Conversion of glassy antiferromagnetic-insulating phase to equilibrium ferromagnetic-metallic phase by devitrification and recrystallization in Al substituted Pr0.5{_{0.5}}Ca0.5_{0.5}MnO3{_3}

We show that Pr${_{0.5}}$Ca$_{0.5}$MnO${_3}$ with 2.5% Al substitution and La${_{0.5}}$Ca$_{0.5}$MnO${_3}$ (LCMO) exhibit qualitatively similar and visibly anomalous M-H curves at low temperature. Magnetic field causes a broad first-order but irreversible antiferromagnetic (AF)-insulating (I) to ferromagnetic (FM)-metallic (M) transition in both and gives rise to soft FM state. However, the low temperature equilibrium state of Pr$_{0.5}$Ca$_{0.5}$Mn$_{0.975}$Al$_{0.025}$O$_3$ (PCMAO) is FM-M whereas that of LCMO is AF-I. In both the systems the respective equilibrium phase coexists with the other phase with contrasting order, which is not in equilibrium, and the cooling field can tune the fractions of the coexisting phases. It is shown earlier that the coexisting FM-M phase behaves like `magnetic glass' in LCMO. Here we show from specially designed measurement protocols that the AF-I phase of PCMAO has all the characteristics of magnetic glassy states. It devitrifies on heating and also recrystallizes to equilibrium FM-M phase after annealing. This glass-like AF-I phase also shows similar intriguing feature observed in FM-M magnetic glassy state of LCMO that when the starting coexisting fraction of glass is larger, successive annealing results in larger fraction of equilibrium phase. This similarity between two manganite systems with contrasting magnetic orders of respective glassy and equilibrium phases points toward a possible universality.Comment: Highlights potential of CHUF (Cooling and Heating in Unequal Fields), a new measurement protoco

Erasing Distinguishability Using Quantum Frequency Up-Conversion

The frequency distinguishability of two single photons was successfully erased using single photon frequency up-conversion. A frequency non-degenerate photon pair generated via spontaneous four-wave mixing in a dispersion shifted fiber was used to emulate two telecom-band single photons that were in the same temporal mode but in different frequency modes. The frequencies of these photons were converted to the same frequency by using the sum frequency generation process in periodically poled lithium niobate waveguides, while maintaining their temporal indistinguishability. As a result, the two converted photons exhibited a non-classical dip in a Hong-Ou-Mandel quantum interference experiment. The present scheme will add flexibility to networking quantum information systems that use photons with various wavelengths.Comment: 4 pages, 5 figure