540 research outputs found

    Anomalous Magnetic Properties in Ni50Mn35In15

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    We present here a comprehensive investigation of the magnetic ordering in Ni50Mn35In15 composition. A concomitant first order martensitic transition and the magnetic ordering occurring in this off-stoichiometric Heusler compound at room temperature signifies the multifunctional character of this magnetic shape memory alloy. Unusual features are observed in the dependence of the magnetization on temperature that can be ascribed to a frustrated magnetic order. It is compelling to ascribe these features to the cluster type description that may arise due to inhomogeneity in the distribution of magnetic atoms. However, evidences are presented from our ac susceptibility, electrical resistivity and dc magnetization studies that there exists a competing ferromagnetic and antiferromagnetic order within crystal structure of this system. We show that excess Mn atoms that substitute the In atoms have a crucial bearing on the magnetic order of this compound. These excess Mn atoms are antiferromagnetically aligned to the other Mn, which explains the peculiar dependence of magnetization on temperature.Comment: Accepted in J. Phys. D.:Appl. Physic

    Premartensitic Transition in Ni2+xMn1-xGa Heusler Alloys

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    The temperature dependencies of the resistivity and magnetization of a series of Ni2+XMn1-XGa (X = 0 - 0.09) alloys were investigated. Along with the anomalies associated with ferromagnetic and martensitic transitions, well-defined anomalies were observed at the temperature of premartensitic transformation. The premartensitic phase existing in a temperature range 200 - 260 K in the stoichiometric Ni2MnGa is suppressed by the martensitic phase with increasing Ni content and vanishes in Ni2.09Mn0.91Ga composition

    Raman, infrared and optical spectra of the spin-Peierls compound NaV_2O_5

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    We have measured polarized spectra of Raman scattering, infrared and optical transmission of NaV_2O_5 single crystals above the temperature of the spin-Peierls transition Tsp=35 K. Some of the far-infrared (FIR) phonon lines are strongly asymmetric, due to the spin-phonon interaction. In addition to the phonon lines, a broad band was observed in the c(aa)c Raman spectrum and in the E||a FIR transmission spectrum. A possible origin of these bands is discussed. The absorption band at 10000 cm-1 1.25 eV is attributed to vanadium d-d electronic transitions while the absorption edge above 3 eV is supposed to correspond to the onset of charge-transfer transitions.Comment: 7 figures, 8 page

    Anomalous thermal conductivity of NaV2O5 as compared to conventional spin-Peierls system CuGeO3

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    A huge increase of thermal conductivity k is observed at the phase transition in stoichiometric NaV2O5. This anomaly decreases and gradually disappears with deviation from stoichiometry in Na(1-x}V2O5 (x = 0.01, 0.02, 0.03, and 0.04). This behavior is compared with that of pure and Zn-doped CuGeO3 where only modest kinks in the k(T) curves are observed at the spin-Peierls transition. The change of k at critical temperature Tc could be partially attributed to the opening of an energy gap in the magnetic excitation spectrum excluding the scattering of thermal phonons on spin fluctuations. However, the reason for such a strong anomaly in the k(T) may lie not only in the different energy scales of CuGeO3 and NaV2O5, but also in the different character of the phase transition in NaV2O5 which can have largely a structural origin, e.g. connected with the charge ordering.Comment: PostScript 4 pages, 4 PostScript pictures. Submitted to Physical Review Letter

    High frequency ESR investigation on dynamical charge disproportionation and spin gap excitation in NaV_2O_5

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    A significant frequency dependence of the ESR line width is found in NaV_2O_5 between 34-100 K and the line width increases as the resonance frequency is increased from 95 GHz to 760 GHz. The observed frequency dependence is qualitatively explained in terms of the dynamical charge disproportionation. The present results show the essential role of the internal charge degree of freedom in a V-O-V bond. We have also proposed the existence of the Dzyaloshinsky-Moriya interaction in the low temperature charge ordered phase considering the breaking of the selection rule of ESR realized as the direct observation of the spin gap excitation.Comment: 9 figures submitted to J. Phys.Soc. Jp

    Integral Transforms for Conformal Field Theories with a Boundary

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    A new method is developed for solving the conformally invariant integrals that arise in conformal field theories with a boundary. The presence of a boundary makes previous techniques for theories without a boundary less suitable. The method makes essential use of an invertible integral transform, related to the radon transform, involving integration over planes parallel to the boundary. For successful application of this method several nontrivial hypergeometric function relations are also derived.Comment: 20 pagess, LateX fil

    A Model Study of the Low-Energy Charge Dynamics of NaV_2O_5

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    An exact-diagonalization technique on small clusters is used to calculate the dynamical density correlation functions of the dimerized t-J chain and coupled anisotropic t-J ladders (trellis lattice) at quarter filling, i.e., the systems regarded as a network of pairs (dimers or rungs) of sites coupled weakly via the hopping and exchange interactions. We thereby demonstrate that the intersite Coulomb repulsions between the pairs induce a low-energy collective mode in the charge excitations of the systems where the internal charge degrees of freedom of the pairs play an essential role. Implications to the electronic states of NaV_2O_5, i.e., fluctuations of the valence state of V ions and phase transition as a charge ordering, are discussed.Comment: 4 pages, 4 gif figures. Hardcopies of figures (or the entire manuscript) can be obtained by e-mail request to [email protected]
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