Repulsive Casimir forces between solid materials with high refractive index intervening liquids

In order to explore repulsive Casimir/van der Waals forces between solid materials with liquid as the intervening medium, we analyze dielectric data for a wide range of materials as for example PTFE, polystyrene, silica and more than twenty liquids. Although significant variation in the dielectric data from different sources exist, we provide a scheme based on measured static dielectric constants, refractive indices, and applying Kramers Kronig (KK) consistency to dielectric data to create accurate dielectric functions at imaginary frequencies. The latter is necessary for more accurate force calculations via the Lifshitz theory allowing reliable predictions of repulsive Casimir forces.Comment: 20 pages, 7 figures, 1 tabl

Tuning near field radiative heat flux through surface excitations with a metal insulator transition

The control of heat flow is a formidable challenge due to lack of good thermal insulators. Promising new oppor-tunities for heat flow control were recently theoretically discovered for radiative heat flow in near field, where large heat flow contrasts may be achieved by tuning electronic excitations on surfaces. Here we show experi-mentally that the phase transition of VO2 entails a change of surface polariton states that significantly affects radiative heat transfer in near field. In all cases the Derjaguin approximation correctly predicted radiative heat transfer in near field, but it underestimated the farfield limit. Our results indicate that heat flow contrasts can be realized in near field that can be larger than those obtained in farfield.Comment: 3 figure

Experimental observation of nanoscale radiative heat flow due to surface plasmons in graphene and doped silicon

Owing to its two dimensional electronic structure, graphene exhibits many unique properties. One of them is a wave vector and temperature dependent plasmon in the infrared range. Theory predicts that due to these plasmons, graphene can be used as a universal material to enhance nanoscale radiative heat exchange for any dielectric substrate. Here we report on radiative heat transfer experiments between SiC and a SiO2 sphere which have non matching phonon polariton frequencies, and thus only weakly exchange heat in near field. We observed that the heat flux contribution of graphene epitaxially grown on SiC dominates at short distances. The influence of plasmons on radiative heat transfer is further supported with measurements for doped silicon. These results highlight graphenes strong potential in photonic nearfield and energy conversion devices.Comment: 4 pages, 3 figure

Weak dispersive forces between glass-gold macroscopic surfaces in alcohols

In this work we concentrate on an experimental validation of the Lifshitz theory for van der Waals and Casimir forces in gold-alcohol-glass systems. From this theory weak dispersive forces are predicted when the dielectric properties of the intervening medium become comparable to one of the interacting surfaces. Using inverse colloid probe atomic force microscopy dispersive forces were measured occasionally and under controlled conditions by addition of salt to screen the electrostatic double layer force if present. The dispersive force was found to be attractive, and an order of magnitude weaker than that in air. Although the theoretical description of the forces becomes less precise for these systems even with full knowledge of the dielectric properties, we find still our results in reasonable agreement with Lifshitz theory.Comment: 19 pages, 7 figure

Influence of random roughness on the adhesion between metal surfaces due to capillary condensation

The capillary force was measured by atomic force microscopy between a gold coated sphere mounted on a cantilever and gold surfaces with different roughness. For smooth surfaces the capillary adhesive force surpasses in magnitude any dispersion, e.g. van der Waals/Casimir, and/or electrostatic forces. A substantial decrease in the capillary force was observed by increasing the roughness ampltitude a few nanometers between 1-10 nm. From these measurements two limits can be defined: a smooth limit where a closely macroscopic size contact surface interacts through the capillary force, and the rough limit where only a few asperities give a capillary contribution.Comment: 8 pages, 3 figures, To appear in Appl. Phys. Lett. (2007

Roughness corrections to the Casimir force: The importance of local surface slope

This paper concentrates on a study where finite conductivity corrections are included in the theoretical description of the effects of roughness on the Casimir force. The roughness data were taken from gold films evaporated onto Silicon and polysterene spheres. We conclude that for a detailed comparison with experimental data, i.e. at the level of at least 5 % at short separations below 200 nm, the lateral dimensions of roughness for real films should be included in the theoretical considerations. Moreover, if the RMS roughness is considerable, high local surface slopes are shown to have a significant effect on the Casimir force.Comment: 13 pages. To be publishe

Transition from Casimir to van der Waals force between macroscopic bodies

The transition of van der Waals to Casimir forces between macroscopic gold surfaces is investigated by Atomic Force Microscopy in the plane-sphere geometry. It was found that the transition appears to take place at separations about 10 % the plasma wavelength for evaporated gold surfaces, which compares to theoretical predictions by incorporation of experimental optical data and roughness corrections. Moreover, the force data allow estimation of the Hamaker constant AH in the van der Waals regime, which is in good agreement with the Lifshitz theory predictions (even if roughness corrections are taken into account) and former surface force apparatus measurements.Comment: 12 pages, 3 figure