1,025 research outputs found
Quantum transport in semiconductor quantum dot superlattices: electron-phonon resonances and polaron effects
Electron transport in periodic quantum dot arrays in the presence of
interactions with phonons was investigated using the formalism of
nonequilibrium Green's functions. The self-consistent Born approximation was
used to model the self-energies. Its validity was checked by comparison with
the results obtained by direct diagonalization of the Hamiltonian of
interacting electrons and longitudinal optical phonons. The nature of charge
transport at electron -- phonon resonances was investigated in detail and
contributions from scattering and coherent tunnelling to the current were
identified. It was found that at larger values of the structure period the main
peak in the current -- field characteristics exhibits a doublet structure which
was shown to be a transport signature of polaron effects. At smaller values of
the period, electron -- phonon resonances cause multiple peaks in the
characteristics. A phenomenological model for treatment of nonuniformities of a
realistic quantum dot ensemble was also introduced to estimate the influence of
nonuniformities on current -- field characteristics
Time-Resolved Intraband Relaxation of Strongly-Confined Electrons and Holes in Colloidal PbSe Nanocrystals
The relaxation of strongly-confined electrons and holes between 1P and 1S
levels in colloidal PbSe nanocrystals has been time-resolved using femtosecond
transient absorption spectroscopy. In contrast to II-VI and III-V semiconductor
nanocrystals, both electrons and holes are strongly confined in PbSe
nanocrystals. Despite the large electron and hole energy level spacings (at
least 12 times the optical phonon energy), we consistently observe picosecond
time-scale relaxation. Existing theories of carrier relaxation cannot account
for these experimental results. Mechanisms that could possibly circumvent the
phonon bottleneck in IV-VI quantum dots are discussed
Estimation of number of runaway electrons per avalanche in Earth's atmosphere
The connection between thunderstorms and relativistic runaway electron
avalanches is an important topic that has attracted the attention of many
researchers. Among other things, there are a lot of various simulations of the
dynamics of electron avalanches. This article was written mostly in response to
the article "The critical avalanche of runaway electrons" by Evgeny Oreshkin et
al, which shows rather large numbers for an estimate of the number of runaway
electrons, but it also contains the results of our own simulation and
comparison with other papers
Probing Interband Coulomb Interactions in Semiconductor Nanocrystals with 2D Double-Quantum Coherence Spectroscopy
Using previously developed exciton scattering model accounting for the
interband, i.e., exciton-biexciton, Coulomb interactions in semiconductor
nanocrystals (NCs), we derive a closed set of equations for 2D double-quantum
coherence signal. The signal depends on the Liouville space pathways which
include both the interband scattering processes and the inter- and intraband
optical transitions. These processes correspond to the formation of different
cross-peaks in the 2D spectra. We further report on our numerical calculations
of the 2D signal using reduced level scheme parameterized for PbSe NCs. Two
different NC excitation regimes considered and unique spectroscopic features
associated with the interband Coulomb interactions are identified.Comment: 11 pages, 5 figure
Ultrafast supercontinuum spectroscopy of carrier multiplication and biexcitonic effects in excited states of PbS quantum dots
We examine the multiple exciton population dynamics in PbS quantum dots by
ultrafast spectrally-resolved supercontinuum transient absorption (SC-TA). We
simultaneously probe the first three excitonic transitions over a broad
spectral range. Transient spectra show the presence of first order bleach of
absorption for the 1S_h-1S_e transition and second order bleach along with
photoinduced absorption band for 1P_h-1P_e transition. We also report evidence
of the one-photon forbidden 1S_{h,e}-1P_{h,e} transition. We examine signatures
of carrier multiplication (multiexcitons for the single absorbed photon) from
analysis of the first and second order bleaches, in the limit of low absorbed
photon numbers (~ 10^-2), at pump energies from two to four times the
semiconductor band gap. The multiexciton generation efficiency is discussed
both in terms of a broadband global fit and the ratio between early- to
long-time transient absorption signals.. Analysis of population dynamics shows
that the bleach peak due to the biexciton population is red-shifted respect the
single exciton one, indicating a positive binding energy.Comment: 16 pages, 5 figure
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