Squeezed state evolution and entanglement in lossy coupled resonator optical waveguides

We investigate theoretically the temporal evolution of a squeezed state in lossy coupled-cavity systems. We present a general formalism based upon the tight binding approximation and apply this to a two-cavity system as well as to a coupled resonator optical waveguide in a photonic crystal. We derive analytical expressions for the number of photons and the quadrature noise in each cavity as a function of time when the initial excited state is a squeezed state in one of the cavities. We also analytically evaluate the time dependant cross correlation between the photons in different cavities to evaluate the degree of quantum entanglement. We demonstrate the effects of loss on the properties of the coupled-cavity systems and derive approximate analytic expressions for the maximum photon number, maximum squeezing and maximum entanglement for cavities far from the initially excited cavity in a lossless coupled resonator optical waveguide.Comment: 10 pages, 6 figure

Third Harmonic THz Generation from Graphene in a Parallel-Plate Waveguide

Graphene as a zero-bandgap two-dimensional semiconductor with a linear electron band dispersion near the Dirac points has the potential to exhibit very interesting nonlinear optical properties. In particular, third harmonic generation of terahertz radiation should occur due to the nonlinear relationship between the crystal momentum and the current density. In this work, we investigate the terahertz nonlinear response of graphene inside a parallel-plate waveguide. We optimize the plate separation and Fermi energy of the graphene to maximize third harmonic generation, by maximizing the nonlinear interaction while minimizing the loss and phase mismatch. The results obtained show an increase by more than a factor of 100 in the power efficiency relative to a normal-incidence configuration for a 2 terahertz incident field

High harmonic generation in undoped graphene: Interplay of inter- and intraband dynamics

We develop a density matrix formalism in the length gauge to calculate the nonlinear response of intrinsic monolayer graphene at terahertz frequencies. Employing a tight-binding model, we find that the interplay of the interband and intraband dynamics leads to strong harmonic generation at moderate field amplitudes. In particular, we find that at low temperature, the reflected field of undoped suspended graphene exhibits a third harmonic amplitude that is 32% of the fundamental for an incident field of 100 V/cm. Moreover, we find that up to the seventh harmonic and beyond are generated

Valley-polarization in biased bilayer graphene using circularly polarized light

Achieving a population imbalance between the two inequivalent valleys is a critical first step for any valleytronic device. A valley-polarization can be induced in biased bilayer graphene using circularly polarized light. In this paper, we present a detailed theoretical study of valley-polarization in biased bilayer graphene. We show that a nearly perfect valley-polarization can be achieved with the proper choices of external bias and pulse frequency. We find that the optimal pulse frequency $\omega$ is given by $\hbar\omega=2a,$ where $2a$ is the potential energy difference between the graphene layers. We also find that the valley-polarization originates not from the Dirac points themselves, but rather from a ring of states surrounding each. Intervalley scattering is found to greatly reduce the valley-polarization for high frequency pulses. Thermal populations are found to significantly reduce the valley-polarization for small biases. This work provides insight into the origin of valley-polarization in bilayer graphene and will aid experimentalists seeking to study valley-polarization in the lab.Comment: 18 pages, 9 figures, v2: elaboration and readability improvement

Optimized nonlinear terahertz response of graphene in a parallel-plate waveguide

Third harmonic generation of terahertz radiation is expected to occur in monolayer graphene due to the nonlinear relationship between the crystal momentum and the current density. In this work, we calculate the terahertz nonlinear response of graphene inside a parallel-plate waveguide including pump depletion, self-phase, and cross-phase modulation. To overcome the phase mismatching between the pump field and third-harmonic field at high input fields due to self-phase and cross-phase modulation, we design a waveguide with two dielectric layers with different indices of refraction. We find that, by tuning the relative thicknesses of the two layers, we are able to improve phase matching, and thereby increase the power efficiency of the system by more than a factor of two at high powers. With this approach, we find that dispite the loss in this system, for an incident frequency of $2$ THz, we are able to achieve power efficiencies of $75 \%$ for graphene with low Fermi energies of $20$ meV and up to $35\%$ when the Fermi energy is $100$ meV

The effects of microscopic scattering on terahertz third harmonic generation in monolayer graphene

Due to its linear dispersion, monolayer graphene is expected to generate a third harmonic response at terahertz frequencies. There have been a variety of different models of this effect and recently it has been experimentally observed. However, there is still considerable uncertainty as to the role of scattering on harmonic generation in graphene. In this work, we model third-harmonic generation in doped monolayer graphene at THz frequencies by employing a nearest-neighbour tight-binding model in the length gauge. We include optical phonon and neutral impurity scattering at the microscopic level, and examine the effects of scattering on the third harmonic response. We also compare the results of a phenomenological semiclassical theory, using a field-dependent scattering time extracted from the simulation, and find a significantly lower third harmonic field than that found from the microscopic model. This demonstrates that third-harmonic generation is much more sensitive to the nature of the scattering than is the linear response. We also compare the results of our full simulation to recent experimental results and find qualitative agreement

Optimization of a Lossy Microring Resonator System for the Generation of Quadrature-Squeezed States

The intensity buildup of light inside a lossy microring resonator can be used to enhance the generation of squeezed states via spontaneous parametric downconversion (SPDC). In this work, we model the generation of squeezed light in a microring resonator that is pumped with a Gaussian pulse via a side-coupled channel waveguide. We theoretically determine the optimum pump pulse duration and ring-to-channel coupling constant to minimize the quadrature noise (maximize the squeezing) in the ring for a fixed input pump energy. We derive approximate analytic expressions for the optimal coupling and pump pulse duration as a function of scattering loss in the ring. These results will enable researchers to easily determine the optimal design of microring resonator systems for the generation of quadrature-squeezed states.Comment: 16 pages, 11 figure

Continuous-variable entanglement in a two-mode lossy cavity: an exact solution

Continuous-variable (CV) entanglement is a valuable resource in the field of quantum information. One source of CV entanglement is the correlations between the position and momentum of photons in a two-mode squeezed state of light. In this paper, we theoretically study the generation of squeezed states, via spontaneous parametric downconversion (SPDC), inside a two-mode lossy cavity that is pumped with a classical optical pulse. The dynamics of the density operator in the cavity is modelled using the Lindblad master equation, and we show that the exact solution to this model is the density operator for a two-mode squeezed thermal state, with a time-dependent squeezing amplitude and average thermal photon number for each mode. We derive an expression for the maximum entanglement inside the cavity that depends crucially on the difference in the losses between the two modes. We apply our exact solution to the important example of a microring resonator that is pumped with a Gaussian pulse. The expressions that we derive will help researchers optimize CV entanglement in lossy cavities.Comment: 12 pages, 6 figure

Counterpropagating continuous variable entangled states in lossy coupled-cavity optical waveguides

We present an integrated source of counterpropagating entangled states based on a coupled resonator optical waveguide that is pumped by a classical pulsed source incident from above the waveguide. We investigate theoretically the generation and propagation of continuous variable entangled states in this coupled-cavity system in the presence of intrinsic loss. Using a tight-binding approximation, we derive analytic time-dependent expressions for the number of photons in each cavity, as well as for the correlation variance between the photons in different pairs of cavities, to evaluate the degree of quantum entanglement. We also derive simple approximate expressions for these quantities that can be used to guide the design of such systems, and discuss how pumping configurations and physical properties of the system affect the photon statistics and the degree of quantum correlation.Comment: 14 pages, 9 figure

The impact of nitrogen doping on the linear and nonlinear terahertz response of graphene

It is well known that impurities play a central role in the linear and nonlinear response of graphene at optical and terahertz frequencies. In this work, we calculate the bands and intraband dipole connection elements for nitrogen-doped monolayer graphene using a density functional tight binding approach. Employing these results, we calculate the linear and nonlinear response of the doped graphene to terahertz pulses using a density-matrix approach in the length gauge. We present the results for the linear and nonlinear mobility as well as third harmonic generation in graphene for adsorbed and substitutional nitrogen doping for a variety of doping densities. We show that the conduction bands are more parabolic in graphene structures with substitutional nitrogen doping than for those with adsorbed nitrogen. As a result, substitutional doping has a greater impact on the terahertz mobility and nonlinear response of graphene than adsorbed nitrogen does.Comment: 16 pages, 9 figure