Summing NaI(Tl) (SuN) detector in the first-ever application of total absorption spectroscopy with a fast beam produced via projectile fragmentation. The β-decay feeding intensity and Gamow-Teller transition strength distributions were extracted for these three decays. The extracted distributions were compared to three different quasiparticle random-phase approximation (QRPA) models based on different mean-field potentials. A comparison with calculations from one of the QRPA models was performed to learn about the ground-state shape of the parent nucleus. For Zr101 and Zr102, calculations assuming a pure shape configuration (oblate or prolate) were not able to reproduce the extracted distributions. These results may indicate that some type of mixture between oblate and prolate shapes is necessary to reproduce the extracted distributions. For Tc109, a comparison of the extracted distributions with QRPA calculations suggests a dominant oblate configuration. The other two QRPA models are commonly used to provide β-decay properties in r-process network calculations. This work shows the importance of making comparisons between the experimental and theoretical β-decay distributions, rather than just half-lives and β-delayed neutron emission probabilities, as close to the r-process path as possible.A.A. acknowledges support from the Spanish Ministerio de Economía y Competitividad under Grants No. FPA2011-24553, No. FPA2014-52823-C2-1-P, and No. FPA2017-83946-C2-1-P and the program Severo Ochoa (SEV-2014-0398). P.S. acknowledges support from MCIU/AEI/FEDER,UE (Spain) under Contract No. PGC2018-093636-B-I00. S.V. acknowledges support from Czech Science Foundation Project No. 19-14048 and the Charles University Project No. UNCE/SCI/013. This work was supported by the National Science Foundation under Grants No. PHY 1565546 (NSCL), No. PHY 1430152 (JINA-CEE), and No. PHY 1350234 (CAREER). This material is based upon work supported by the Department of Energy National Nuclear Security Administration through the Nuclear Science and Security Consortium under Awards No. DE-NA0003180 and/or No. DE-NA000097

Search for intruder states in 68Ni and 67Co

The level schemes of 68Ni and 67Co were extended following 70Zninduced deep-inelastic reactions. No evidence for a previously reported proton intruder 0+ state at 2202 keV in 68Ni was found. In 67Co, two new states at 3216 and 3415 keV have been established; additional states associated with the intruder configuration have yet to be identified

Low-spin states and the non-observation of a proposed 2202-keV, 0 + isomer in 68Ni

The low-spin level scheme of 68Ni was investigated with the Gammasphere array following reactions between a 70Zn beam and 238U, 208Pb, and 197Au targets. Spin assignments for some states have been verified through γ-ray angular correlations, including the 0+ assignment for the 2511-keV level. Two previously unknown states at 3302 and 3405 keV have been identified. No evidence was found for a recently reported 216-ns, 0+ isomer at 2202 keV that was attributed to a proton two-particle, two-hole intruder configuration, despite experimental conditions similar to those used in the measurement reporting its discovery

Neutron single-particle strengths at N=40, 42: Neutron knockout from Ni 68,70 ground and isomeric states

The distribution of single-particle strength in Ni67,69 was characterized with one-neutron knockout reactions from intermediate-energy Ni68,70 secondary beams, selectively populating neutron-hole configurations at N=39 and 41, respectively. The spectroscopic strengths deduced from the measured partial cross sections to the individual final states, as tagged by their γ-ray decays, are used to identify and quantify neutron configurations in the wave functions. While Ni69 compares well with shell-model predictions, the results for Ni67 challenge the validity of current effective shell-model Hamiltonians by revealing discrepancies that cannot be explained so far. These results suggest that our understanding of the low-lying states in the neutron-rich, semimagic Ni isotopes may be incomplete and requires further investigation on both the experimental and theoretical sides

Neutron knockout from 68,70Ni ground and isomeric states.

Neutron-rich isotopes are an important source of new information on nuclear physics. Specifically, the spin-isospin components in the nucleon-nucleon (NN) interaction, e.g., the proton-neutron tensor force, are expected to modify shell structure in exotic nuclei. These potential changes in the intrinsic shell structure are of fundamental interest. The study of the excitation energy of states corresponding to specific configurations in even-even isotopes, together with the single-particle character of the first excited states of odd-A, neutron-rich Ni isotopes, probes the evolution of the neutron orbitals around the Fermi surface as a function of the neutron number a step forward in the understanding of the region and the nature of the NN interaction at large N/Z ratios. In an experiment carried out at the National Superconducting Cyclotron Laboratory [1], new spectroscopic information was obtained for 68Ni and the distribution of single-particle strengths in 67,69Ni was characterized by means of single-neutron knockout from 68,70Ni secondary beams. The spectroscopic strengths, deduced from the measured partial cross sections to the individual states tagged by their de-exciting gamma rays, is used to identify and quantify configurations that involve neutron excitations across the N = 40 harmonic oscillator shell closure. The de-excitation γ rays were measured with the GRETINA tracking array [2]. The results challenge the validity of the most current shell-model Hamiltonians and effective interactions, highlighting shortcomings that cannot yet be explained. These results suggest that our understanding of the low-energy states in such nuclei is not complete and requires further investigation

Configuration mixing and relative transition rates between low-spin states in 68Ni

The low-spin level scheme of 68Ni was investigated following two-neutron-knockout and multinucleon-transfer reactions. The energy of the first excited state was determined to be Ex(02+)=1603.5(3) keV. Relative B(E2) transition probabilities were deduced and compared with shell-model calculations using several modern effective interactions. Theory reproduces the data well, but indicates substantial mixing of multi-particle, multi-hole configurations for the lowest observed 0+ and 2 + states

Identification of deformed intruder states in semi-magic Ni 70

The structure of semi-magic 2870Ni42 was investigated following complementary multinucleon-transfer and secondary fragmentation reactions. Changes to the higher-spin, presumed negative-parity states based on observed γ-ray coincidence relationships result in better agreement with shell-model calculations using effective interactions in the neutron f5/2pg9/2 model space. The second 2+ and (4+) states, however, can only be successfully described when proton excitations across the Z=28 shell gap are included. Monte Carlo shell-model calculations suggest that the latter two states are part of a prolate-deformed intruder sequence, establishing an instance of shape coexistence at low excitation energies similar to that observed recently in neighboring Ni68