391 research outputs found
Pressure-Induced Magnetic Quantum Phase Transitions from Gapped Ground State in TlCuCl3
Magnetization maesurements under hydrostatic pressure were performed on an
S=1/2 coupled spin system TlCuCl3 with a gapped ground state under magnetic
field H parallel to the [2,0,1] direction. With increasing applied pressure P,
the gap decreases and closes completely at Pc=0.42 kbar. For P>Pc, TlCuCl3
undergoes antiferromagnetic ordering. A spin-flop transition was observed at
Hsf=0.7T. The spin-flop field is approximately independent of pressure,
although the sublattice magnetization increases with pressure. The gap and Neel
temperature are presented as function is attributed to to the relative
enhancement of the interdimer exchange interactions compared with the
intradimer exchange interaction.Comment: 4pages,3figures To be published in J. Phys. Soc. Jpn. Vol.73 No.1
Neutron Scattering Study of Magnetic Ordering and Excitations in the Doped Spin Gap System Tl(CuMg)Cl
Neutron elastic and inelastic scattering measurements have been performed in
order to investigate the spin structure and the magnetic excitations in the
impurity-induced antiferromagnetic ordered phase of the doped spin gap system
Tl(CuMg)Cl with . The magnetic Bragg reflections
indicative of the ordering were observed at with integer
and odd below K. It was found that the spin structure
of the impurity-induced antiferromagnetic ordered phase on average in
Tl(CuMg)Cl with is the same as that of the
field-induced magnetic ordered phase for in the parent
compound TlCuCl. The triplet magnetic excitation was clearly observed in
the - plane and the dispersion relations of the triplet excitation
were determined along four different directions. The lowest triplet excitation
corresponding to the spin gap was observed at with integer
and odd , as observed in TlCuCl. It was also found that the spin gap
increases steeply below upon decreasing temperature. This strongly
indicates that the impurity-induced antiferromagnetic ordering coexists with
the spin gap state in Tl(CuMg)Cl with .Comment: 24 pages, 7 figures, 11 eps files, revtex style, will appear in Phys.
Rev.
Random Bond Effect in the Quantum Spin System (TlK)CuCl
The effect of exchange bond randomness on the ground state and the
field-induced magnetic ordering was investigated through magnetization
measurements in the spin-1/2 mixed quantum spin system
(TlK)CuCl for . Both parent compounds TlCuCl and
KCuCl are coupled spin dimer systems, which have the singlet ground state
with excitation gaps K and 31 K, respectively. Due to
bond randomness, the singlet ground state turns into the magnetic state with
finite susceptibility, nevertheless, the excitation gap remains. Field-induced
magnetic ordering, which can be described by the Bose condensation of excited
triplets, magnons, was observed as in the parent systems. The phase transition
temperature is suppressed by the bond randomness. This behavior may be
attributed to the localization effect.Comment: 19 pages, 7 figures, 12 eps files, revtex, will appear in PR
Impurity-Induced Antiferromagnetic Ordering in the Spin Gap System TlCuCl_3
The magnetization measurements have been performed on the doped spin gap
system TlCu_{1-x}Mg_xCl_3 with x <= 0.025. The parent compound TlCuCl_3 is a
three-dimensional coupled spin dimer system with the excitation gap Delta/k_B =
7.7 K. The impurity-induced antiferromagnetic ordering was clearly observed.
The easy axis lies in the (0,1,0) plane. It was found that the transition
temperature increases with increasing Mg^{2+} concentration x, while the
spin-flop transition field is almost independent of x. The magnetization curve
suggests that the impurity-induced antiferromagnetic ordering coexists with the
spin gap for x <= 0.017.Comment: 5 pages, 6 figures, revtex styl
Spin-resonance modes of the spin-gap magnet TlCuCl_3
Three kinds of magnetic resonance signals were detected in crystals of the
spin-gap magnet TlCuCl_3.
First, we have observed the microwave absorption due to the excitation of the
transitions between the singlet ground state and the excited triplet states.
This mode has the linear frequency-field dependence corresponding to the
previously known value of the zero-field spin-gap of 156 GHz and to the closing
of spin-gap at the magnetic field H_c of about 50 kOe.
Second, the thermally activated resonance absorption due to the transitions
between the spin sublevels of the triplet excitations was found. These
sublevels are split by the crystal field and external magnetic field.
Finally, we have observed antiferromagnetic resonance absorption in the
field-induced antiferromagnetic phase above the critical field H_c. This
resonance frequency is strongly anisotropic with respect to the direction of
the magnetic field.Comment: v.2: typo correction (one of the field directions was misprinted in
the v.1
Observation of Field-Induced Transverse N\'{e}el Ordering in the Spin Gap System TlCuCl
Neutron elastic scattering experiments have been performed on the spin gap
system TlCuCl in magnetic fields parallel to the -axis. The magnetic
Bragg peaks which indicate the field-induced N\'{e}el ordering were observed
for magnetic field higher than the gap field T at with odd in the plane. The spin structure in the ordered
phase was determined. The temperature and field dependence of the Bragg peak
intensities and the phase boundary obtained were discussed in connection with a
recent theory which describes the field-induced N\'{e}el ordering as a
Bose-Einstein condensation of magnons.Comment: 4 pages, 5 eps figures, jpsj styl
Softening of Magnetic Excitations Leading to Pressure-Induced Quantum Phase Transition in Gapped Spin System KCuCl
KCuCl is a three dimensionally coupled spin dimer system, which undergoes
a pressure-induced quantum phase transition from a gapped ground state to an
antiferromagnetic state at a critical pressure of kbar.
Magnetic excitations in KCuCl at a hydrostatic pressure of 4.7 kbar have
been investigated by conducting neutron inelastic scattering experiments using
a newly designed cylindrical high-pressure clamp cell. A well-defined single
excitation mode is observed. The softening of the excitation mode due to the
applied pressure is clearly observed. From the analysis of the dispersion
relations, it is found that an intradimer interaction decreases under
hydrostatic pressure, while most interdimer interactions increase.Comment: 4 pages, 5 figures, 1 table, jpsj2.cls, to be published in J. Phys.
Soc. Jpn. Vol.76 (2007), the graphic problem of Fig.2 was fixe
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