Nonlinear optical response and exciton dephasing in quantum dots

The full time-dependent four-wave mixing polarization in quantum dots is microscopically calculated, taking into account acoustic phonon-assisted transitions between different exciton states of the dot. It is shown that quite different dephasing times of higher exciton states in pancake anisotropic InGaAs quantum dots are responsible for the experimentally observed [1] double-exponential decay in the photon echo signal.Comment: NOEKS-8 contribution; 4 pages, 3 figure

Exciton dephasing in quantum dots: Coupling to LO phonons via excited states

We have found a novel mechanism of spectral broadening and dephasing in quantum dots (QDs) due to the coupling to longitudinal-optical (LO) phonons. In theory, this mechanism comes into play only if the complete manifold of exciton levels (including those in the wetting-layer continuum) is taken into account. We demonstrate this nontrivial dephasing in different types of QDs, using the exactly solvable quadratic coupling model, here generalized to an arbitrary number of excitonic states.Comment: OECS10 contribution pape

Resonant-state expansion for open optical systems: Generalization to magnetic, chiral, and bi-anisotropic materials

The resonant-state expansion, a recently developed powerful method in electrodynamics, is generalized here for open optical systems containing magnetic, chiral, or bi-anisotropic materials. It is shown that the key matrix eigenvalue equation of the method remains the same, but the matrix elements of the perturbation now contain variations of the permittivity, permeability, and bi-anisotropy tensors. A general normalization of resonant states in terms of the electric and magnetic fields is presented.Comment: 4 page

Resonant states in double and triple quantum wells

The full set of resonant states in double and triple quantum well/barrier structures is investigated. This includes bound, anti-bound and normal resonant states which are all eigensolutions of Schrodinger's equation with generalized outgoing wave boundary conditions. The transformation of resonant states and their transitions between different subgroups as well as the role of each subgroup in observables, such as the quantum transmission, is analyzed. The quantum well potentials are modeled by Dirac delta functions; therefore, as part of this study, the well-known problem of bound states in delta-like potentials is also revisited.Comment: 10 pages, 11 figure

Exciton effective mass enhancement in coupled quantum wells in electric and magnetic fields

We present a calculation of exciton states in semiconductor coupled quantum wells (CQWs) in the presence of electric and magnetic fields applied perpendicular to the QW plane. The exciton Schr\"odinger equation is solved in real space in three dimensions to obtain the Landau levels of both direct and indirect excitons. Calculation of the exciton energy levels and oscillator strengths enables mapping of the electric and magnetic field dependence of the exciton absorption spectrum. For the ground state of the system, we evaluate the Bohr radius, optical lifetime, binding energy and dipole moment. The exciton mass renormalization due to the magnetic field is calculated using a perturbative approach. We predict a non-monotonous dependence of the exciton ground state effective mass on magnetic field. Such a trend is explained in a classical picture, in terms of the ground state tending from an indirect to a direct exciton with increasing magnetic field.Comment: 20 pages, 7 figure

Phonon-Induced Dephasing in Quantum Dot-Cavity QED

We present a semi-analytic and asymptotically exact solution to the problem of phonon-induced decoherence in a quantum dot-microcavity system. Particular emphasis is placed on the linear polarization and optical absorption, but the approach presented herein may be straightforwardly adapted to address any elements of the exciton-cavity density matrix. At its core, the approach combines Trotter's decomposition theorem with the linked cluster expansion. The effects of the exciton-cavity and exciton-phonon couplings are taken into account on equal footing, thereby providing access to regimes of comparable polaron and polariton timescales. We show that the optical decoherence is realized by real phonon-assisted transitions between different polariton states of the quantum dot-cavity system, and that the polariton line broadening is well-described by Fermi's golden rule in the polariton frame. We also provide purely analytic approximations which accurately describe the system dynamics in the limit of longer polariton timescales

Exact mode volume and Purcell factor of open optical systems

The Purcell factor quantifies the change of the radiative decay of a dipole in an electromagnetic environment relative to free space. Designing this factor is at the heart of photonics technology, striving to develop ever smaller or less lossy optical resonators. The Purcell factor can be expressed using the electromagnetic eigenmodes of the resonators, introducing the notion of a mode volume for each mode. This approach allows to use an analytic treatment, consisting only of sums over eigenmode resonances, a so-called spectral representation. We show in the present work that the expressions for the mode volumes known and used in literature are only approximately valid for modes of high quality factor, while in general they are incorrect. We rectify this issue, introducing the exact normalization of modes. We present an analytic theory of the Purcell effect based on the exact mode normalization and resulting effective mode volume. We use a homogeneous dielectric sphere in vacuum, which is analytically solvable, to exemplify these findings.Comment: Letter: 5 pages, 2 figures. Supplementary material: 16 pages, 10 figure

Controlled strong coupling and absence of dark polaritons in microcavities with double quantum wells

We demonstrate an efficient switching between strong and weak exciton-photon coupling regimes in microcavity-embedded asymmetric double quantum wells, controlled by an applied electric field. We show that a fine tuning of the electric field leads to drastic changes in the polariton properties, with the polariton ground state being red-shifted by a few meV and having acquired prominent features of a spatially indirect dipolar exciton. We study the properties of dipolar exciton polaritons, called dipolaritons, on a microscopic level and show that, unlike recent findings, they are not dark polaritons but, owing to the finite size of the excition, are mixed states with comparable contribution of the cavity photon, bright direct, and long-living indirect exciton modes.Comment: 5 pages, 5 figures, and supplementary materia

Comment on "Dephasing Times in Quantum Dots due to Elastic LO Phonon-Carrier Collisions"

This paper is a Comment on Phys. Rev. Lett. 85, 1516 (2000) by A.V. Uskov, A.-P. Jauho, B. Tromborg, J. Mork, and R. Lang.Comment: 1 page, 1 figure. Phys. Rev. Lett., accepte