141 research outputs found
Fluctuating Cu-O-Cu Bond model of high temperature superconductivity in cuprates
Twenty years of extensive research has yet to produce a general consensus on
the origin of high temperature superconductivity (HTS). However, several
generic characteristics of the cuprate superconductors have emerged as the
essential ingredients of and/or constraints on any viable microscopic model of
HTS. Besides a Tc of order 100K, the most prominent on the list include a
d-wave superconducting gap with Fermi liquid nodal excitations, a d-wave
pseudogap with the characteristic temperature scale T*, an anomalous
doping-dependent oxygen isotope shift, nanometer-scale gap inhomogeneity, etc..
The key role of planar oxygen vibrations implied by the isotope shift and other
evidence, in the context of CuO2 plane symmetry and charge constraints from the
strong intra-3d Coulomb repulsion U, enforces an anharmonic mechanism in which
the oxygen vibrational amplitude modulates the strength of the in-plane Cu-Cu
bond. We show, within a Fermi liquid framework, that this mechanism can lead to
strong d-wave pairing and to a natural explanation of the salient features of
HTS
Marginal Fermi liquid analysis of 300 K reflectance of Bi2Sr2CaCu2O8+x
We use 300 K reflectance data to investigate the normal-state electrodynamics
of the high temperature superconductor BiSrCaCuO
over a wide range of doping levels. The data show that at this temperature the
free carriers are coupled to a continuous spectrum of fluctuations. Assuming
the Marginal Fermi Liquid (MFL) form as a first approximation for the
fluctuation spectrum, the doping-dependent coupling constant can
be estimated directly from the slope of the reflectance spectrum. We find that
decreases smoothly with the hole doping level, from underdoped
samples with ( K) where to overdoped
samples with , ( K) where . An analysis of
the intercept and curvature of the reflectance spectrum shows deviations from
the MFL spectrum symmetrically placed at the optimal doping point . The
Kubo formula for the conductivity gives a better fit to the experiments with
the MFL spectrum up to 2000 cm and with an additional Drude component or
an additional Lorentz component up to 7000 cm. By comparing three
different model fits we conclude that the MFL channel is necessary for a good
fit to the reflectance data. Finally, we note that the monotonic variation of
the reflectance slope with doping provides us with an independent measure of
the doping level for the Bi-2212 system.Comment: 11 pages, 11 figure
Coherent quasiparticle weight and its connection to high-T_c superconductivity from angle-resolved photoemission
In conventional superconductors, the pairing energy gap (\Delta) and
superconducting phase coherence go hand-in-hand. As the temperature is lowered,
both the energy gap and phase coherence appear at the transition temperature
T_c. In contrast, in underdoped high-T_c superconductors (HTSCs), a pseudogap
appears at a much higher temperature T^*, smoothly evolving into the
superconducting gap at T_c. Phase coherence on the other hand is only
established at T_c, signaled by the appearance of a sharp quasiparticle (QP)
peak in the excitation spectrum. Another important difference between the two
types of superconductors is in the ratio of 2\Delta / T_c=R. In BCS theory,
R~3.5, is constant. In the HTSCs this ratio varies widely, continuing to
increase in the underdoped region, where the gap increases while T_c decreases.
Here we report that in HTSCs it is the ratio z_A\Delta_m/T_c which is
approximately constant, where \Delta_m is the maximum value of the d-wave gap,
and z_A is the weight of the coherent excitations in the spectral function.
This is highly unusual, since in nearly all phase transitions, T_c is
determined by an energy scale alone. We further show that in the
low-temperature limit, z_{\it A} increases monotonically with increasing doping
x. The growth is linear, i.e. z_A(x)\propto x, in the underdoped to optimally
doped regimes, and slows down in overdoped samples. The reduction of z_A with
increasing temperature resembles that of the c-axis superfluid density.Comment: 11 pages, 5 figures, revised versio
Thermal Conductivity across the Phase Diagram of Cuprates: Low-Energy Quasiparticles and Doping Dependence of the Superconducting Gap
Heat transport in the cuprate superconductors YBaCuO and
LaSrCuO was measured at low temperatures as a function of
doping. A residual linear term kappa_{0}/T is observed throughout the
superconducting region and it decreases steadily as the Mott insulator is
approached from the overdoped regime. The low-energy quasiparticle gap
extracted from kappa_{0}/T is seen to scale closely with the pseudogap. The
ubiquitous presence of nodes and the tracking of the pseudogap shows that the
overall gap remains of the pure d-wave form throughout the phase diagram, which
excludes the possibility of a complex component (ix) appearing at a putative
quantum phase transition and argues against a non-superconducting origin to the
pseudogap. A comparison with superfluid density measurements reveals that the
quasiparticle effective charge is weakly dependent on doping and close to
unity.Comment: 12 pages, 9 figure
Vortex Solid-Liquid Transition in BiSrCaCuO with a High Density of Strong Pins
The introduction of a large density of columnar defects in %underdoped
BiSrCaCuO crystals does not, at sufficiently low
vortex densities, increase the irreversibility line beyond the first order
transition (FOT) field of pristine crystals. At such low fields, the flux line
wandering length behaves as in pristine
%BiSrCaCuO crystals. Next, vortex positional
correlations along the --axis in the vortex Bose glass at fields above the
FOT are smaller than in the low--field vortex solid. Third, the
Bose-glass-to-vortex liquid transition is signaled by a rapid decrease in
c-axis phase correlations. These observations are understood in terms of the
``discrete superconductor'' model.Comment: 4 pages, 4 figures Submitted to Phys. Rev. B Rapid Comm. 16-1-2004
Revised version 18-3-200
Electronic structure of the trilayer cuprate superconductor BiSrCaCuO
The low-energy electronic structure of the trilayer cuprate superconductor
BiSrCaCuO near optimal doping is investigated by
angle-resolved photoemission spectroscopy. The normal state quasiparticle
dispersion and Fermi surface, and the superconducting d-wave gap and coherence
peak are observed and compared with those of single and bilayer systems. We
find that both the superconducting gap magnitude and the relative
coherence-peak intensity scale linearly with for various optimally doped
materials. This suggests that the higher of the trilayer system should be
attributed to parameters that simultaneously enhance phase stiffness and
pairing strength.Comment: 5 pages, 5 figre
Observation of Andreev reflection in the c-axis transport of Bi_2Sr_2CaCu_2O_{8+x} single crystals near T_c and search for the preformed-pair state
We observed an enhancement of the -axis differential conductance around
the zero-bias in AuBiSrCaCuO (Bi2212) junctions near the
superconducting transition temperature . We attribute the conductance
enhancement to the Andreev reflection between the surface Cu-O bilayer with
suppressed superconductivity and the neighboring superconducting inner bilayer.
The continuous evolution from depression to an enhancement of the zero-bias
differential conductance, as the temperature approaches from below,
points to weakening of the barrier strength of the non-superconducting layer
between adjacent Cu-O bilayers. We observed that the conductance enhancement
persisted up to a few degrees above in junctions prepared on slightly
overdoped Bi2212 crystals. However, no conductance enhancement was observed
above in underdoped crystals, although recently proposed theoretical
consideration suggests an even wider temperature range of enhanced zero-bias
conductance. This seems to provide negative perspective to the existence of the
phase-incoherent preformed pairs in the pseudogap state.Comment: 17 pages including 4 figure
Origin of the Pseudogap in High-Temperature Cuprate Superconductors
Cuprate high-temperature superconductors exhibit a pseudogap in the normal
state that decreases monotonically with increasing hole doping and closes at x
\approx 0.19 holes per planar CuO2 while the superconducting doping range is
0.05 < x < 0.27 with optimal Tc at x \approx 0.16. Using ab initio quantum
calculations at the level that leads to accurate band gaps, we found that
four-Cu-site plaquettes are created in the vicinity of dopants. At x \approx
0.05 the plaquettes percolate, so that the Cu dx2y2/O p{\sigma} orbitals inside
the plaquettes now form a band of states along the percolating swath. This
leads to metallic conductivity and below Tc to superconductivity. Plaquettes
disconnected from the percolating swath are found to have degenerate states at
the Fermi level that split and lead to the pseudogap. The pseudogap can be
calculated by simply counting the spatial distribution of isolated plaquettes,
leading to an excellent fit to experiment. This provides strong evidence in
favor of inhomogeneous plaquettes in cuprates.Comment: 24 pages (4 pages main text plus 20 pages supplement
Molecular Identification and Expression Analysis of Filaggrin-2, a Member of the S100 Fused-Type Protein Family
Genes of the S100 fused-type protein (SFTP) family are clustered within the epidermal differentiation complex and encode essential components that maintain epithelial homeostasis and barrier functions. Recent genetic studies have shown that mutations within the gene encoding the SFTP filaggrin cause ichthyosis vulgaris and are major predisposing factors for atopic dermatitis. As a vital component of healthy skin, filaggrin is also a precursor of natural moisturizing factors. Here we present the discovery of a member of this family, designated as filaggrin-2 (FLG2) that is expressed in human skin. The FLG2 gene encodes a histidine- and glutamine-rich protein of approximately 248 kDa, which shares common structural features with other SFTP members, in particular filaggrin. We found that FLG2 transcripts are present in skin, thymus, tonsils, stomach, testis and placenta. In cultured primary keratinocytes, FLG2 mRNA expression displayed almost the same kinetics as that of filaggrin following Ca2+ stimulation, suggesting an important role in molecular regulation of epidermal terminal differentiation. We provide evidences that like filaggrin, FLG2 is initially expressed by upper granular cells, proteolytically processed and deposited in the stratum granulosum and stratum corneum (SC) layers of normal epidermis. Thus, FLG2 and filaggrin may have overlapping and perhaps synergistic roles in the formation of the epidermal barrier, protecting the skin from environmental insults and the escape of moisture by offering precursors of natural moisturizing factors
High-Tc Superconductivity and Antiferromagnetism in Multilayered Copper Oxides - A New Paradigm of Superconducting Mechanism -
High-temperature superconductivity (HTSC) in copper oxides emerges on a
layered CuO2 plane when an antiferromagnetic Mott insulator is doped with
mobile hole carriers. We review extensive studies of multilayered copper oxides
by site-selective nuclear magnetic resonance (NMR), which have uncovered the
intrinsic phase diagram of antiferromagnetism (AFM) and HTSC for a
disorder-free CuO2 plane with hole carriers. We present our experimental
findings such as the existence of the AFM metallic state in doped Mott
insulators, the uniformly mixed phase of AFM and HTSC, and the emergence of
d-wave SC with a maximum Tc just outside a critical carrier density, at which
the AFM moment on a CuO2 plane disappears. These results can be accounted for
by the Mott physics based on the t-J model. The superexchange interaction J_in
among spins plays a vital role as a glue for Cooper pairs or mobile
spin-singlet pairs, in contrast to the phonon-mediated attractive interaction
among electrons established in the Bardeen-Cooper-Schrieffer (BCS) theory. We
remark that the attractive interaction for raising the of HTSC up to
temperatures as high as 160 K is the large J_in (~0.12 eV), which binds
electrons of opposite spins to be on neighboring sites, and that there are no
bosonic glues. It is the Coulomb repulsive interaction U(> 6 eV) among Cu-3d
electrons that plays a central role in the physics behind high-Tc phenomena. A
new paradigm of the SC mechanism opens to strongly correlated electron matter.Comment: 20 pages, 25 figures, Special topics "Recent Developments in
Superconductivity" in J. Phys. Soc. Jpn., Published December 26, 201
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