1 research outputs found
Electronic transport in films of colloidal CdSe nanocrystals
We present results for electronic transport measurements on large
three-dimensional arrays of CdSe nanocrystals. In response to a step in the
applied voltage, we observe a power-law decay of the current over five orders
of magnitude in time. Furthermore, we observe no steady-state dark current for
fields up to 10^6 V/cm and times as long as 2x10^4 seconds. Although the
power-law form of the decay is quite general, there are quantitative variations
with temperature, applied field, sample history, and the material parameters of
the array. Despite evidence that the charge injected into the film during the
measurement causes the decay of current, we find field-scaling of the current
at all times. The observation of extremely long-lived current transients
suggests the importance of long-range Coulomb interactions between charges on
different nanocrystals.Comment: 11 pages, 10 figure