Fabrication and tuning of plasmonic optical nanoantennas around droplet epitaxy quantum dots by cathodoluminescence

We use cathodoluminescence to locate droplet epitaxy quantum dots with a precision $\lesssim$ nm before fabricating nanoantennas in their vicinity by electron-beam lithography. Cathodoluminescence is further used to evidence the effect of the antennas as a function of their length on the light emitted by the dot. Experimental results are in good agreement with numerical simulations of the structures

Microtraps for neutral atoms using superconducting structures in the critical state

Recently demonstrated superconducting atom-chips provide a platform for trapping atoms and coupling them to solid-state quantum systems. Controlling these devices requires a full understanding of the supercurrent distribution in the trapping structures. For type-II superconductors, this distribution is hysteretic in the critical state due to the partial penetration of the magnetic field in the thin superconducting film through pinned vortices. We report here an experimental observation of this memory effect. Our results are in good agreement with the redictions of the Bean model of the critical state without adjustable parameters. The memory effect allows to write and store permanent currents in micron-sized superconducting structures and paves the way towards new types of engineered trapping potentials.Comment: accepted in Phys. Rev.

Cathodoluminescence of stacking fault bound excitons for local probing of the exciton diffusion length in single GaN nanowires

We perform correlated studies of individual GaN nanowires in scanning electron microscopy combined to low temperature cathodoluminescence, microphotoluminescence, and scanning transmission electron microscopy. We show that some nanowires exhibit well localized regions emitting light at the energy of a stacking fault bound exciton (3.42 eV) and are able to observe the presence of a single stacking fault in these regions. Precise measurements of the cathodoluminescence signal in the vicinity of the stacking fault give access to the exciton diffusion length near this location

Coherence-preserving trap architecture for long-term control of giant Rydberg atoms

We present a way to trap a single Rydberg atom, make it long-lived and preserve an internal coherence over time scales reaching into the minute range. We propose to trap using carefully designed electric fields, to inhibit the spontaneous emission in a non resonant conducting structure and to maintain the internal coherence through a tailoring of the atomic energies using an external microwave field. We thoroughly identify and account for many causes of imperfection in order to verify at each step the realism of our proposal.Comment: accepted for publication in PR

Deterministic radiative coupling between plasmonic nanoantennas and semiconducting nanowire quantum dots

International audienceWe report on the deterministic coupling between single semiconducting nanowire quantum dots emitting in the visible and plasmonic Au nanoantennas. Both systems are separately carefully characterized through microphotoluminescence and cathodoluminescence. A two-step realignment process using cathodoluminescence allows for electron beam lithography of Au antennas near individual nanowire quantum dots with a precision of 50 nm. A complete set of optical properties are measured before and after antenna fabrication. They evidence both an increase of the NW absorption, and an improvement of the quantum dot emission rate up to a factor two in presence of the antenna

Wave-mixing origin and optimization in single and compact aluminum nanoantennas

The outstanding optical properties for plasmon resonances in noble metal nanoparticles enable the observation of non-linear optical processes such as second-harmonic generation (SHG) at the nanoscale. Here, we investigate the SHG process in single rectangular aluminum nanoantennas and demonstrate that i) a doubly resonant regime can be achieved in very compact nanostructures, yielding a 7.5 enhancement compared to singly resonant structures and ii) the $\chi_{\perp\perp\perp}$ local surface and $\gamma_{bulk}$ nonlocal bulk contributions can be separated while imaging resonant nanostructures excited by a tightly focused beam, provided the $\chi_{\perp\parallel\parallel}$ local surface is assumed to be zero, as it is the case in all existing models for metals. Thanks to the quantitative agreement between experimental and simulated far-field SHG maps, taking into account the real experimental configuration (focusing and substrate), we identify the physical origin of the SHG in aluminum nanoantennas as arising mainly from $\chi_{\perp\perp\perp}$ local surface sources

Optical properties of single ZnTe nanowires grown at low temperature

Optically active gold-catalyzed ZnTe nanowires have been grown by molecular beam epitaxy, on a ZnTe(111) buffer layer, at low temperature 350\degree under Te rich conditions, and at ultra-low density (from 1 to 5 nanowires per micrometer^{2}. The crystalline structure is zinc blende as identified by transmission electron microscopy. All nanowires are tapered and the majority of them are oriented. Low temperature micro-photoluminescence and cathodoluminescence experiments have been performed on single nanowires. We observe a narrow emission line with a blue-shift of 2 or 3 meV with respect to the exciton energy in bulk ZnTe. This shift is attributed to the strain induced by a 5 nm-thick oxide layer covering the nanowires, and this assumption is supported by a quantitative estimation of the strain in the nanowires

Exploring coherence of individual excitons in InAs quantum dots embedded in natural photonic defects : influence of the excitation intensity

We acknowledge the financial support by the European Research Council (ERC) Starting Grant PICSEN (grant no. 306387)The exact optical response of quantum few-level systems depends crucially on the exact choice of the incoming pulse areas. We use four-wave mixing (FWM) spectroscopy to infer the coherent response and dynamics of single InAs quantum dots (QDs) and study their pulse area dependence. By combining atomic force microscopy with FWM hyperspectral imaging, we show that the retrieved FWM signals originate from individual QDs enclosed in natural photonic defects. The optimized light-matter coupling in these defects allows us to perform our studies in a wide range of driving field amplitudes. When varying the pulse areas of the exciting laser pulses Rabi rotations of microscopic interband coherences can be resolved by the two-pulse FWM technique. We investigate these Rabi coherence rotations within two- and three-level systems, both theoretically and experimentally, and explain their damping by the coupling to acoustic phonons. To highlight the importance of the pulse area in uence, we show that the phonon-induced dephasing of QD excitons depends on the pulse intensity.PostprintPeer reviewe