4 research outputs found
The resonant acousto-optic effect
This dissertation is theoretical investigation of the resonant acousto-optic effect in
ionic crystals and thin metal foils. The optical properties of these types of materials,
in the presence of coherent acoustic pump excitation, are numerically modelled and
compared with analytical results.
The resonant acousto-optic effect in bulk ionic materials is shown to be dependent on
the coupling of a bulk acoustic wave to the TO-phonon component of a TO-phonon
polariton. This requires that the material used is not only an ionic crystal but also
has a strongly anharmonic interatomic potential. It is also demonstrated that the
process “TO phonon ± one (two) transverse acoustic phonon(s)→ TO phonon” is
responsible for the cubic (quartic) resonant acousto-optic effect. The role of acoustic
intensity and frequency in the optical properties of CuCl and TlCl is considered.
Higher order transitions are also investigated.
It is shown that, in the ferroelectric material LiNbO3, both cubic and quartic scattering
channels are sufficiently strong enough to consider the resonant acousto-optic
effect associated with them on an equal footing. The coupling strength of both scattering
channels is estimated to the nearest order of magnitude. The cubic coupling is
found be σ3 = 5 meV and the quartic coupling strength is found to be σ4 = 0.3 meV
both for the acoustic intensity Iac = 25 kWcm−2. The effect the phase difference
between the two anharmonic terms has on the optical properties of LiNbO3 is then
investigated. A tunable THz filter is proposed, based on the resonant acousto-optic
effect in LiNbO3.
A numerical method is developed to calculated the partial wave amplitudes and optical
properties of metal foils with acoustically excited, propagating sinusoidally corrugated
surfaces. It is then used on a system of a thin acoustically perturbed Au foil
on a glass substrate. The effects of varying the angle of incidence, acoustic wavevector,
corrugation amplitude and foil thickness are investigated. The numerical method
is shown to remain stable even for strong coupling between the acoustic wave and
surface plasmon polariton
Far-infrared response of acoustically modulated transverse optical-phonon polaritons
The authors propose a scheme to achieve strong modification of the light properties in the terahertz (THz) range and in particular up to 70% changes in the THz reflectivity of CuCl, TlCl and LiNbO3 crystals. This is realised by using transverse optical (TO) phonons as a mediator in the interaction between an acoustic wave (AW) and a THz light field, via the strong anharmonicities of the interatomic potential. Their numerical modeling of CuCl, TlCl and LiNbO3 crystals also predicts that these effects are tunable by applying various coherent AWs from sub-GHz to few GHz frequency. The length of the interaction between electromagnetic and acoustic fields is also greatly reduced compared to conventional acousto-optics. The modifications of the reflectivity spectrum are because of single and multiple intra-branch phonon transitions within the TO-phonon polariton dispersion branches