44 research outputs found
Neutron scattering study of magnetic phase separation in nanocrystalline LaCaMnO
We demonstrate that magnetic phase separation and competing spin order in the
colossal magnetoresistive (CMR) manganites can be directly explored via tuning
strain in bulk samples of nanocrystalline LaCaMnO. Our results
show that strain can be reversibly frozen into the lattice in order to
stabilize coexisting antiferromagnetic domains within the nominally
ferromagnetic metallic state of LaCaMnO. The measurement of
tunable phase separation via magnetic neutron powder diffraction presents a
direct route of exploring the correlated spin properties of phase separated
charge/magnetic order in highly strained CMR materials and opens a potential
avenue for realizing intergrain spin tunnel junction networks with enhanced CMR
behavior in a chemically homogeneous material.Comment: 6 pages, 4 figures. New figure and text added to manuscrip
Spin ordering and electronic texture in the bilayer iridate SrIrO
Through a neutron scattering, charge transport, and magnetization study, the
correlated ground state in the bilayer iridium oxide SrIrO is
explored. Our combined results resolve scattering consistent with a high
temperature magnetic phase that persists above 600 K, reorients at the
previously defined K, and coexists with an electronic ground state
whose phase behavior suggests the formation of a fluctuating charge or orbital
phase that freezes below K. Our study provides a window into
the emergence of multiple electronic order parameters near the boundary of the
metal to insulator phase transition of the 5d Mott phase.Comment: Revised text and figures. 4 pages, 4 figure
Experimental Determination of the Lorenz Number in Cu0.01Bi2Te2.7Se0.3 and Bi0.88Sb0.12
Nanostructuring has been shown to be an effective approach to reduce the
lattice thermal conductivity and improve the thermoelectric figure of merit.
Because the experimentally measured thermal conductivity includes contributions
from both carriers and phonons, separating out the phonon contribution has been
difficult and is mostly based on estimating the electronic contributions using
the Wiedemann-Franz law. In this paper, an experimental method to directly
measure electronic contributions to the thermal conductivity is presented and
applied to Cu0.01Bi2Te2.7Se0.3, [Cu0.01Bi2Te2.7Se0.3]0.98Ni0.02, and
Bi0.88Sb0.12. By measuring the thermal conductivity under magnetic field,
electronic contributions to thermal conductivity can be extracted, leading to
knowledge of the Lorenz number in thermoelectric materials
Band structure of SnTe studied by Photoemission Spectroscopy
We present an angle-resolved photoemission spectroscopy study of the
electronic structure of SnTe, and compare the experimental results to ab initio
band structure calculations as well as a simplified tight-binding model of the
p-bands. Our study reveals the conjectured complex Fermi surface structure near
the L-points showing topological changes in the bands from disconnected
pockets, to open tubes, and then to cuboids as the binding energy increases,
resolving lingering issues about the electronic structure. The chemical
potential at the crystal surface is found to be 0.5eV below the gap,
corresponding to a carrier density of p =1.14x10^{21} cm^{-3} or 7.2x10^{-2}
holes per unit cell. At a temperature below the cubic-rhombohedral structural
transition a small shift in spectral energy of the valance band is found, in
agreement with model predictions.Comment: 4 figure