444 research outputs found
A bulk 2D Pauli Limited Superconductor
We present a nearly perfect Pauli-limited critical field phase diagram for
the anisotropic organic superconductor \-(ET)NH(SCN) when
the applied magnetic field is oriented parallel to the conducting layers. The
critical fields ({H_{c_2}) were found by use of penetration depth
measurements. Because {H_{c_2} is Pauli-limited, the size of the
superconducting energy gap can be calculated. The role of spin-orbit scattering
and many-body effects play a role in explaining our measurements.Comment: 4 pages, 5 figures. V5, corrections were made to the text, present
data was include
Substitution Effect by Deuterated Donors on Superconductivity in -(BEDT-TTF)Cu[N(CN)]Br
We investigate the superconductivity in the deuterated BEDT-TTF molecular
substitution system
-[(h8-BEDT-TTF)(d8-BEDT-TTF)]Cu[N(CN)]Br, where h8
and d8 denote fully hydrogenated and deuterated molecules, respectively.
Systematic and wide range ( = 0 -- 1) substitution can control chemical
pressure finely near the Mott boundary, which results in the modification of
the superconductivity. After cooling slowly, the increase of
observed up to 0.1 is evidently caused by the chemical pressure
effect. Neither reduction of nor suppression of
superconducting volume fraction is found below 0.5. This demonstrates
that the effect of disorder by substitution is negligible in the present
system. With further increase of , both and superconducting
volume fraction start to decrease toward the values in = 1.Comment: J. Phys. Soc. Jp
Critical State Behaviour in a Low Dimensional Metal Induced by Strong Magnetic Fields
We present the results of magnetotransport and magnetic torque measurements
on the alpha-(BEDT-TTF)2KHg(SCN)4 charge-transfer salt within the high magnetic
field phase, in magnetic fields extending to 33 T and temperatures as low as 27
mK. While the high magnetic field phase (at fields greater than ~ 23 T) is
expected, on theoretical grounds, to be either a modulated charge-density wave
phase or a charge/spin-density wave hybrid, the resistivity undergoes a
dramatic drop below ~ 3 K within the high magnetic field phase, falling in an
approximately exponential fashion at low temperatures, while the magnetic
torque exhibits pronounced hysteresis effects. This hysteresis, which occurs
over a broad range of fields, is both strongly temperature-dependent and has
several of the behavioural characteristics predicted by critical-state models
used to describe the pinning of vortices in type II superconductors in strong
magnetic fields. Thus, rather than exhibiting the usual behaviour expected for
a density wave ground state, both the transport and the magnetic properties of
alpha-(BEDT-TTF)2KHg(SCN)4, at high magnetic fields, closely resembles those of
a type II superconductor
Experimental observation of Frohlich superconductivity in high magnetic fields
Resistivity and irreversible magnetisation data taken within the
high-magnetic-field CDWx phase of the quasi-two-dimensional organic metal
alpha-(BEDT-TTF)2KHg(SCN)4 are shown to be consistent with a field-induced
inhomogeneous superconducting phase. In-plane skin-depth measurements show that
the resistive transition on entering the CDWx phase is both isotropic and
representative of the bulk.Comment: ten pages, four figure
Disorder Effect on the Vortex Pinning by the Cooling Process Control in the Organic Superconductor -(BEDT-TTF)Cu[N(CN)]Br
We investigate the influence of disorders in terminal ethylene groups of
BEDT-TTF molecules (ethylene-disorders) on the vortex pinning of the organic
superconductor -(BEDT-TTF)Cu[N(CN)]Br. Magnetization
measurements are performed under different cooling-processes. The second peak
in the magnetization hysteresis curve is observed for all samples studied, and
the hysteresis width of the magnetization becomes narrower by cooling faster.
In contradiction to the simple pinning effect of disorder, this result shows
the suppression of the vortex pinning force by introducing more
ethylene-disorders. The ethylene-disorder domain model is proposed for
explaining the observed result. In the case of the system containing a moderate
number of the ethylene-disorders, the disordered molecules form a domain
structure and it works as an effective pinning site. On the contrary, an excess
number of the ethylene-disorders may weaken the effect of the domain structure,
which results in the less effective pinning force on the vortices.Comment: 6 pages, 6 figure
Superconductivity in an organic insulator at very high magnetic fields
We investigate by electrical transport the field-induced superconducting
state (FISC) in the organic conductor -(BETS)FeCl. Below 4 K,
antiferromagnetic-insulator, metallic, and eventually superconducting (FISC)
ground states are observed with increasing in-plane magnetic field. The FISC
state survives between 18 and 41 T, and can be interpreted in terms of the
Jaccarino-Peter effect, where the external magnetic field {\em compensates} the
exchange field of aligned Fe ions. We further argue that the Fe
moments are essential to stabilize the resulting singlet, two-dimensional
superconducting stateComment: 9 pages 3 figure
Isotope effect in superconductors with coexisting interactions of phonon and nonphonon mechanisms
We examine the isotope effect of superconductivity in systems with coexisting
interactions of phonon and nonphonon mechanisms in addition to the direct
Coulomb interaction. The interaction mediated by the spin fluctuations is
discussed as an example of the nonphonon interaction. Extended formulas for the
transition temperature Tc and the isotope-effect coefficient alpha are derived
for cases (a) omega_np omega_D, where omega_np is
an effective cutoff frequency of the nonphonon interaction that corresponds to
the Debye frequency omega_D in the phonon interaction. In case (a), it is found
that the nonphonon interaction does not change the condition for the inverse
isotope effect, i.e., mu^* > lambda_ph/2, but it modifies the magnitude of
alpha markedly. In particular, it is found that a giant isotope shift occurs
when the phonon and nonphonon interactions cancel each other largely. For
instance, strong critical spin fluctuations may give rise to the giant isotope
effect. In case (b), it is found that the inverse isotope effect occurs only
when the nonphonon interaction and the repulsive Coulomb interaction, in total
effect, work as repulsive interactions against the superconductivity. We
discuss the relevance of the present result to some organic superconductors,
such as kappa-(ET)2Cu(NCS)2 and Sr2RuO4 superconductors, in which inverse
isotope effects have been observed, and briefly to high-Tc cuprates, in which
giant isotope effects have been observed.Comment: 4 pages, 2 figures, (with jpsj2.cls, ver.1.2), v2:linguistic
correction
Impurity Effect on the In-plane Penetration Depth of the Organic Superconductors -(BEDT-TTF) ( = Cu(NCS) and Cu[N(CN)]Br)
We report the in-plane penetration depth of single
crystals -(BEDT-TTF) ( Cu(NCS) and Cu[N(CN)]Br) by
means of the reversible magnetization measurements under the control of
cooling-rate. In = Cu(NCS), as an
extrapolation toward = 0 K does not change by the cooling-rate within the
experimental accuracy, while is slightly reduced. On the other
hand, in = Cu[N(CN)]Br, indicates a distinct
increase by cooling faster. The different behavior of
on cooling-rate between the two salts is quantitatively explained in terms of
the local-clean approximation (London model), considering that the former salt
belongs to the very clean system and the later the moderate clean one. The good
agreement with this model demonstrates that disorders of ethylene-group in
BEDT-TTF introduced by cooling faster increase the
electron(quasiparticle)-scattering, resulting in shorter mean free path.Comment: 8 pages, 9 figure
Competition between Pauli and orbital effects in a charge-density wave system
We present angular dependent magneto-transport and magnetization measurements
on alpha-(ET)2MHg(SCN)4 compounds at high magnetic fields and low temperatures.
We find that the low temperature ground state undergoes two subsequent
field-induced density-wave type phase transitions above a critical angle of the
magnetic field with respect to the crystallographic axes. This new phase
diagram may be qualitatively described assuming a charge density wave ground
state which undergoes field-induced transitions due to the interplay of Pauli
and orbital effects.Comment: 11 pages, 4 figures, shown at the APS march meeting 2000, appears in
the Ph.D. thesis of J. S. Qualls (Florida State University, 1999), and
submitted to PR
Surface characterization and surface electronic structure of organic quasi-one-dimensional charge transfer salts
We have thoroughly characterized the surfaces of the organic charge-transfer
salts TTF-TCNQ and (TMTSF)2PF6 which are generally acknowledged as prototypical
examples of one-dimensional conductors. In particular x-ray induced
photoemission spectroscopy turns out to be a valuable non-destructive
diagnostic tool. We show that the observation of generic one-dimensional
signatures in photoemission spectra of the valence band close to the Fermi
level can be strongly affected by surface effects. Especially, great care must
be exercised taking evidence for an unusual one-dimensional many-body state
exclusively from the observation of a pseudogap.Comment: 11 pages, 12 figures, v2: minor changes in text and figure labellin
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