288 research outputs found
Observation of Modulated Quadrupolar Structures in PrPb3
Neutron diffraction measurements have been performed on the cubic compound
PrPb3 in a [001] magnetic field to examine the quadrupolar ordering.
Antiferromagnetic components with q=(1/2+-d 1/2 0), (1/2 1/2+-d 0) (d~1/8) are
observed below the transition temperature TQ (0.4 K at H=0) whose amplitudes
vary linear with H and vanish at zero field, providing the first evidence for a
modulated quadrupolar phase. For H<1 T, a non-square modulated state persists
even below 100 mK suggesting quadrupole moments associated with a Gamma3
doublet ground state to be partially quenched by hybridization with conduction
electrons.Comment: Physical Review Letters, in press. 4 pages, 4 figure
Antiferro-quadrupole state of orbital-degenerate Kondo lattice model with f^2 configuration
To clarify a key role of orbitals in the emergence of
antiferro-quadrupole structure in PrPb, we investigate the ground-state
property of an orbital-degenerate Kondo lattice model by numerical
diagonalization techniques. In PrPb, Pr has a
configuration and the crystalline-electric-field ground state is a non-Kramers
doublet . In a - coupling scheme, the state is
described by two local singlets, each of which consists of two electrons
with one in and another in orbitals. Since in a cubic
structure, has localized nature, while orbitals are
rather itinerant, we propose the orbital-degenerate Kondo lattice model for an
effective Hamiltonian of PrPb. We show that an antiferro-orbital state is
favored by the so-called double-exchange mechanism which is characteristic of
multi-orbital systems.Comment: 3 pages, 3 figures, Proceedings of Skutterudite2007 (September 26-30,
2007, Kobe
Effective optical identification of type "0-IIb" early gastric cancer with narrow band imaging magnification endoscopy, successfully treated by endoscopic submucosal dissection
Background Endoscopic submucosal dissection (ESD) is currently considered the minimal invasive endoscopic treatment for early gastric cancer. Most superficial gastric neoplastic lesions are depressed type ”0-IIc” (70-80%), while totally flat, classified as type ”0-IIb” early gastric cancer, is rarely reported (0.4%). The aim of the present study was to assess the efficacy of narrow band imaging (NBI) magnification endoscopy in identifying type “0-IIb” early gastric cancer and ESD treatment with curative intention.Methods Twelve of 615 (2%) patients (10 males, median 72 years), treated by ESD at our center, were diagnosed as type “0-IIb” gastric cancer. Ten had exclusively type “0-IIb”, while two had combined types “0-IIb+IIc” and “0-IIa+IIb” gastric cancer. Initial diagnosis was made during screening gastroscopy, while NBI magnification endoscopy combined with indigo-carmine chromoendoscopy were also used.Results White light endoscopy showed only superficial redness. One patient with signet-ring carcinoma showed whitish appearance. Indigo-carmine chromoendoscopy showed better visualization, while NBI magnification endoscopy revealed abnormal mucosal microsurface and microvascular findings which enabled border marking. ESD with curative intention was completed without complications. Histological examination showed complete (R0) resection, in 10 patients (83%). One patient with positive margins received additional surgery (8%). Mean procedure time was 149 (range 60-190) min. One to six years post-ESD all patients remain alive.Conclusions ESD is considered a safe and effective curative treatment for type “0-IIb” gastric cancer, resulting in long-term disease-free survival. NBI magnification endoscopy is effective for accurate optical identification and border marking of type “0-IIb” early gastric cancer
Superconductivity in the Ferroquadrupolar State in the Quadrupolar Kondo Lattice PrTiAl
The cubic compound PrTiAl is a quadrupolar Kondo lattice system
that exhibits quadrupolar ordering due to the non-Kramers ground
doublet and has strong hybridization between and conduction electrons. Our
study using high-purity single crystal reveals that PrTiAl exhibits
type-II superconductivity at mK in the nonmagnetic
ferroquadrupolar state. The superconducting critical temperature and field
phase diagram suggests moderately enhanced effective mass of
Divergent thermal expansion and Grüneisen ratio in a quadrupolar Kondo metal
We report on the low-temperature thermal expansion and magnetostriction of the single-impurity quadrupolar Kondo candidate Y1−xPrxIr2Zn20. In the dilute limit, we find a quadrupolar strain that possesses a singular dependence on temperature T, ɛu∼H2log(1/T), for a small but finite magnetic field H. Together with the previously reported anomalous specific heat C, this implies a quadrupolar Grüneisen ratio Γu=∂Tɛu/C∼H2/[T2log(1/T)] whose divergence for finite H is consistent with the scenario of a quadrupolar Kondo effect. In addition, we find a singular behavior of the isotropic strain ɛB in zero magnetic field resulting in a divergence of both the volume thermal expansion and the volume Grüneisen parameter. We speculate that this behavior might be also induced by putative Kondo correlations via elastic anharmonicities or static strain disorder
Neutron scattering study of magnetic ordering and excitations in the ternary rare-earth diborocarbide Ce^{11}B_2C_2
Neutron scattering experiments have been performed on the ternary rare-earth
diborocarbide CeBC. The powder diffraction experiment confirms
formation of a long-range magnetic order at K, where a
sinusoidally modulated structure is realized with the modulation vector . Inelastic excitation spectra in the
paramagnetic phase comprise significantly broad quasielastic and inelastic
peaks centered at and 65 meV.
Crystalline-electric-field (CEF) analysis satisfactorily reproduces the
observed spectra, confirming their CEF origin. The broadness of the
quasielastic peak indicates strong spin fluctuations due to coupling between
localized spins and conduction electrons in the paramagnetic phase. A
prominent feature is suppression of the quasielastic fluctuations, and
concomitant growth of a sharp inelastic peak in a low energy region below
. This suggests dissociation of the conduction and localized
electrons on ordering, and contrasts the presently observed incommensurate
phase with spin-density-wave order frequently seen in heavy fermion compounds,
such as Ce(RuLa)Si.Comment: accepted for publication in Phys. Rev.
Itinerant-Electron Magnet of the Pyrochlore Lattice: Indium-Doped YMn2Zn20
We report on a ternary intermetallic compound, "YMn2Zn20", comprising a
pyrochlore lattice made of Mn atoms. A series of In-doped single crystals
undergo no magnetic long-range order down to 0.4 K, in spite of the fact that
the Mn atom carries a local magnetic moment at high temperatures, showing
Curie-Weiss magnetism. However, In-rich crystals exhibit spin-glass transitions
at approximately 10 K due to a disorder arising from the substitution, while,
with decreasing In content, the spin-glass transition temperature is reduced to
1 K. Then, heat capacity divided by temperature approaches a large value of 280
mJ K-2 mol-1, suggesting a significantly large mass enhancement for conduction
electrons. This heavy-fermion-like behavior is not induced by the Kondo effect
as in ordinary f-electron compounds, but by an alternative mechanism related to
the geometrical frustration on the pyrochlore lattice, as in (Y,Sc)Mn2 and
LiV2O4, which may allow spin entropy to survive down to low temperatures and to
couple with conduction electrons.Comment: 5 pages, 4 figures, J. Phys. Soc. Jpn., in pres
Magnetic Phase Diagrams with Possible Field-induced Antiferroquadrupolar Order in TbBC
Magnetic phase diagrams of a tetragonal antiferromagnet TbBC were
clarified by temperature and field dependence of magnetization. It is
noticeable that the N{\'e}el temperature in TbBC is anomalously
enhanced with magnetic fields, in particular the enhancement reaches 13.5 K for
the direction at 10 T. The magnetization processes as well as the
phase diagrams are well interpreted assuming that there appear field-induced
antiferroquadrupolar ordered phases in TbBC. The phase diagrams of the
AFQ compounds in RBC are systematically understood in terms of the
competition with AFQ and AFM interactions.Comment: 4 pages, 4 figures, RevTeX
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