195 research outputs found
Hyperbolic Metamaterial Resonator-Antenna Scheme for Large, Broadband Emission Enhancement and Single Photon Collection
We model the broadband enhancement of single-photon emission from color
centres in silicon carbide nanocrystals coupled to a planar hyperbolic
metamaterial, HMM resonator. The design is based on positioning the single
photon emitters within the HMM resonator, made of a dielectric index-matched
with silicon-carbide material. The broadband response results from the
successive resonance peaks of the lossy Fabry Perot structure modes arising
within the high-index HMM cavity. To capture this broadband enhancement in the
single photon emitters spontaneous emission, we placed a simple gold based
cylindrical antenna on top of the HMM resonator. We analyzed the performance of
this HMM coupled antenna structure in terms of the Purcell enhancement, quantum
efficiency, collection efficiency and overall collected photon rate. For
perpendicular dipole orientation relative to the interface, the HMM coupled
antenna resonator leads to a significantly large spontaneous emission
enhancement with Purcell factor of the order of 250 along with a very high
average total collected photon rate, CPR of about 30 over a broad emission
spectrum, 700 nm to 1000 nm. The peak CPR increases to about 80 at 900 nm,
corresponding to the emission of silicon-carbide quantum emitters. This is a
state of the art improvement considering the previous computational designs
have reported a maximum average CPR of 25 across the nitrogen-vacancy centre
emission spectrum, 600 nm to 800 nm with the highest value being about 40 at
650 nm
Optimizing single-photon-source heralding efficiency at 1550 nm using periodically poled lithium niobate
We explore the feasibility of using high conversion-efficiency
periodically-poled crystals to produce photon pairs for photon-counting
detector calibrations at 1550 nm. The goal is the development of an appropriate
parametric down-conversion (PDC) source at telecom wavelengths meeting the
requirements of high-efficiency pair production and collection in single
spectral and spatial modes (single-mode fibers). We propose a protocol to
optimize the photon collection, noise levels and the uncertainty evaluation.
This study ties together the results of our efforts to model the single-mode
heralding efficiency of a two-photon PDC source and to estimate the heralding
uncertainty of such a source.Comment: 14 pages, 2 tables and 3 figures, final version accepted by
Metrologi
Towards achieving strong coupling in 3D-cavity with solid state spin resonance
We investigate the microwave magnetic field confinement in several microwave
3D-cavities, using 3D finite-element analysis to determine the best design and
achieve strong coupling between microwave resonant cavity photons and solid
state spins. Specifically, we design cavities for achieving strong coupling of
electromagnetic modes with an ensemble of nitrogen vacancy (NV) defects in
diamond. We report here a novel and practical cavity design with a magnetic
filling factor of up to 4 times (2 times higher collective coupling) than
previously achieved using 1D superconducting cavities with small mode volume.
In addition, we show that by using a double-split resonator cavity, it is
possible to achieve up to 200 times better cooperative factor than the
currently demonstrated with NV in diamond. These designs open up further
opportunities for studying strong and ultra-strong coupling effects on spins in
solids using alternative systems with a wider range of design parameters.Comment: 20 pages, 9 figure
Quantum and Classical Noise in Practical Quantum Cryptography Systems based on polarization-entangled photons
Quantum-cryptography key distribution (QCKD) experiments have been recently
reported using polarization-entangled photons. However, in any practical
realization, quantum systems suffer from either unwanted or induced
interactions with the environment and the quantum measurement system, showing
up as quantum and, ultimately, statistical noise. In this paper, we investigate
how ideal polarization entanglement in spontaneous parametric downconversion
(SPDC) suffers quantum noise in its practical implementation as a secure
quantum system, yielding errors in the transmitted bit sequence. Because all
SPDC-based QCKD schemes rely on the measurement of coincidence to assert the
bit transmission between the two parties, we bundle up the overall quantum and
statistical noise in an exhaustive model to calculate the accidental
coincidences. This model predicts the quantum-bit error rate and the sifted key
and allows comparisons between different security criteria of the hitherto
proposed QCKD protocols, resulting in an objective assessment of performances
and advantages of different systems.Comment: Rev Tex Style, 2 columns, 7 figures, (a modified version will appear
on PRA
Single-photon emitting diode in silicon carbide
Electrically driven single-photon emitting devices have immediate
applications in quantum cryptography, quantum computation and single-photon
metrology. Mature device fabrication protocols and the recent observations of
single defect systems with quantum functionalities make silicon carbide (SiC)
an ideal material to build such devices. Here, we demonstrate the fabrication
of bright single photon emitting diodes. The electrically driven emitters
display fully polarized output, superior photon statistics (with a count rate
of 300 kHz), and stability in both continuous and pulsed modes, all at room
temperature. The atomic origin of the single photon source is proposed. These
results provide a foundation for the large scale integration of single photon
sources into a broad range of applications, such as quantum cryptography or
linear optics quantum computing.Comment: Main: 10 pages, 6 figures. Supplementary Information: 6 pages, 6
figure
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Self-assembly, nematic phase formation and organocatalytic behaviour of a proline-functionalized lipopeptide
The self-assembly of the amphiphilic lipopeptide PAEPKI-C16 (P = proline, A = alanine, E = glutamic acid, K = lysine, I = isoleucine, C16 = hexadecyl) was investigated using a combination of spectroscopic, microscopic and scattering methods and compared to C16-IKPEAP with the same (reversed) peptide sequence and the alkyl chain positioned N-terminally and which lacks a free N-terminal proline residue. The catalytic activity of these peptides were then compared using a model aldol reaction system. For PAEPKI-C16, Cryo-TEM images showed the formation of micrometer length fibers, which by Small-angle X-ray scattering (SAXS) were found to have a radius of 2.5 - 2.6 nm. Spectroscopic analysis shows these fibers are built from -sheets. This behaviour is in complete contrast to that of C16-IKPEAP which forms spherical micelles with peptides in a disordered conformation [Hutchinson, J. A. et al. J. Phys. Chem. B 2019, 123, 613]. For PAEPKI-C16, the spontaneous alignment of fibers was observed upon increasing pH, which was accompanied by observed birefringence and anisotropy of SAXS patterns. This shows the formation of a nematic liquids and unprecedented nematic hydrogel formation was also observed these lipopeptides at sufficiently high concentrations. SAXS shows retention of an ultrafine (1.7 nm core radius) fibrillar network within the hydrogel. PAEPKI-C16 with free N-terminal proline shows enhanced anti:syn diastereoselectivity and better conversion compared to C16-IKPEAP. The cytotoxicity of PAEPKI-C16 was also lower than C16-IKPEAP for both fibroblast and cancer cell lines. These results highlight the sensitivity of lipopeptide properties to the presence of a free proline residue. The spontaneous nematic phase formation by PAEPKI-C16 points to the highly anisotropy of its ultrafine fibrillar structure and the formation of such a phase at low concentration in aqueous solution may be valuable for future applications
A silicon carbide room temperature single-photon source
Over the past few years, single-photon generation has been realized in numerous systems: single molecules 1 , quantum dots 2-4 , diamond colour centres 5 and others 6 . The generation and detection of single photons play a central role in the experimental foundation of quantum mechanics 7 and measurement theory 8 . An efficient and high-quality single-photon source is needed to implement quantum key distribution, quantum repeaters and photonic quantum information processing 9 . Here we report the identification and formation of ultrabright, room-temperature, photostable single-photon sources in a device-friendly material, silicon carbide (SiC). The source is composed of an intrinsic defect, known as the carbon antisite- vacancy pair, created by carefully optimized electron irradiation and annealing of ultrapure SiC. An extreme brightness (210 6 counts s 1 ) resulting from polarization rules and a high quantum efficiency is obtained in the bulk without resorting to the use of a cavity or plasmonic structure. This may benefit future integrated quantum photonic devices 9
Addressing a single NV spin with a macroscopic dielectric microwave cavity
We present a technique for addressing single NV center spins in diamond
over macroscopic distances using a tunable dielectric microwave cavity. We
demonstrate optically detected magnetic resonance (ODMR) for a single NV
center in a nanodiamond (ND) located directly under the macroscopic microwave
cavity. By moving the cavity relative to the ND, we record the ODMR signal as a
function of position, mapping out the distribution of the cavity magnetic field
along one axis. In addition, we argue that our system could be used to
determine the orientation of the NV major axis in a straightforward
manner
Reduced Deadtime and Higher Rate Photon-Counting Detection using a Multiplexed Detector Array
We present a scheme for a photon-counting detection system that can be
operated at incident photon rates higher than otherwise possible by suppressing
the effects of detector deadtime. The method uses an array of N detectors and a
1-by-N optical switch with a control circuit to direct input light to live
detectors. Our calculations and models highlight the advantages of the
technique. In particular, using this scheme, a group of N detectors provides an
improvement in operation rate that can exceed the improvement that would be
obtained by a single detector with deadtime reduced by 1/N, even if it were
feasible to produce a single detector with such a large improvement in
deadtime. We model the system for continuous and pulsed light sources, both of
which are important for quantum metrology and quantum key distribution
applications.Comment: 6 figure
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