1,050 research outputs found
Magnetic Susceptibility for
We examine experimental magnetic susceptibility for
CaVO by fitting with fitting function .
The function is a power series of 1/T and the lowest order
term is fixed as , where is the Curie constant as determined by the
experimental -value (g=1.96). Fitting parameters are , and
expansion coefficients except for the first one in .
We determine and as 0.73 and 0 for an
experimental sample. We interpret as the volume fraction of
CaVO in the sample and as the susceptibility for the
pure CaVO. The result of means that the sample includes
nonmagnetic components. This interpretation consists with the result of a
perturbation theory and a neutron scattering experiment.Comment: 4pages, 4figure
On the presence of mid-gap states in CaV4O9
Using exact diagonalizations of finite clusters with up to 32 sites, we study
the model on the 1/5 depleted square lattice. Spin-spin correlation
functions are consistent with plaquette order in the spin gap phase which
exists for intermediate values of . Besides, we show that singlet
states will be present in the singlet-triplet gap if is not too small
(). We argue that this property should play a central
role in determining the exchange integrals in Comment: 4 pages, 5 postscript figure
Exchange interactions and magnetic properties of the layered vanadates CaV2O5, MgV2O5, CaV3O7 and CaV4O9
We have performed ab-initio calculations of exchange couplings in the layered
vanadates CaV2O5, MgV2O5, CaV3O7 and CaV4O9. The uniform susceptibility of the
Heisenberg model with these exchange couplings is then calculated by quantum
Monte Carlo method; it agrees well with the experimental measurements. Based on
our results we naturally explain the unusual magnetic properties of these
materials, especially the huge difference in spin gap between CaV2O5 and
MgV2O5, the unusual long range order in CaV3O7 and the "plaquette resonating
valence bond (RVB)" spin gap in CaV4O9
Ab Initio Calculation of Spin Gap Behavior in CaV4O9
Second neighbor dominated exchange coupling in CaV4O9 has been obtained from
ab initio density functional (DF) calculations. A DF-based self-consistent
atomic deformation model reveals that the nearest neighbor coupling is small
due to strong cancellation among the various superexchange processes. Exact
diagonalization of the predicted Heisenberg model yields spin-gap behavior in
good agreement with experiment. The model is refined by fitting to the
experimental susceptibility. The resulting model agrees very well with the
experimental susceptibility and triplet dispersion.Comment: 4 pages; 3 ps figures included in text; Revte
The Heisenberg model on the 1/5-depleted square lattice and the CaV4O9 compound
We investigate the ground state structure of the Heisenberg model on the
1/5-depleted square lattice for arbitrary values of the first- and
second-neighbor exchange couplings. By using a mean-field Schwinger-boson
approach we present a unified description of the rich ground-state diagram,
which include the plaquette and dimer resonant-valence-bond phases, an
incommensurate phase and other magnetic orders with complex magnetic unit
cells. We also discuss some implications of ours results for the experimental
realization of this model in the CaV4O9 compound.Comment: 4 pages, Latex, 7 figures included as eps file
Two-Dimensional Quantum Spin Systems with Ladder and Plaquette Structure
We investigate low-energy properties of two-dimensional quantum spin systems
with the ladder and plaquette structures, which are described by a generalized
antiferromagnetic Heisenberg model with both of the bond and spin alternations.
By exploiting a non-linear model technique and a modified spin wave
approach, we evaluate the spin gap and the spontaneous magnetization to discuss
the quantum phase transition between the ordered and disordered states. We
argue how the spin-gapped phase is driven to the antiferromagnetic phase in the
phase diagram.Comment: 8 pages (9 figures), accepted by JPS
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