21,442 research outputs found

    Antisite Disorder-induced Exchange Bias Effect in Multiferroic Y2CoMnO6

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    Exchange bias effect in the ferromagnetic double perovskite compound Y2_2CoMnO6_6, which is also a multiferroic, is reported. The exchange bias, observed below 8~K, is explained as arising due to the interface effect between the ferromagnetic and antiferromagnetic clusters created by {\it antisite} disorder in this material. Below 8~K, prominent ferromagnetic hysteresis with metamagnetic "steps" and significant coercive field, HcH_c \approx 10~kOe are observed in this compound which has a TcT_c \approx 75~K. A model based on growth of ferromagnetic domains overcoming the elastic energy of structurally pinned magnetic interfaces, which closely resembles martensitic-like transitions, is adapted to explain the observed effects. The role of {\it antisite} disorder in creating the domain structure leading to exchange bias effect is highlighted in the present work.Comment: 4 pages two-column, 4 figures, accepted to Appl. Phys. Let

    Spin Freezing in the Spin Liquid Compound FeAl2O4

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    Spin freezing in the AA-site spinel FeAl2_2O4_4 which is a spin liquid candidate is studied using remnant magnetization and nonlinear magnetic susceptibility and isofield cooling and heating protocols. The remnant magnetization behavior of FeAl2_2O4_4 differs significantly from that of a canonical spin glass which is also supported by analysis of the nonlinear magnetic susceptibility term χ3(T)\chi_3 (T). Through the power-law analysis of χ3(T)\chi_3 (T), a spin-freezing temperature, TgT_g = 11.4±\pm0.9~K and critical exponent, γ\gamma = 1.48±\pm0.59 are obtained. Cole-Cole analysis of magnetic susceptibility shows the presence of broad spin relaxation times in FeAl2_2O4_4, however, the irreversible dc susceptibility plot discourages an interpretation based on conventional spin glass features. The magnetization measured using the cooling-and-heating-in-unequal-fields protocol brings more insight to the magnetic nature of this frustrated magnet and reveals unconventional glassy behaviour. Combining our results, we arrive at the conclusion that the present sample of FeAl2_2O4_4 consists of a majority spin liquid phase with "glassy" regions embedded.Comment: 5 pages, 6 figs, 2-column, Accepted to Phys. Rev.
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