254 research outputs found
Observation of Modulated Quadrupolar Structures in PrPb3
Neutron diffraction measurements have been performed on the cubic compound
PrPb3 in a [001] magnetic field to examine the quadrupolar ordering.
Antiferromagnetic components with q=(1/2+-d 1/2 0), (1/2 1/2+-d 0) (d~1/8) are
observed below the transition temperature TQ (0.4 K at H=0) whose amplitudes
vary linear with H and vanish at zero field, providing the first evidence for a
modulated quadrupolar phase. For H<1 T, a non-square modulated state persists
even below 100 mK suggesting quadrupole moments associated with a Gamma3
doublet ground state to be partially quenched by hybridization with conduction
electrons.Comment: Physical Review Letters, in press. 4 pages, 4 figure
Antiferro-quadrupole state of orbital-degenerate Kondo lattice model with f^2 configuration
To clarify a key role of orbitals in the emergence of
antiferro-quadrupole structure in PrPb, we investigate the ground-state
property of an orbital-degenerate Kondo lattice model by numerical
diagonalization techniques. In PrPb, Pr has a
configuration and the crystalline-electric-field ground state is a non-Kramers
doublet . In a - coupling scheme, the state is
described by two local singlets, each of which consists of two electrons
with one in and another in orbitals. Since in a cubic
structure, has localized nature, while orbitals are
rather itinerant, we propose the orbital-degenerate Kondo lattice model for an
effective Hamiltonian of PrPb. We show that an antiferro-orbital state is
favored by the so-called double-exchange mechanism which is characteristic of
multi-orbital systems.Comment: 3 pages, 3 figures, Proceedings of Skutterudite2007 (September 26-30,
2007, Kobe
Superconductivity in the Ferroquadrupolar State in the Quadrupolar Kondo Lattice PrTiAl
The cubic compound PrTiAl is a quadrupolar Kondo lattice system
that exhibits quadrupolar ordering due to the non-Kramers ground
doublet and has strong hybridization between and conduction electrons. Our
study using high-purity single crystal reveals that PrTiAl exhibits
type-II superconductivity at mK in the nonmagnetic
ferroquadrupolar state. The superconducting critical temperature and field
phase diagram suggests moderately enhanced effective mass of
Highly anisotropic strain dependencies in PrIrZn
We report thermal expansion and magnetostriction of the cubic non-Kramers
system PrIrZn with a non-magnetic ground state
doublet. In previous experiments, antiferroquadrupolar order at
\hbox{\,K} and a Fermi liquid state around
\,T for \hbox{},
indicative of possible ferrohastatic order, were discovered. For magnetic
fields \hbox{}, the low temperature longitudinal
and transverse thermal expansion and magnetostriction are highly anisotropic.
The resulting volume strain is very small, indicating that the Pr valence
remains nearly constant as a function of magnetic field. We conclude that the
Fermi liquid state around forms through a very little change
in c-f hybridization. This result is in sharp contrast to Ce- and Yb-based
Kramers Kondo lattices which show significantly larger volume strains due to
the high sensitivity of the Kondo temperature to hydrostatic pressure.Comment: 8 pages, 8 figure
Ferromagnetic Transition in a Caged Compound NdOs2Zn20
AbstractMagnetic properties in a caged compound NdOs2Zn20 have been studied by the measurements of magnetization M, magnetic susceptibility M/B, and specific heat C. The measurements indicate that NdOs2Zn20 shows a structural transition at Ts = 62K and a ferromagnetic transition at TC = 0.6K. The structural transition is also observed in the La counter-part LaOs2Zn20 at Ts = 151K. The results of M (T)/B, M (B), and C(T) of NdOs2Zn20 are reproduced by a crystalline electrical field scheme with a Kramers doublet ground state
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