Spin Dynamical Properties of the Layered Perovskite La1.2Sr1.8Mn2O7

Inelastic neutron-scattering measurements were performed on a single crystal of the layered colossal magnetoresistance (CMR) material La1.2Sr1.8Mn2O7 (Tc ~ 120K). We found that the spin wave dispersion is almost perfectly two-dimensional with the in-plane spin stiffness constant D ~ 151meVA. The value is similar to that of similarly doped La1-xSrxMnO3 though its Tc is three times higher, indicating a large renormalization due to low dimensionality. There exist two branches due to a coupling between layers within a double-layer. The out-of-plane coupling is about 30% of the in-plane coupling though the Mn-O bond lengths are similar.Comment: 3 pages, 3 figures J. Phys. Chem. Solids in pres

Interplay of the CE-type charge ordering and the A-type spin ordering in a half-doped bilayer manganite La{1}Sr{2}Mn{2}O{7}

We demonstrate that the half-doped bilayer manganite La_{1}Sr_{2}Mn_{2}O_{7} exhibits CE-type charge-ordered and spin-ordered states below $T_{N, CO}^A = 210$ K and below $T_{N}^{CE} \sim 145$ K, respectively. However, the volume fraction of the CE-type ordering is relatively small, and the system is dominated by the A-type spin ordering. The coexistence of the two types of ordering is essential to understand its transport properties, and we argue that it can be viewed as an effective phase separation between the metallic $d(x^{2}-y^{2})$ orbital ordering and the charge-localized $d(3x^{2}-r^{2})/d(3y^{2}-r^{2})$ orbital ordering.Comment: 5 pages, 4 figures, submitted to Phys. Rev.

Novel stripe-type charge ordering in the metallic A-type antiferromagnet Pr{0.5}Sr{0.5}MnO{3}

We demonstrate that an A-type antiferromagnetic (AFM) state of Pr{0.5}Sr{0.5}MnO{3} exhibits a novel charge ordering which governs the transport property. This charge ordering is stripe-like, being characterized by a wave vector q ~ (0,0,0.3) with very anisotropic correlation parallel and perpendicular to the stripe direction. This charge ordering is specific to the manganites with relatively wide one-electron band width (W) which often exhibit a metallic A-type AFM state, and should be strictly distinguished from the CE-type checkerboard-like charge ordering which is commonly observed in manganites with narrower W such as La{1-x}Ca{x}MnO{3} and Pr{1-x}Ca{x}MnO{3}.Comment: REVTeX4, 5 pages, 4 figure

Large thermal Hall coefficient in bismuth

We present a systematical study of thermal Hall effect on a bismuth single crystal by measuring resistivity, Hall coefficient, and thermal conductivity under magnetic field, which shows a large thermal Hall coefficient comparable to the largest one in a semiconductor HgSe. We discuss that this is mainly due to a large mobility and a low thermal conductivity comparing theoretical calculations, which will give a route for controlling heat current in electronic devices.Comment: 4pages, 3 figure

Spin and orbital ordering in double-layered manganites

We study theoretically the phase diagram of the double-layered perovskite manganites taking into account the orbital degeneracy, the strong Coulombic repulsion, and the coupling with the lattice deformation. Observed spin structural changes as the increased doping are explained in terms of the orbital ordering and the bond-length dependence of the hopping integral along $c$-axis. Temperature dependence of the neutron diffraction peak corresponding to the canting structure is also explained. Comparison with the 3D cubic system is made.Comment: 7 figure

Spin dynamical properties and orbital states of the layered perovskite La_2-2x_Sr_1+2x_Mn_2_O_7 (0.3 <= x < 0.5)

Low-temperature spin dynamics of the double-layered perovskite La_2-2x_Sr_1+2x_Mn_2_O_7 (LSMO327) was systematically studied in a wide hole concentration range (0.3 <= x < 0.5). The spin-wave dispersion, which is almost perfectly 2D, has two branches due to a coupling between layers within a double-layer. Each branch exhibits a characteristic intensity oscillation along the out-of-plane direction. We found that the in-plane spin stiffness constant and the gap between the two branches strongly depend on x. By fitting to calculated dispersion relations and cross sections assuming Heisenberg models, we have obtained the in-plane (J_para), intra-bilayer (J_perp) and inter-bilayer (J') exchange interactions at each x. At x=0.30, J_para=-4meV and J_perp=-5meV, namely almost isotropic and ferromagnetic. Upon increasing x, J_perp rapidly approaches zero while |J_para| increases slightly, indicating an enhancement of the planar magnetic anisotropy. At x=0.48, J_para reaches -9meV, while J_perp turns to +1meV indicating an antiferromagnetic interaction. Such a drastic change of the exchange interactions can be ascribed to the change of the relative stability of the d_x^2-y^2 and d_3z^2-r^2 orbital states upon doping. However, a simple linear combination of the two states results in an orbital state with an orthorhombic symmetry, which is inconsistent with the tetragonal symmetry of the crystal structure. We thus propose that an ``orbital liquid'' state realizes in LSMO327, where the charge distribution symmetry is kept tetragonal around each Mn site.Comment: 10 pages including 7 figure

Observation of anomalous single-magnon scattering in half-metallic ferromagnets by chemical pressure control

Temperature variation of resistivity and specific heat have been measured for prototypical half-metallic ferromagnets, R_0.6Sr_0.4MnO_3, with controlling the one-electron bandwidth W. We have found variation of the temperature scalings in the resistivity from T^2 (R = La, and Nd) to T^3 (R = Sm), and have interpreted the $T^3-law in terms of the anomalous single-magnon scattering (AMS) process in the half-metallic system.Comment: To appear in Phys. Rev. Lett., 3 pages + 4 EPS figure