Relaxation time spectrum of low-energy excitations in one- and two-dimensional materials with charge or spin density waves

The long-time thermal relaxation of (TMTTF)$_2$Br, Sr$_{14}$Cu$_{24}$O$_{41}$ and Sr$_2$Ca$_{12}$Cu$_{24}$O$_{41}$ single crystals at temperatures below 1 K and magnetic field up to 10 T is investigated. The data allow us to determine the relaxation time spectrum of the low energy excitations caused by the charge-density wave (CDW) or spin-density wave (SDW). The relaxation time is mainly determined by a thermal activated process for all investigated materials. The maximum relaxation time increases with increasing magnetic field. The distribution of barrier heights corresponds to one or two Gaussian functions. The doping of Sr$_{14-x}$Ca$_{x}$Cu$_{24}$O$_{41}$ with Ca leads to a drastic shift of the relaxation time spectrum to longer time. The maximum relaxation time changes from 50 s (x = 0) to 3000 s (x = 12) at 0.1 K and 10 T. The observed thermal relaxation at x=12 clearly indicates the formation of the SDW ground state at low temperatures

Toward equilibrium ground state of charge density waves in rare-earth tritellurides

We show that the charge density wave (CDW) ground state below the Peierls transition temperature, $T_{CDW}$, of rare-earth tritellurides is not at its equilibrium value, but depends on the time where the system was kept at a fixed temperature below $T_{CDW}$. This ergodicity breaking is revealed by the increase of the threshold electric field for CDW sliding which depends exponentially on time. We tentatively explain this behavior by the reorganization of the oligomeric (Te$_x$)$^{2-}$ sequence forming the CDW modulation.Comment: 10 pages, 5 figures, accepted in PR

Anomalous asymmetry of magnetoresistance in NbSe3_3 single crystals

A pronounced asymmetry of magnetoresistance with respect to the magnetic field direction is observed for NbSe$_3$ crystals placed in a magnetic field perpendicular to their conducting planes. It is shown that the effect persists in a wide temperature range and manifests itself starting from a certain magnetic induction value $B_0$, which at $T=4.2$ K corresponds to the transition to the quantum limit, i.to the state where the Landay level splitting exceeds the temperature.Comment: 4 pages, 6 figures, to be appeared in JETP Let

Charge density wave sliding driven by an interplay of conventional and Hall voltages in NbSe3_3 microbridges

Collective charge-density wave (CDW) transport was measured under a high magnetic field in NbSe$_3$ microbridges which have been cut transversely and at an angle to the chains' direction. We give evidences that the CDW sliding is driven by the Hall voltage generated by the inter-chain current of normal carriers. We have discovered a re-entrance effect of the Hall-driven sliding above a crossover temperature at which the Hall constant has been known to change sign. For the narrow channel, cut at 45$^\circ$ relative to the chain axis, we observed an evolution from the Hall-driven sliding at low temperatures, to the conventional sliding at higher temperatures, which corroborates with falling of the Hall constant. In this course, the nonlinear contribution to the conductivity coming from the collective sliding changes sign. The quantization of Shapiro-steps, generated presumably by a coherent sequence of phase slips, indicates that their governing changes from the applied voltage to the current.Comment: 6 pages, 5 figures, accepted in PR

Luttinger-liquid-like transport in long InSb nanowires

Long nanowires of degenerate semiconductor InSb in asbestos matrix (wire diameter is around 50 \AA, length 0.1 - 1 mm) were prepared. Electrical conduction of these nanowires is studied over a temperature range 1.5 - 350 K. It is found that a zero-field electrical conduction is a power function of the temperature $G\propto T^\alpha$ with the typical exponent $\alpha \approx 4$. Current-voltage characteristics of such nanowires are found to be nonlinear and at sufficiently low temperatures follows the power law $I\propto V^\beta$. It is shown that the electrical conduction of these nanowires cannot be accounted for in terms of ordinary single-electron theories and exhibits features expected for impure Luttinger liquid. For a simple approximation of impure LL as a pure one broken into drops by weak links, the estimated weak-link density is around $10^3-10^4$ per cm.Comment: 5 pages, 2 figure

Fractional power-law susceptibility and specific heat in low temperature insulating state of o-TaS_{3}

Measurements of the magnetic susceptibility and its anisotropy in the quasi-one-dimensional system o-TaS_{3} in its low-T charge density wave (CDW) ground state are reported. Both sets of data reveal below 40 K an extra paramagnetic contribution obeying a power-law temperature dependence \chi(T)=AT^{-0.7}. The fact that the extra term measured previously in specific heat in zero field, ascribed to low-energy CDW excitations, also follows a power law C_{LEE}(0,T)=CT^{0.3}, strongly revives the case of random exchange spin chains. Introduced impurities (0.5% Nb) only increase the amplitude C, but do not change essentially the exponent. Within the two-level system (TLS) model, we estimate from the amplitudes A and C that there is one TLS with a spin s=1/2 localized on the chain at the lattice site per cca 900 Ta atoms. We discuss the possibility that it is the charge frozen within a soliton-network below the glass transition T_{g}~40 K determined recently in this system.Comment: 7 pages, 3 figures, submitted to Europhysics Letter

Statistics of charged solitons and formation of stripes

The 2-fold degeneracy of the ground state of a quasi-one-dimensional system allows it to support topological excitations such as solitons. We study the combined effects of Coulomb interactions and confinement due to interchain coupling on the statistics of such defects. We concentrate on a 2D case which may correspond to monolayers of polyacetylene or other charge density waves. The theory is developped by a mapping to the 2D Ising model with long-range 4-spin interactions. The phase diagram exhibits deconfined phases for liquids and Wigner crystals of kinks and confined ones for bikinks. Also we find aggregated phases with either infinite domain walls of kinks or finite rods of bikinks. Roughening effects due to both temperature and Coulomb repulsion are observed. Applications may concern the melting of stripes in doped correlated materials.Comment: 16 pages, 7 figure

Low-temperature conductivity of quasi-one-dimensional conductors: Luttinger liquid stabilized by impurities

A new non-Fermi-liquid state of quasi-one-dimensional conductors is suggested in which electronic system exists in a form of collection of bounded Luttinger liquids stabilized by impurities. This state is shown to be stable towards interchain electron hopping at low temperatures. Electronic spectrum of the system contains zero modes and collective excitations of the bounded Luttinger liquids in the segments between impurities. Zero modes give rise to randomly distributed localized electronic levels, and long-range interaction generates the Coulomb gap in the density of states at the Fermi energy. Mechanism of conductivity at low temperatures is phonon-assisted hopping via zero-mode states. At higher voltages the excitations of Luttinger liquid are involved in electron transport, and conductivity obeys power-law dependence on voltage. The results provide a qualitative explanation for recent experimental data for NbSe3 and TaS3 crystals.Comment: 12 pages, 1 figur