A class of Heisenberg models with the orthogonal dimer ground states

Extensions of the Shastry-Sutherland model are possible in various ways. In particular, it is possible to construct a natural model in three dimensions which has the exact dimer ground state. Recently found spin gap system SrCu_2(BO_3)_2 has this structure. The exchange constants between the layers is expected to be smaller than the intra-layer couplings. However, the exactness of the dimer state for the three dimensional structure is important to understand why magnetic properties of SrCu_2(BO_3)_2 are described well by the two dimensional model.Comment: 3 pages, 5 figures, to appear in Journal of Physics: Condensed Matte

Low-Lying Magnetic Excitation of the Shastry-Sutherland Model

By using perturbation calculation and numerical diagonalization, low-energy spin dynamics of the Shastry-Sutherland model is investigated paying particular attention to the two-particle coherent motion. In addition to spin-singlet- and triplet bound states, we find novel branches of coherent motion of a bound quintet pair, which are usually unstable because of repulsion. Unusual dispersion observed in neutron-scattering measurements are explained by the present theory. The importance of the effects of phonon is also pointed out.Comment: 4 pages, 6 figures combined into 1 PSfile. Final version to appear in Phys.Rev.Lett. (Jan. 2000

Magnon Dispersion and Anisotropies in SrCu2_2(BO3_3)2_2

We study the dispersion of the magnons (triplet states) in SrCu$_2$(BO$_3$)$_2$ including all symmetry-allowed Dzyaloshinskii-Moriya interactions. We can reduce the complexity of the general Hamiltonian to a new simpler form by appropriate rotations of the spin operators. The resulting Hamiltonian is studied by both perturbation theory and exact numerical diagonalization on a 32-site cluster. We argue that the dispersion is dominated by Dzyaloshinskii-Moriya interactions. We point out which combinations of these anisotropies affect the dispersion to linear-order, and extract their magnitudes.Comment: 11 pages, 7 figures, 1 table, v2 conclusion shortened, figs clarifie

Strong coupling theory of the spinless charges on the triangular lattices: possibility of a new quantum liquid

We propose a new type of charge liquid state in the spinless fermion system on a triangular lattice under strong inter-site Coulomb interactions, $V$. In the strong coupling limit ($t=0$), the ground state is classical and disordered due to geometrical frustration. The introduction of small t will drive the system to a partially ordered phase which we call a "pinball liquid". A possibly long range ordered Wigner crystal solid coexist with a liquid component which are moving around them like a pinball. This liquid is dominant over wide range of filling, even away from the regular triangle, and is also realized in the hard core boson systems. Relevance to the organic theta-ET_2X is discsussed.Comment: 4pages, 7figure

Ferroelectricity induced by spin-dependent metal-ligand hybridization in Ba2_2CoGe2_2O7_7

We have investigated the variation of induced ferroelectric polarization under magnetic field with various directions and magnitudes in a staggered antiferromagnet Ba$_2$CoGe$_2$O$_7$. While the ferroelectric polarization cannot be explained by the well-accepted spin current model nor exchange striction mechanism, we have shown that it is induced by the spin-dependent $p$-$d$ hybridization between the transition-metal (Co) and ligand (O) via the spin-orbit interaction. On the basis of the correspondence between the direction of electric polarization and the magnetic state, we have also demonstrated the electrical control of the magnetization direction.Comment: 4 pages, 4 figure

Field-Induced Effects of Anisotropic Magnetic Interactions in SrCu2(BO3)2

We observed a field-induced staggered magnetization in the 2D frustrated dimer-singlet spin system SrCu2(BO3)2 by 11B NMR, from which the magnitudes of the intradimer Dzyaloshinsky-Moriya interaction and the staggered g-tensor were determined. These anisotropic interactions cause singlet-triplet mixing and eliminate a quantum phase transition at the expected critical field Hc for gap closing. They also provide a quantitative account for some puzzling phenomena such as the onset of a uniform magnetization below the and the persistence of the excitation gap above Hc. The gap was accurately determined from the activation energy of the nuclear relaxation rate.Comment: 8 pages, 5 figures, published versio