169 research outputs found
Beyond single-photon localization at the edge of a Photonic Band Gap
We study spontaneous emission in an atomic ladder system, with both
transitions coupled near-resonantly to the edge of a photonic band gap
continuum. The problem is solved through a recently developed technique and
leads to the formation of a ``two-photon+atom'' bound state with fractional
population trapping in both upper states. In the long-time limit, the atom can
be found excited in a superposition of the upper states and a ``direct''
two-photon process coexists with the stepwise one. The sensitivity of the
effect to the particular form of the density of states is also explored.Comment: to appear in Physical Review
From colloidal CdSe quantum dots to microscale optically anisotropic supercrystals through bottom-up self-assembly
This is the author accepted manuscript. The final version is available on open access from Royal Society of Chemistry via the DOI in this recordThe development of fabrication techniques for novel nanostructured materials is one of the key tasks of modern materials science. One pathway to successfully complete this task is the bottom-up assembly of colloidal nanoparticles into ordered superstructures, possessing both the properties of individual nanoparticles and further novel properties resulting from their interactions. However, nanoparticle self-assembly depends on a variety of parameters, which makes the precise control of this process a complicated problem. Here, the time course of quantum dot (QD) self-assembly into ordered superstructures has been analyzed, along with the evolution of their morphological and optical properties. QD self-assembly occurs through two distinct stages (homo- and hetero-geneous), leading to the formation of supercrystals with a layered morphology. Analysis of the optical properties throughout the superstructures’ growth has shown that the absorption and photoluminescence (PL) bands are blue shifted, retaining almost the same PL lifetimes as in the initial QD solution. The supercrystals formed possess a further unique optical property caused by their layered morphology; namely, a four-fold symmetry characterized by strong birefringence. Such supercrystals may be used for the fabrication of microscale optical paths with high extinction coefficients and specific polarization properties for novel optoelectronic devices.This study was supported by the Ministry of Education and
Science of the Russian Federation through the grant No.
14.584.21.0032 (ID RFMEFI58417X0032), the Engineering
and Physical Sciences Research Council (EPSRC) of the United
Kingdom via the EPSRC Centre for Doctoral Training in Electromagnetic
Metamaterials (Grant No. EP/L015331/1) and
via EP/N035569/1, and the Royal Society via International
Exchange Grant No. 2016/R1
Modern studies of the cryosphere of the Zeravshan and Gissar Ranges (Tien Shan)
The paper presents brief results of the modern studies of the cryosphere of the Zeravshan and Gissar ranges. Also the rate of decrease in the area of glaciers over the last almost a hundred years and the presence and degradation of permafrost during that time were considered. The actual description of the methodic for estimation of the depth of the ground freezing based on air temperature and snow thickness data were also given. An experience of application of this method for estimating the depth of ground freezing on the mountain slopes in order to compile the maps of the permafrost zone of the Zeravshan and Gissar ranges was described
Entanglement Sudden Death in Band Gaps
Using the pseudomode method, we evaluate exactly time-dependent entanglement
for two independent qubits, each coupled to a non-Markovian structured
environment. Our results suggest a possible way to control entanglement sudden
death by modifying the qubit-pseudomode detuning and the spectrum of the
reservoirs. Particularly, in environments structured by a model of a
density-of-states gap which has two poles, entanglement trapping and prevention
of entanglement sudden death occur in the weak-coupling regime
Processing and Use of Solid Technogenic Waste - Damping Metallurgical Slags for Producing Calcium-Containing Ferro-Alloys
In the given article there are presented the results of complex calcium-containing ferroalloy from high-ash coals of the Saryadyr deposit, dump blast-furnace slag and slag of refined ferromanganese, which related to technogenic waste. There is established the possibility of smelting calcium-containing ferroalloy, the recovery of basic elements reached 91.56% manganese, 87.75% silicon, 76% aluminum and calcium up to 40%
Surface ligands affect photoinduced modulation of the quantum dots optical performance
ABSTRACT Changes of optical properties of the solutions of CdSe/ZnS quantum dots (QDs) covered with the trioctylphosphine oxide (TOPO) ligands under the pulsed ultraviolet (UV) laser irradiation are observed. The fluorescence quantum yield (QY) of QDs decreases by more than an order of magnitude when the radiation dose approaches 2 × 10 -15 J per particle. This process is accompanied by a blue shift of both fluorescence and the first excitonic absorption peaks. The fluorescence quenching becomes less pronounced when the overall TOPO content in the solution is increased. When ТОРО ligands are replaced with n-hexadecylamine (HDA), QY and spectral properties are not changed at the same irradiation conditions. We assume that the above changes of the optical properties are associated with photooxidation of TOPO ligands by excited QD. Such process is less probable for the HDA ligand due to its different energy structure
The influence of density of modes on dark lines in spontaneous emission
We study two distinct multi-level atomic models in which one transition is
coupled to a Markovian reservoir, while another linked transition is coupled to
a non-Markovian reservoir. We show that by choosing appropriately the density
of modes of the non-Markovian reservoir the spontaneous emission to the
Markovian reservoir is greatly altered. The existence of `dark lines' in the
spontaneous emission spectrum in the Markovian reservoir due to the coupling to
specific density of modes of the non-Markovian reservoir is also predicted.Comment: 11 pages including 9 figure
Plasmonic Control of Radiative Properties of Semiconductor Quantum Dots Coupled to Plasmonic Ring Cavities
In recent years, a lot of effort has been made to achieve controlled delivery of target particles to the hotspots of plasmonic nanoantennas, in order to probe and/or exploit the extremely large field enhancements produced by such structures. While in many cases such high fields are advantageous, there are instances where they should be avoided. In this work, we consider the implications of using the standard nanoantenna geometries when colloidal quantum dots are employed as target entities. We show that in this case, and for various reasons, dimer antennas are not the optimum choice. Plasmonic ring cavities are a better option despite low field enhancements, as they allow collective coupling of many quantum dots in a reproducible and predictable manner. In cases where larger field enhancements are required, or for larger quantum dots, nonconcentric ring-disk cavities can be employed instead
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