Relaxation to non-equilibrium in expanding ultracold neutral plasmas

We investigate the strongly correlated ion dynamics and the degree of coupling achievable in the evolution of freely expanding ultracold neutral plasmas. We demonstrate that the ionic Coulomb coupling parameter $\Gamma_{\rm i}$ increases considerably in later stages of the expansion, reaching the strongly coupled regime despite the well-known initial drop of $\Gamma_{\rm i}$ to order unity due to disorder-induced heating. Furthermore, we formulate a suitable measure of correlation and show th at $\Gamma_{\rm i}$ calculated from the ionic temperature and density reflects the degree of order in the system if it is sufficiently close to a quasisteady state. At later times, however, the expansion of the plasma cloud becomes faster than the relaxation of correlations, and the system does not reach thermodynamic equilibrium anymore

Influence of electron-ion collisions on Coulomb crystallization of ultracold neutral plasmas

While ion heating by elastic electron-ion collisions may be neglected for a description of the evolution of freely expanding ultracold neutral plasmas, the situation is different in scenarios where the ions are laser-cooled during the system evolution. We show that electron-ion collisions in laser-cooled plasmas influence the ionic temperature, decreasing the degree of correlation obtainable in such systems. However, taking into account the collisions increases the ion temperature much less than what would be estimated based on static plasma clouds neglecting the plasma expansion. The latter leads to both adiabatic cooling of the ions as well as, more importantly, a rapid decrease of the collisional heating rate

Ultracold Neutral Plasmas

Ultracold neutral plasmas, formed by photoionizing laser-cooled atoms near the ionization threshold, have electron temperatures in the 1-1000 kelvin range and ion temperatures from tens of millikelvin to a few kelvin. They represent a new frontier in the study of neutral plasmas, which traditionally deals with much hotter systems, but they also blur the boundaries of plasma, atomic, condensed matter, and low temperature physics. Modelling these plasmas challenges computational techniques and theories of non-equilibrium systems, so the field has attracted great interest from the theoretical and computational physics communities. By varying laser intensities and wavelengths it is possible to accurately set the initial plasma density and energy, and charged-particle-detection and optical diagnostics allow precise measurements for comparison with theoretical predictions. Recent experiments using optical probes demonstrated that ions in the plasma equilibrate in a strongly coupled fluid phase. Strongly coupled plasmas, in which the electrical interaction energy between charged particles exceeds the average kinetic energy, reverse the traditional energy hierarchy underlying basic plasma concepts such as Debye screening and hydrodynamics. Equilibration in this regime is of particular interest because it involves the establishment of spatial correlations between particles, and it connects to the physics of the interiors of gas-giant planets and inertial confinement fusion devices.Comment: 89 pages, 54 image

Kinetic modelling and molecular dynamics simulation of ultracold neutral plasmas including ionic correlations

A kinetic approach for the evolution of ultracold neutral plasmas including interionic correlations and the treatment of ionization/excitation and recombination/deexcitation by rate equations is described in detail. To assess the reliability of the approximations inherent in the kinetic model, we have developed a hybrid molecular dynamics method. Comparison of the results reveals that the kinetic model describes the atomic and ionic observables of the ultracold plasma surprisingly well, confirming our earlier findings concerning the role of ion-ion correlations [Phys. Rev. A {\bf 68}, 010703]. In addition, the molecular dynamics approach allows one to study the relaxation of the ionic plasma component towards thermodynamical equilibrium

Universal shape function for the double ionization cross section of negative ions by electron impact

It is shown that recently measured cross sections for double ionization of negative ions ($H^-, O^-$, and $C^-$) possess a universal shape when plotted in suitable dimensionless units. The shape can be represented with a simple analytical function, following the same principles as it has been done in establishing a universal shape function for single ionization [Rost and Pattard 1997 Phys. Rev. A {\bf 55} R5]. Thereby, it is demonstrated that direct double ionization dominates the cross section for the targets considered

Many-body theory of excitation dynamics in an ultracold Rydberg gas

We develop a theoretical approach for the dynamics of Rydberg excitations in ultracold gases, with a realistically large number of atoms. We rely on the reduction of the single-atom Bloch equations to rate equations, which is possible under various experimentally relevant conditions. Here, we explicitly refer to a two-step excitation-scheme. We discuss the conditions under which our approach is valid by comparing the results with the solution of the exact quantum master equation for two interacting atoms. Concerning the emergence of an excitation blockade in a Rydberg gas, our results are in qualitative agreement with experiment. Possible sources of quantitative discrepancy are carefully examined. Based on the two-step excitation scheme, we predict the occurrence of an antiblockade effect and propose possible ways to detect this excitation enhancement experimentally in an optical lattice as well as in the gas phase.Comment: 12 pages, 8 figure

On the role of shake-off in single-photon double ionization

The role of shake-off for double ionization of atoms by a single photon with finite energy has become the subject of debate. In this letter, we attempt to clarify the meaning of shake-off at low photon energies by comparing different formulations appearing in the literature and by suggesting a working definition. Moreover, we elaborate on the foundation and justification of a mixed quantum-classical ansatz for the calculation of single-photon double ionization

Coulomb crystallization in expanding laser-cooled neutral plasmas

We present long-time simulations of expanding ultracold neutral plasmas, including a full treatment of the strongly coupled ion dynamics. Thereby, the relaxation dynamics of the expanding laser-cooled plasma is studied, taking into account elastic as well as inelastic collisions. It is demonstrated that, depending on the initial conditions, the ionic component of the plasma may exhibit short-range order or even a superimposed long-range order resulting in concentric ion shells. In contrast to ionic plasmas confined in traps, the shell structures are built up from the center of the plasma cloud rather than from the periphery