3 research outputs found
Electrical transport signatures of metallic surface state formation in the strongly-correlated insulator FeSb2
We present local and nonlocal electrical transport measurements of the
correlated insulator FeSb. By employing wiring configurations that
delineate between bulk- and surface-dominated conduction, we reveal the
formation of a metallic surface state in FeSb for temperatures ~K. This result is corroborated by an angular rotation study of this
material's magnetotransport, which also shows signatures of the transition from
bulk- to surface-dominated conduction over the same temperature interval as the
local/nonlocal transport divergence. Notable similarities with the topological
Kondo insulator candidate SmB are discussed
Room Temperature Optically and Magnetically Active Edges in Phosphorene Nanoribbons
Nanoribbons - nanometer wide strips of a two-dimensional material - are a
unique system in condensed matter physics. They combine the exotic electronic
structures of low-dimensional materials with an enhanced number of exposed
edges, where phenomena including ultralong spin coherence times, quantum
confinement and topologically protected states can emerge. An exciting prospect
for this new material concept is the potential for both a tunable
semiconducting electronic structure and magnetism along the nanoribbon edge.
This combination of magnetism and semiconducting properties is the first step
in unlocking spin-based electronics such as non-volatile transistors, a route
to low-energy computing, and has thus far typically only been observed in doped
semiconductor systems and/or at low temperatures. Here, we report the magnetic
and semiconducting properties of phosphorene nanoribbons (PNRs). Static (SQUID)
and dynamic (EPR) magnetization probes demonstrate that at room temperature,
films of PNRs exhibit macroscopic magnetic properties, arising from their edge,
with internal fields of ~ 250 to 800 mT. In solution, a giant magnetic
anisotropy enables the alignment of PNRs at modest sub-1T fields. By leveraging
this alignment effect, we discover that upon photoexcitation, energy is rapidly
funneled to a dark-exciton state that is localized to the magnetic edge and
coupled to a symmetry-forbidden edge phonon mode. Our results establish PNRs as
a unique candidate system for studying the interplay of magnetism and
semiconducting ground states at room temperature and provide a stepping-stone
towards using low-dimensional nanomaterials in quantum electronics.Comment: 18 pages, 4 figure
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Quasi-2D Fermi surface in the anomalous superconductor UTe2
The heavy fermion paramagnet UTe2 exhibits numerous characteristics of spin-triplet superconductivity. Efforts to understand the microscopic details of this exotic superconductivity have been impeded by uncertainty regarding the underlying electronic structure. Here we directly probe the Fermi surface of UTe2 by measuring magnetic quantum oscillations in pristine quality crystals. We find an angular profile of quantum oscillatory frequency and amplitude that is characteristic of a quasi-2D Fermi surface, which we find is well described by two cylindrical Fermi sheets of electron- and hole-type respectively. Additionally, we find that both cylindrical Fermi sheets possess considerable undulation but negligible small-scale corrugation, which may allow for their near-nesting and therefore promote magnetic fluctuations that enhance the triplet pairing mechanism. Importantly, we find no evidence for the presence of any 3D Fermi surface sections. Our results place strong constraints on the possible symmetry of the superconducting order parameter in UTe2