375 research outputs found
Dzyaloshinsky-Moriya interaction in vesignieite: A route to freezing in a quantum kagome antiferromagnet
We report an electron spin resonance investigation of the geometrically
frustrated spin-1/2 kagome antiferromagnet vesignieite,
BaCuVO(OH). Analysis of the line widths and line shifts
indicates the dominance of in-plane Dzyaloshinsky-Moriya anisotropy that is
proposed to suppress strongly quantum spin fluctuations and thus to promote
long-range ordering rather than a spin-liquid state. We also evidence an
enhanced spin-phonon contribution that might originate from a lattice
instability and discuss the origin of a low-temperature mismatch between
intrinsic and bulk susceptibility in terms of local inhomogeneity
Ga-NMR local susceptibility of the kagome-based magnet SrCr_9pGa_(12-9p)O_19. A high temperature study
We report a high- Ga-NMR study in the kagome-based antiferromagnetic
compound SrCrGaO (), and present a
refined mean-field analysis of the high T local NMR susceptibility of Cr
frustrated moments. We find that the intralayer kagome coupling is K,
and the interlayer coupling through non-kagome Cr moments is K. The ratio confirms the common belief that
the frustrated entity is a pyrochlore slab.Comment: 8 pages, 4 figures Conference paper: Highly Frustrated Magnetism
2000, Waterloo (Canada) Submitted to Canadian Journal of Physic
Interplay of thermal and quantum spin fluctuations on the kagome lattice
We present a Raman spectroscopic investigation of the Herbertsmithite
ZnCu3(OH)6Cl2, the first realization of a Heisenberg s=1/2 antiferromagnet on a
perfect kagome lattice. The magnetic excitation spectrum of this compound is
dominated by two components, a high temperature quasi elastic signal and a low
temperature, broad maximum. The latter has a linear low energy slope and
extends to high energy. We have investigated the temperature dependence and
symmetry properties of both signals. Our data agree with previous calculations
and point to a spin liquid ground state.Comment: 5 figure
Antiferromagnetic correlations and impurity broadening of NMR linewidths in cuprate superconductors
We study a model of a d-wave superconductor with strong potential scatterers
in the presence of antiferromagnetic correlations and apply it to experimental
nuclear magnetic resonance (NMR) results on Zn impurities in the
superconducting state of YBCO. We then focus on the contribution of
impurity-induced paramagnetic moments, with Hubbard correlations in the host
system accounted for in Hartree approximation. We show that local magnetism
around individual impurities broadens the line, but quasiparticle interference
between impurity states plays an important role in smearing out impurity
satellite peaks. The model, together with estimates of vortex lattice effects,
provides a semi-quantitative description of the impurity concentration
dependence of the NMR line shape in the superconducting state, and gives a
qualitative description of the temperature dependence of the line asymmetry. We
argue that impurity-induced paramagnetism and resonant local density of states
effects are both necessary to explain existing experiments.Comment: 15 pages, 23 figures, submitted to Phys. Rev.
Quantum Kagome antiferromagnet ZnCu3(OH)6Cl2
The frustration of antiferromagnetic interactions on the loosely connected
kagome lattice associated to the enhancement of quantum fluctuations for S=1/2
spins was acknowledged long ago as a keypoint to stabilize novel ground states
of magnetic matter. Only very recently, the model compound Herbersmithite,
ZnCu3(OH)6Cl2, a structurally perfect kagome antiferromagnet, could be
synthesized and enables a close comparison to theories. We review and classify
various experimental results obtained over the past years and underline some of
the pending issues.Comment: 23 pages, 16 figures, invited paper in J. Phys. Soc. Jpn, special
topics issue on "Novel States of Matter Induced by Frustration", to be
published in Jan. 201
A numerical test of differential equations for one- and two-loop sunrise diagrams using configuration space techniques
We use configuration space methods to write down one-dimensional integral
representations for one- and two-loop sunrise diagrams (also called Bessel
moments) which we use to numerically check on the correctness of the second
order differential equations for one- and two-loop sunrise diagrams that have
recently been discussed in the literature.Comment: 11 pages, no figures, published versio
Low-energy spin dynamics of the s = 1/2 kagome system herbertsmithite
The low-energy (epsilon = (h) over bar < 1 meV), low-temperature (T = 0.05 K) spin dynamics of the s = 1/2 kagome candidate herbertsmithite are probed in the presence of magnetic fields up to 2.5 T. The zero-field spectra reveal a very weak continuum of scattering at T = 10 K and a broad inelastic peak centred at epsilon(max) = 0.2 meV at lower temperatures, T < 1 K. The broad peak is found to be strongly damped, with a liquid-like structure factor implying correlations at length scales up to r = 6 angstrom. The field dependence of the peak appears to follow the Zeeman splitting of s = 1/2 excitations, consistent with the weakly split 'doublets' observed in low-temperature specific heat. A possible explanation of these observations is a short-range correlated state involving defect spins between the kagome planes and moments in the kagome layers
Spin dynamics and disorder effects in the S=1/2 kagome Heisenberg spin liquid phase of kapellasite
We report Cl NMR, ESR, SR and specific heat measurements on the
frustrated kagom\'e magnet kapellasite,
CuZn(OH)Cl, where a gapless spin liquid phase is
stabilized by a set of competing exchange interactions. Our measurements
confirm the ferromagnetic character of the nearest-neighbour exchange
interaction and give an energy scale for the competing interactions K. The study of the temperature-dependent ESR lineshift reveals a
moderate symmetric exchange anisotropy term , with %. These
findings validate a posteriori the use of the Heisenberg
model to describe the magnetic properties of kapellasite [Bernu et al., Phys.
Rev. B 87, 155107 (2013)]. We further confirm that the main deviation from this
model is the severe random depletion of the magnetic kagom\'e lattice by 27%,
due to Cu/Zn site mixing, and specifically address the effect of this disorder
by Cl NMR, performed on an oriented polycrystalline sample.
Surprisingly, while being very sensitive to local structural deformations, our
NMR measurements demonstrate that the system remains homogeneous with a unique
spin susceptibility at high temperature, despite a variety of magnetic
environments. Unconventional spin dynamics is further revealed by NMR and
SR in the low-, correlated, spin liquid regime, where a broad
distribution of spin-lattice relaxation times is observed. We ascribe this to
the presence of local low-energy modes.Comment: 15 pages, 11 figures. To appear in Phys. Rev.
Spinless impurities in high Tc cuprates: Kondo-like behavior
We compare the effects of in-plane non magnetic Li and Zn
impurities on the normal state of high-T cuprates. Y NMR shows that the
extra hole introduced by Li is not localized in its vicinity. The Tc depression
and induced moments on near neighbour Cu sites of Zn or Li are found identical.
These universal effects of spinless impurities establish the major influence of
the spin perturbation with respect to the charge defect. The susceptibility of
the induced moment measured by Li NMR displays a 1/(T+Theta) behavior. Theta
increases with doping up to about 200 K in the overdoped regime. We attribute
this to a "Kondo like" effect.Comment: To appear in Phys.Rev.Lett. (22 nov. 99) Minor modifications compared
to previous version. 8 pages (4 pages for text + 4 figures
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