Disproportionation Transition at Critical Interaction Strength: Na1/2_{1/2}CoO2_2

Charge disproportionation (CD) and spin differentiation in Na$_{1/2}$CoO$_2$ are studied using the correlated band theory approach. The simultaneous CD and gap opening seen previously is followed through a first order charge disproportionation transition 2Co$^{3.5+} \to$ Co$^{3+}$+Co$^{4+}$, whose ionic identities are connected more closely to spin (S=0, S=1/2 respectively) than to real charge. Disproportionation in the Co $a_g$ orbital is compensated by opposing charge rearrangement in other 3d orbitals. At the transition large and opposing discontinuities in the (all-electron) kinetic and potential energies are slightly more than balanced by a gain in correlation energy. The CD state is compared to characteristics of the observed charge-ordered insulating phase in Na$_{1/2}$CoO$_2$, suggesting the Coulomb repulsion value $U$ is concentration-dependent, with $U(x=1/2)\simeq$3.5 eV.Comment: 4 pages and 4 embedded figure

Coherent control of magnetization precession in ferromagnetic semiconductor (Ga,Mn)As

We report single-color, time resolved magneto-optical measurements in ferromagnetic semiconductor (Ga,Mn)As. We demonstrate coherent optical control of the magnetization precession by applying two successive ultrashort laser pulses. The magnetic field and temperature dependent experiments reveal the collective Mn-moment nature of the oscillatory part of the time-dependent Kerr rotation, as well as contributions to the magneto-optical signal that are not connected with the magnetization dynamics.Comment: 6 pages, 3 figures, accepted in Applied Physics Letter

Laser-induced Precession of Magnetization in GaMnAs

We report on the photo-induced precession of the ferromagnetically coupled Mn spins in (Ga,Mn)As, which is observed even with no external magnetic field applied. We concentrate on various experimental aspects of the time-resolved magneto-optical Kerr effect (TR-MOKE) technique that can be used to clarify the origin of the detected signals. We show that the measured data typically consist of several different contributions, among which only the oscillatory signal is directly connected with the ferromagnetic order in the sample.Comment: 4 pages, 5 figure

Pressure on charged domain walls and additional imprint mechanism in ferroelectrics

The impact of free charges on the local pressure on a charged ferroelectric domain wall produced by an electric field has been analyzed. A general formula for the local pressure on a charged domain wall is derived considering full or partial compensation of bound polarization charges by free charges. It is shown that the compensation can lead to a very strong reduction of the pressure imposed on the wall from the electric field. In some cases this pressure can be governed by small nonlinear effects. It is concluded that the free charge compensation of bound polarization charges can lead to substantial reduction of the domain wall mobility even in the case when the mobility of free charge carriers is high. This mobility reduction gives rise to an additional imprint mechanism which may play essential role in switching properties of ferroelectric materials. The effect of the pressure reduction on the compensated charged domain walls is illustrated for the case of 180-degree ferroelectric domain walls and of 90-degree ferroelectric domain walls with the head-to-head configuration of the spontaneous polarization vectors.Comment: subm. to PRB. This verion is extended by appendi

Spin-dependent phenomena and device concepts explored in (Ga,Mn)As

Over the past two decades, the research of (Ga,Mn)As has led to a deeper understanding of relativistic spin-dependent phenomena in magnetic systems. It has also led to discoveries of new effects and demonstrations of unprecedented functionalities of experimental spintronic devices with general applicability to a wide range of materials. In this article we review the basic material properties that make (Ga,Mn)As a favorable test-bed system for spintronics research and discuss contributions of (Ga,Mn)As studies in the general context of the spin-dependent phenomena and device concepts. Special focus is on the spin-orbit coupling induced effects and the reviewed topics include the interaction of spin with electrical current, light, and heat.Comment: 47 pages, 41 figure

Magnetization dynamics in the single-molecule magnet Fe8 under pulsed microwave irradiation

We present measurements on the single molecule magnet Fe8 in the presence of pulsed microwave radiation at 118 GHz. The spin dynamics is studied via time resolved magnetization experiments using a Hall probe magnetometer. We investigate the relaxation behavior of magnetization after the microwave pulse. The analysis of the experimental data is performed in terms of different contributions to the magnetization after-pulse relaxation. We find that the phonon bottleneck with a characteristic relaxation time of 10 to 100 ms strongly affects the magnetization dynamics. In addition, the spatial effect of spin diffusion is evidenced by using samples of different sizes and different ways of the sample's irradiation with microwaves.Comment: 14 pages, 12 figure