Usage History of Scientific Literature: Nature Metrics and Metrics of Nature Publications

In this study, we analyze the dynamic usage history of Nature publications over time using Nature metrics data. We conduct analysis from two perspectives. On the one hand, we examine how long it takes before the articles' downloads reach 50%/80% of the total; on the other hand, we compare the percentage of total downloads in 7 days, 30 days, and 100 days after publication. In general, papers are downloaded most frequently within a short time period right after their publication. And we find that compared with Non-Open Access papers, readers' attention on Open Access publications are more enduring. Based on the usage data of a newly published paper, regression analysis could predict the future expected total usage counts.Comment: 11 pages, 5 figures and 4 table

A Review of Electrospun Carbon Fibers as Electrode Materials for Energy Storage

The applications of electrospun carbon fiber webs to the development of energy storages devices, including both supercapacitors and lithium ion batteries (LIB) , are reviewed. Following a brief discussion of the fabrication process and characterization methods for ultrafine electrospun carbon fibers, recent advances in their performance as supercapacitors and LIBs anode materials are summarized. Optimization of the overall electrochemical properties of these materials through choice of thermal treatment conditions, incorporation of additional active components (such as carbon nanotubes, metal oxides, and catalysts), and generation of novel fibrous structures (such as core-shell, multi-channel or porous fibers) is highlighted. Further challenges related to improving the conductivity, surface area, and mechanical properties of the carbon nanofiber webs, as well as the scale-up ability of the fabrication technique, are discussed.United States. Dept. of Energ

Metallocene/carbon hybrids prepared by a solution process for supercapacitor applications

Efficient and scalable solution-based processes are not generally available to integrate well-studied pseudocapacitive materials (i.e., metal oxides and conducting polymers) with other components such as porous carbon, mainly because these classes of pseudocapacitive systems have poor solubilities in solvents and exhibit no specific interactions with the other component. Here we report, for the first time, the integration of a metallocene polymer, polyvinylferrocene (PVF), with carbon nanotubes (CNTs) via a simple solution process for supercapacitor applications. The solution processability of the PVF/CNT hybrid is due to the high solubilities of PVF in organic solvents and the unique ability of the metallocene/carbon system to form stable dispersions through the π–π stacking interactions between the two components. The nanostructure and electrochemical properties of the hybrid can be manipulated systematically by adjusting the composition of the dispersion. The hybrid with the optimized composition exhibits unusually high capacitance (1452 F g[superscript −1]) and energy density (79.5 W h kg[superscript −1]) obtained in a standard two-electrode configuration, outperforming previously reported pseudocapacitive materials.United States. Dept. of EnergyMIT Energy Initiative (Seed Fund Grant