An automated and versatile ultra-low temperature SQUID magnetometer

We present the design and construction of a SQUID-based magnetometer for operation down to temperatures T = 10 mK, while retaining the compatibility with the sample holders typically used in commercial SQUID magnetometers. The system is based on a dc-SQUID coupled to a second-order gradiometer. The sample is placed inside the plastic mixing chamber of a dilution refrigerator and is thermalized directly by the 3He flow. The movement though the pickup coils is obtained by lifting the whole dilution refrigerator insert. A home-developed software provides full automation and an easy user interface.Comment: RevTex, 10 pages, 10 eps figures. High-resolution figures available upon reques

Decomposition of time-covariant operations on quantum systems with continuous and/or discrete energy spectrum

Every completely positive map G that commutes which the Hamiltonian time evolution is an integral or sum over (densely defined) CP-maps G_\sigma where \sigma is the energy that is transferred to or taken from the environment. If the spectrum is non-degenerated each G_\sigma is a dephasing channel followed by an energy shift. The dephasing is given by the Hadamard product of the density operator with a (formally defined) positive operator. The Kraus operator of the energy shift is a partial isometry which defines a translation on R with respect to a non-translation-invariant measure. As an example, I calculate this decomposition explicitly for the rotation invariant gaussian channel on a single mode. I address the question under what conditions a covariant channel destroys superpositions between mutually orthogonal states on the same orbit. For channels which allow mutually orthogonal output states on the same orbit, a lower bound on the quantum capacity is derived using the Fourier transform of the CP-map-valued measure (G_\sigma).Comment: latex, 33 pages, domains of unbounded operators are now explicitly specified. Presentation more detailed. Implementing the shift after the dephasing is sometimes more convenien

Quantum Magnetic Deflagration in Mn12 Acetate

We report controlled ignition of magnetization reversal avalanches by surface acoustic waves in a single crystal of Mn12 acetate. Our data show that the speed of the avalanche exhibits maxima on the magnetic field at the tunneling resonances of Mn12. Combined with the evidence of magnetic deflagration in Mn12 acetate (Suzuki et al., cond-mat/0506569) this suggests a novel physical phenomenon: deflagration assisted by quantum tunneling.Comment: 4 figure

Dynamics of Metal Centers Monitored by Nuclear Inelastic Scattering

Nuclear inelastic scattering of synchrotron radiation has been used now since 10 years as a tool for vibrational spectroscopy. This method has turned out especially useful in case of large molecules that contain a M\"ossbauer active metal center. Recent applications to iron-sulfur proteins, to iron(II) spin crossover complexes and to tin-DNA complexes are discussed. Special emphasis is given to the combination of nuclear inelastic scattering and density functional calculations

Decision-Making Under Risk in Children, Adolescents, and Young Adults

Adolescents often make risky and impulsive decisions. Such behavior has led to the common assumption that a dysfunction in risk-related decision-making peaks during this age. Differences in how risk has been defined across studies, however, make it difficult to draw conclusions about developmental changes in risky decision-making. Here, we developed a non-symbolic economic decision-making task that can be used across a wide age span and that uses coefficient of variation (CV) in reward as an index of risk. We found that young children showed the strongest preference for risky compared to sure bet options of equal expected value, adolescents were intermediate in their risk preference, and young adults showed the strongest risk aversion. Furthermore, children's preference for the risky option increased for larger CVs, while adolescents and young adults showed the opposite pattern, favoring the sure bet more often as CV increased. Finally, when faced with two gambles in a risk–return tradeoff, all three age groups exhibited a greater preference for the option with the lower risk and return as the disparity in risk between the two options increased. These findings demonstrate clear age-related differences in economic risk preferences that vary with choice set and risk. Importantly, adolescence appears to represent an intermediate decision-making phenotype along the transition from childhood to adulthood, rather than an age of heightened preference for economic risk

Pressure Evolution of the Magnetic Field induced Ferromagnetic Fluctuation through the Pseudo-Metamagnetism of CeRu2Si2

Resistivity measurements performed under pressure in the paramagnetic ground state of CeRu2Si2 are reported. They demonstrate that the relative change of effective mass through the pseudo metamagnetic transition is invariant under pressure. The results are compared with the first order metamagnetic transition due to the antiferromagnetism of Ce0.9La0.1Ru2Si2 which corresponds to the "negative" pressure of CeRu2Si2 by volume expansion. Finally, we describe the link between the spin-depairing of quasiparticles on CeRu2Si2 and that of Cooper pairs on the unconventional heavy fermion superconductor CeCoIn5.Comment: 5 pages, 6 figures, accepted for publication in J. Phys. Soc. Jp

Low-Temperature Quantum Relaxation in a System of Magnetic Nanomolecules

We argue that to explain recent resonant tunneling experiments on crystals of Mn$_{12}$ and Fe$_8$, particularly in the low-T limit, one must invoke dynamic nuclear spin and dipolar interactions. We show the low-$T$, short-time relaxation will then have a $\sqrt{t/\tau}$ form, where $\tau$ depends on the nuclear $T_2$, on the tunneling matrix element $\Delta_{10}$ between the two lowest levels, and on the initial distribution of internal fields in the sample, which depends very strongly on sample shape. The results are directly applicable to the $Fe_8$ system. We also give some results for the long-time relaxation.Comment: 4 pages, 3 PostScript figures, LaTe

Resonant Magnetization Tunneling in Mn12 Acetate: The Absence of Inhomogeneous Hyperfine Broadening

We present the results of a detailed study of the thermally-assisted-resonant-tunneling relaxation rate of Mn12 acetate as a function of an external, longitudinal magnetic field and find that the data can be fit extremely well to a Lorentzian function. No hint of inhomogeneous broadening is found, even though some is expected from the Mn nuclear hyperfine interaction. This inconsistency implies that the tunneling mechanism cannot be described simply in terms of a random hyperfine field.Comment: Some minor revisions, title changed, updated figures, two added notes, one added reference. RevTeX, 4 pages, 3 postscript figures. Submitted to Rapid Communication

Zinc stress induces copper depletion in Acinetobacter baumannii

Background: The first row transition metal ions zinc and copper are essential to the survival of many organisms, although in excess these ions are associated with significant toxicity. Here, we examined the impact of zinc and copper stress on Acinetobacter baumannii, a common opportunistic pathogen. Results: We show that extracellular zinc stress induces a copper-specific depletion phenotype in A. baumannii ATCC 17978. Supplementation with copper not only fails to rescue this phenotype, but further exacerbates the copper depletion. Extensive analysis of the A. baumannii ATCC 17978 genome identified 13 putative zinc/copper resistance efflux pumps. Transcriptional analyses show that four of these transporters are responsive to zinc stress, five to copper stress and seven to the combination of zinc and copper stress, thereby revealing a likely foundation for the zinc-induced copper starvation in A. baumannii. In addition, we show that zinc and copper play crucial roles in management of oxidative stress and the membrane composition of A. baumannii. Further, we reveal that zinc and copper play distinct roles in macrophage-mediated killing of this pathogen. Conclusions: Collectively, this study supports the targeting of metal ion homeostatic mechanisms as an effective antimicrobial strategy against multi-drug resistant bacterial pathogens.Karl A. Hassan, Victoria G. Pederick, Liam D. H. Elbourne, Ian T. Paulsen, James C. Paton, Christopher A. McDevitt and Bart A. Eijkelkam

Low temperature microwave emission from molecular clusters

We investigate the experimental detection of the electromagnetic radiation generated in the fast magnetization reversal in Mn12-acetate at low temperatures. In our experiments we used large single crystals and assemblies of several small single crystals of Mn12-acetate placed inside a cylindrical stainless steel waveguide in which an InSb hot electron device was also placed to detect the radiation. All this was set inside a SQUID magnetometer that allowed to change the magnetic field and measure the magnetic moment and the temperature of the sample as the InSb detected simultaneously the radiation emitted from the molecular magnets. Our data show a sequential process in which the fast inversion of the magnetic moment first occurs, then the radiation is detected by the InSb device, and finally the temperature of the sample increases during 15 ms to subsequently recover its original value in several hundreds of milliseconds.Comment: changed conten