244 research outputs found
Spin-orbit effects on the Larmor dispersion relation in GaAs quantum wells
We have studied the relevance of spin-orbit coupling to the dispersion 00009
relation of the Larmor resonance observed in inelastic light scattering and
electron-spin resonance experiments on GaAs quantum wells. We show that the
spin-orbit interaction, here described by a sum of Dresselhaus and
Bychkov-Rashba terms, couples Zeeman and spin-density excitations. We have
evaluated its contribution to the spin splitting as a function of the magnetic
field , and have found that in the small limit, the spin-orbit
interaction does not contribute to the spin splitting, whereas at high magnetic
fields it yields a independent contribution to the spin splitting given by
, with being the intensity of the
Bychkov-Rashba and Dresselhaus spin-orbit terms.Comment: To be published in Physical Review
Excited electron-bubble states in superfluid helium-4: a time-dependent density functional approach
We present a systematic study on the excited electron-bubble states in
superfluid helium-4 using a time-dependent density functional approach. For the
evolution of the 1P bubble state, two different functionals accompanied with
two different time-development schemes are used, namely an accurate
finite-range functional for helium with an adiabatic approximation for electron
versus an efficient zero-range functional for helium with a real-time evolution
for electron. We make a detailed comparison between the quantitative results
obtained from the two methods, which allows us to employ with confidence the
optimal method for suitable problems. Based on this knowledge, we use the
finite-range functional to calculate the time-resolved absorption spectrum of
the 1P bubble, which in principle can be experimentally determined, and we use
the zero-range functional to real-time evolve the 2P bubble for several
hundreds of picoseconds, which is theoretically interesting due to the break
down of adiabaticity for this state. Our results discard the physical
realization of relaxed, metastable 2P electron-bubblesComment: 16 pages, 12 figure
Spinning superfluid He-4 nanodroplets
We have studied spinning superfluid He-4 nanodroplets at zero temperature using density functional theory. Due to the irrotational character of the superfluid flow, the shapes of the spinning nanodroplets are very different from those of a viscous normal fluid drop in steady rotation. We show that when vortices are nucleated inside the superfluid droplets, their morphology, which evolves from axisymmetric oblate to triaxial prolate to two-lobed shapes, is in good agreement with experiments. The presence of vortex arrays confers to the superfluid droplets the rigid-body behavior of a normal fluid in steady rotation, and this is the ultimate reason for the surprising good agreement between recent experiments and the classical models used for their description
Rotating 3He droplets
Motivated by recent experiments, we study normal-phase rotating 3He droplets within density functional theory in a semi-classical approach. The sequence of rotating droplet shapes as a function of angular momentum is found to agree with that of rotating classical droplets, evolving from axisymmetric oblate to triaxial prolate to two-lobed shapes as the angular momentum of the droplet increases. Our results, which are obtained for droplets of nanoscopic size, are rescaled to the mesoscopic size characterizing ongoing experimental measurements, allowing for a direct comparison of shapes. The stability curve in the angular velocity-angular momentum plane shows small deviations from the classical rotating drop model predictions, whose magnitude increases with angular momentum. We attribute these deviations to effects not included in the simplified classical model description of a rotating fluid held together by surface tension, i.e., to surface diffuseness, curvature, and finite compressibility, and to quantum effects associated with deformation of the 3He Fermi surface. The influence of all these effects is expected to diminish as the droplet size increases, making the classical rotating droplet model a quite accurate representation of 3He rotation
From quantum dots to quantum wires: electronic structure of semiconductor nanorods
The transition bridge between zero-dimensional quantum dots and one-dimensional quantum wires is explored theoretically by means of the construction of the addition energy spectra of nanorods with different lengths. Spin density-functional theory supplemented with full configuration interaction calculations are carried out. The addition energy spectra are qualitatively related to the single particle correlation diagram. The transition from charge-density waves to spin-density waves, characterizing the Wigner crystallization in the low density limit is show
Multipole modes and spin features in the Raman spectrum of nanoscopic quantum rings
We present a systematic study of ground state and spectroscopic properties of many-electron nanoscopic quantum rings. Addition energies at zero magnetic field (B) and electrochemical potentials as a function of B are given for a ring hosting up to 24 electrons. We find discontinuities in the excitation energies of multipole spin and charge density modes, and a coupling between the charge and spin density responses that allow to identify the formation of ferromagnetic ground states in narrow magnetic field regions. These effects can be observed in Raman experiments, and are related to the fractional Aharonov-Bohm oscillations of the energy and of the persistent current in the rin
Superfluid helium droplet-mediated surface-deposition of neutral and charged silver atomic species.
Experimental and theoretical work has delivered evidence of the helium nanodroplet-mediated synthesis and soft-landing of metal nanoparticles, nanowires, clusters, and single atoms on solid sup- ports. Recent experimental advances have allowed the formation of charged metal clusters into multiply charged helium nanodroplets. The impact of the charge of immersed metal species in helium nanodroplet-mediated surface deposition is proved by considering silver atoms and cations at zero-temperature graphene as the support. By combining high-level ab initio intermolecular inter- action theory with a full quantum description of the superfluid helium nanodroplet motion, evidence is presented that the fundamental mechanism of soft-deposition is preserved in spite of the much stronger interaction of charged species with surfaces, with high-density fluctuations in the helium droplet playing an essential role in braking them. Corroboration is also presented that the soft- landing becomes favored as the helium nanodroplet size increases
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