2,174 research outputs found
Ordered phase and phase transitions in the three-dimensional generalized six-state clock model
We study the three-dimensional generalized six-state clock model at values of
the energy parameters, at which the system is considered to have the same
behavior as the stacked triangular antiferromagnetic Ising model and the
three-state antiferromagnetic Potts model. First, we investigate ordered phases
by using the Monte Carlo twist method (MCTM). We confirmed the existence of an
incompletely ordered phase (IOP1) at intermediate temperature, besides the
completely ordered phase (COP) at low-temperature. In this intermediate phase,
two neighboring states of the six-state model mix, while one of them is
selected in the low temperature phase. We examine the fluctuation the mixing
rate of the two states in IOP1 and clarify that the mixing rate is very stable
around 1:1.
The high temperature phase transition is investigated by using
non-equilibrium relaxation method (NERM). We estimate the critical exponents
beta=0.34(1) and nu=0.66(4). These values are consistent with the 3D-XY
universality class. The low temperature phase transition is found to be of
first-order by using MCTM and the finite-size-scaling analysis
Monte Carlo Study of the Anisotropic Heisenberg Antiferromagnet on the Triangular Lattice
We report a Monte Carlo study of the classical antiferromagnetic Heisenberg
model with easy axis anisotropy on the triangular lattice. Both the free energy
cost for long wavelength spin waves as well as for the formation of free
vortices are obtained from the spin stiffness and vorticity modulus
respectively. Evidence for two distinct Kosterlitz-Thouless types of
defect-mediated phase transitions at finite temperatures is presented.Comment: 8 pages, 10 figure
Hemoglobin binding activity and hemoglobin-binding protein of Prevotella nigrescens
Prevotella nigrescens, lacking siderophores was found to bind to the hemoproteins. The binding was observed also in the envelope which was prepared by sonication of the cell. The binding occurred in the pH-dependent manner; the binding was observed below neutral pHs of the incubation mixtures but only slightly observed in the neutral and alkaline pHs. Furthermore, hemoglobin bound to the envelope was dissociated at high pHs buffers. Maximum amounts of hemoglobin bound to 1 mg envelope was 51.2 μg. Kd for the reaction at pH 5.0 was 2.1 × 10-10M (210 pM). From the dot blot assay, hemoglobin could bind to a protein solubilized from the envelope by a detergent, referred to as hemoglobin-binding protein (HbBP), then it was purified by the sequential procedures of ion exchange chromatography, affinity chromatography and isoelectric focusing. Molecular weight and isoelectric point of the HbBP were 46 kDa and 6.1, respectively
Phase Transition in a One-Dimensional Extended Peierls-Hubbard Model with a Pulse of Oscillating Electric Field: I. Threshold Behavior in Ionic-to-Neutral Transition
Photoinduced dynamics of charge density and lattice displacements is
calculated by solving the time-dependent Schr\"odinger equation for a
one-dimensional extended Peierls-Hubbard model with alternating potentials for
the mixed-stack organic charge-transfer complex, TTF-CA. A pulse of oscillating
electric field is incorporated into the Peierls phase of the transfer integral.
The frequency, the amplitude, and the duration of the pulse are varied to study
the nonlinear and cooperative character of the photoinduced transition. When
the dimerized ionic phase is photoexcited, the threshold behavior is clearly
observed by plotting the final ionicity as a function of the increment of the
total energy. Above the threshold photoexcitation, the electronic state reaches
the neutral one with equidistant molecules after the electric field is turned
off. The transition is initiated by nucleation of a metastable neutral domain,
for which an electric field with frequency below the linear absorption peak is
more effective than that at the peak. When the pulse is strong and short, the
charge transfer takes place on the same time scale with the disappearance of
dimerization. As the pulse becomes weak and long, the dimerization-induced
polarization is disordered to restore the inversion symmetry on average before
the charge transfer takes place to bring the system neutral. Thus, a
paraelectric ionic phase is transiently realized by a weak electric field. It
is shown that infrared light also induces the ionic-to-neutral transition,
which is characterized by the threshold behavior.Comment: 24 pages, 11 figure
Critical phase of a magnetic hard hexagon model on triangular lattice
We introduce a magnetic hard hexagon model with two-body restrictions for
configurations of hard hexagons and investigate its critical behavior by using
Monte Carlo simulations and a finite size scaling method for discreate values
of activity. It turns out that the restrictions bring about a critical phase
which the usual hard hexagon model does not have. An upper and a lower critical
value of the discrete activity for the critical phase of the newly proposed
model are estimated as 4 and 6, respectively.Comment: 11 pages, 8 Postscript figures, uses revtex.st
A Theory of Ferroelectric Phase Transition in SrTiO induced by Isotope Replacement
A theory to describe the dielectric anomalies and the ferroelectric phase
transition induced by oxygen isotope replacement in SrTiO is developed. The
proposed model gives consistent explanation between apparently contradictory
experimental results on macroscopic dielectric measurements versus microscopic
lattice dynamical measurements by neutron scattering studies. The essential
feature is described by a 3-state quantum order-disorder system characterizing
the degenerated excited states in addition to the ground state of TiO
cluster. The effect of isotope replacement is taken into account through the
tunneling frequency between the excited states. The dielectric properties are
analyzed by the mean field approximation (MFA), which gives qualitative
agreements with experimental results throughout full range of the isotope
concentration.The phase diagram in the temperature-tunneling
frequencycoordinate is studied by a QMC method to confirm the qualitative
validity of the MFA analysis.Comment: 26 pages, 8 figure
Macroscopic nucleation phenomena in continuum media with long-range interactions
Nucleation, commonly associated with discontinuous transformations between
metastable and stable phases, is crucial in fields as diverse as atmospheric
science and nanoscale electronics. Traditionally, it is considered a
microscopic process (at most nano-meter), implying the formation of a
microscopic nucleus of the stable phase. Here we show for the first time, that
considering long-range interactions mediated by elastic distortions, nucleation
can be a macroscopic process, with the size of the critical nucleus
proportional to the total system size. This provides a new concept of
"macroscopic barrier-crossing nucleation". We demonstrate the effect in
molecular dynamics simulations of a model spin-crossover system with two
molecular states of different sizes, causing elastic distortions.Comment: 12 pages, 4 figures. Supplementary information accompanies this paper
at http://www.nature.com/scientificreport
Solar Neutron Events of October-November 2003
During the period when the Sun was intensely active on October-November 2003,
two remarkable solar neutron events were observed by the ground-based neutron
monitors. On October 28, 2003, in association with an X17.2 large flare, solar
neutrons were detected with high statistical significance (6.4 sigma) by the
neutron monitor at Tsumeb, Namibia. On November 4, 2003, in association with an
X28 class flare, relativistic solar neutrons were observed by the neutron
monitors at Haleakala in Hawaii and Mexico City, and by the solar neutron
telescope at Mauna Kea in Hawaii simultaneously. Clear excesses were observed
at the same time by these detectors, with the significance calculated as 7.5
sigma for Haleakala, and 5.2 sigma for Mexico City. The detector onboard the
INTEGRAL satellite observed a high flux of hard X-rays and gamma-rays at the
same time in these events. By using the time profiles of the gamma-ray lines,
we can explain the time profile of the neutron monitor. It appears that
neutrons were produced at the same time as the gamma-ray emission.Comment: 35 pages, 21 figures, accepted for publication in Ap
A Unified Theoretical Description of the Thermodynamical Properties of Spin Crossover with Magnetic Interactions
After the discovery of the phenomena of light-induced excited spin state
trapping (LIESST), the functional properties of metal complexes have been
studied intensively. Among them, cooperative phenomena involving low spin-high
spin (spin-crossover) transition and magnetic ordering have attracted
interests, and it has become necessary to formulate a unified description of
both phenomena. In this work, we propose a model in which they can be treated
simultaneously by extending the Wajnflasz-Pick model including a magnetic
interaction. We found that this new model is equivalent to
Blume-Emery-Griffiths (BEG) Hamiltonian with degenerate levels. This model
provides a unified description of the thermodynamic properties associated with
various types of systems, such as spin-crossover (SC) solids and Prussian blue
analogues (PBA). Here, the high spin fraction and the magnetization are the
order parameters describing the cooperative phenomena of the model. We present
several typical temperature dependences of the order parameters and we
determine the phase diagram of the system using the mean-field theory and Monte
Carlo simulations. We found that the magnetic interaction drives the SC
transition leading to re-entrant magnetic and first-order SC transitions.Comment: 30pages, 11figure
Experimental Signature of Medium Modifications for rho and omega Mesons in the 12 GeV p + A Reactions
The invariant mass spectra of e+e- pairs produced in 12-GeV proton-induced
nuclear reactions are measured at the KEK Proton-Synchrotron. On the low-mass
side of the omega meson peak, a significant enhancement over the known hadronic
sources has been observed. The mass spectra, including the excess, are well
reproduced by a model that takes into account the density dependence of the
vector meson mass modification, as theoretically predicted.Comment: 4 pages, 3 figures, Version accepted for Physical Review Lette
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