Ferromagnetic Kondo-Lattice Model

We present a many-body approach to the electronic and magnetic properties of the (multiband) Kondo-lattice model with ferromagnetic interband exchange. The coupling between itinerant conduction electrons and localized magnetic moments leads, on the one hand, to a distinct temperature-dependence of the electronic quasiparticle spectrum and, on the other hand, to magnetic properties, as e.~g.the Curie temperature T_C or the magnon dispersion, which are strongly influenced by the band electron selfenergy and therewith in particular by the carrier density. We present results for the single-band Kondo-lattice model in terms of quasiparticle densities of states and quasiparticle band structures and demonstrate the density-dependence of the self-consistently derived Curie temperature. The transition from weak-coupling (RKKY) to strong-coupling (double exchange) behaviour is worked out. The multiband model is combined with a tight-binding-LMTO bandstructure calculation to describe real magnetic materials. As an example we present results for the archetypal ferromagnetic local-moment systems EuO and EuS. The proposed method avoids the double counting of relevant interactions and takes into account the correct symmetry of atomic orbitals.Comment: 15 pages, 10 figure

Quantum effects in the quasiparticle structure of the ferromagnetic Kondo lattice model

A new ``Dynamical Mean-field theory'' based approach for the Kondo lattice model with quantum spins is introduced. The inspection of exactly solvable limiting cases and several known approximation methods, namely the second-order perturbation theory, the self-consistent CPA and finally a moment-conserving decoupling of the equations of motion help in evaluating the new approach. This comprehensive investigation gives some certainty to our results: Whereas our method is somewhat limited in the investigation of the J<0-model, the results for J>0 reveal important aspects of the physics of the model: The energetically lowest states are not completely spin-polarized.A band splitting, which occurs already for relatively low interaction strengths, can be related to distinct elementary excitations, namely magnon emission (absorption) and the formation of magnetic polarons. We demonstrate the properties of the ferromagnetic Kondo lattice model in terms of spectral densities and quasiparticle densities of states.Comment: 19 pages, 4 figure

Proper weak-coupling approach to the periodic s-d(f) exchange model

The periodic s-d(f) exchange model is characterized by a wide variety of interesting applications, a simple mathematical structure and a limited number of reliable approximations which take care of the quantum nature of the participating spins. We suggest the use of a projection-operator method for getting information perturbationally, which are not accessible via diagrammatic approaches. In this paper we present in particular results beyond perturbation theory, which are obtained such that almost all exactly known limiting cases are incorporated correctly. We discuss a variety of possible methods and evaluate their consequences for one-particle properties. These considerations serve as a guideline for a more effective approach to the model.Comment: 11 pages, 6 figures; accepted by Phys. Rev.

Spin-polarized tunneling currents through a ferromagnetic insulator between two metallic or superconducting leads

Using the Keldysh formalism the tunneling current through a hybrid structure where a confined magnetic insulator (I) is sandwiched between two non-magnetic leads is calculated. The leads can be either normal metals (M) or superconductors (S). Each region is modelled as a single band in tight-binding approximation in order to understand the formation of the tunneling current as clearly as possible. The tunneling process itself is simulated by a hybridization between the lead and insulator conduction bands. The insulator is assumed to have localized moments which can interact with the tunneling electrons. This is described by the Kondo Lattice Model (KLM) and treated within an interpolating self-energy approach. For the superconductor the mean-field BCS theory is used. The spin polarization of the current shows a strong dependence both on the applied voltage and the properties of the materials. Even for this idealized three band model there is a qualitative agreement with experiment.Comment: 15 pages, 23 figures, accepted for publication in PR

Coupled ferro-antiferromagnetic Heisenberg bilayers investigated by many-body Green's function theory

A theory of coupled ferro- and antiferromagnetic Heisenberg layers is developed within the framework of many-body Green's function theory (GFT) that allows non-collinear magnetic arrangements by introducing sublattice structures. As an example, the coupled ferro- antiferromagnetic (FM-AFM) bilayer is investigated. We compare the results with those of bilayers with purely ferromagnetic or antiferromagnetic couplings. In each case we also show the corresponding results of mean field theory (MFT), in which magnon excitations are completely neglected. There are significant differences between GFT and MFT. A remarkable finding is that for the coupled FM-AFM bilayer the critical temperature decreases with increasing interlayer coupling strength for a simple cubic lattice, whereas the opposite is true for an fcc lattice as well as for MFT for both lattice types.Comment: 17 pages, 6 figures, accepted for publication in J. Phys. Condens. Matter, missing fig.5 adde

The treatment of zero eigenvalues of the matrix governing the equations of motion in many-body Green's function theory

The spectral theorem of many-body Green's function theory relates thermodynamic correlations to Green's functions. More often than not, the matrix governing the equations of motion has zero eigenvalues. In this case, the standard text-book approach requires both commutator and anti-commutator Green's functions to obtain equations for that part of the correlation which does not lie in the null space of the matrix. In this paper, we show that this procedure fails if the projector onto the null space is dependent on the momentum vector. We propose an alternative formulation of the theory in terms of the non-null space alone and we show that a solution is possible if one can find a momentum-independent projector onto some subspace of the non-null space. To do this, we enlist the aid of the singular value decomposition (SVD) of the equation of motion matrix in order to project out the null space, thus reducing the size of the matrix and eliminating the need for the anti-commutator Green's function. We extend our previous work, dealing with a ferromagnetic Heisenberg monolayer and a momentum-independent projector onto the null space, where both multilayer films and a momentum-dependent projector are considered. We develop the numerical methods capable of handling these cases and offer a computational algorithmus that should be applicable to any similar problem arising in Green's function theory.Comment: 16 pages, 7 figure

Kondo-lattice model: Application to the temperature-dependent electronic structure of EuO(100) films

We present calculations for the temperature-dependent electronic structure and magnetic properties of thin ferromagnetic EuO films. The treatment is based on a combination of a multiband-Kondo lattice model with first-principles TB-LMTO band structure calculations. The method avoids the problem of double-counting of relevant interactions and takes into account the correct symmetry of the atomic orbitals. We discuss the temperature-dependent electronic structures of EuO(100) films in terms of quasiparticle densities of states and quasiparticle band structures. The Curie temperature T_C of the EuO films turns out to be strongly thickness-dependent, starting from a very low value = 15K for the monolayer and reaching the bulk value at about 25 layers

Ferromagnetism and Temperature-Driven Reorientation Transition in Thin Itinerant-Electron Films

The temperature-driven reorientation transition which, up to now, has been studied by use of Heisenberg-type models only, is investigated within an itinerant-electron model. We consider the Hubbard model for a thin fcc(100) film together with the dipole interaction and a layer-dependent anisotropy field. The isotropic part of the model is treated by use of a generalization of the spectral-density approach to the film geometry. The magnetic properties of the film are investigated as a function of temperature and film thickness and are analyzed in detail with help of the spin- and layer-dependent quasiparticle density of states. By calculating the temperature dependence of the second-order anisotropy constants we find that both types of reorientation transitions, from out-of-plane to in-plane (``Fe-type'') and from in-plane to out-of-plane (``Ni-type'') magnetization are possible within our model. In the latter case the inclusion of a positive volume anisotropy is vital. The reorientation transition is mediated by a strong reduction of the surface magnetization with respect to the inner layers as a function of temperature and is found to depend significantly on the total band occupation.Comment: 10 pages, 8 figures included (eps), Phys Rev B in pres

Theory of Spin-Resolved Auger-Electron Spectroscopy from Ferromagnetic 3d-Transition Metals

CVV Auger electron spectra are calculated for a multi-band Hubbard model including correlations among the valence electrons as well as correlations between core and valence electrons. The interest is focused on the ferromagnetic 3d-transition metals. The Auger line shape is calculated from a three-particle Green function. A realistic one-particle input is taken from tight-binding band-structure calculations. Within a diagrammatic approach we can distinguish between the \textit{direct} correlations among those electrons participating in the Auger process and the \textit{indirect} correlations in the rest system. The indirect correlations are treated within second-order perturbation theory for the self-energy. The direct correlations are treated using the valence-valence ladder approximation and the first-order perturbation theory with respect to valence-valence and core-valence interactions. The theory is evaluated numerically for ferromagnetic Ni. We discuss the spin-resolved quasi-particle band structure and the Auger spectra and investigate the influence of the core hole.Comment: LaTeX, 12 pages, 8 eps figures included, Phys. Rev. B (in press

Ferromagnetism in the Periodic Anderson Model - a Modified Alloy Analogy

We introduce a new aproximation scheme for the periodic Anderson model (PAM). The modified alloy approximation represents an optimum alloy approximation for the strong coupling limit, which can be solved within the CPA-formalism. Zero-temperature and finite-temperature phase diagrams are presented for the PAM in the intermediate-valence regime. The diversity of magnetic properties accessible by variation of the system parameters can be studied by means of quasiparticle densities of states: The conduction band couples either ferro- or antiferromagneticaly to the f-levels. A finite hybridization is a necessary precondition for ferromagnetism. However, too strong hybridization generally suppresses ferromagnetism, but can for certain system parameters also lead to a semi-metallic state with unusual magnetic properties. By comparing with the spectral density approximation, the influence of quasiparticle damping can be examined.Comment: 20 pages, 13 figure