187 research outputs found
A parity-breaking electronic nematic phase transition in the spin-orbit coupled metal CdReO
Strong electron interactions can drive metallic systems toward a variety of
well-known symmetry-broken phases, but the instabilities of correlated metals
with strong spin-orbit coupling have only recently begun to be explored. We
uncovered a multipolar nematic phase of matter in the metallic pyrochlore
CdReO using spatially resolved second-harmonic optical anisotropy
measurements. Like previously discovered electronic nematic phases, this
multipolar phase spontaneously breaks rotational symmetry while preserving
translational invariance. However, it has the distinguishing property of being
odd under spatial inversion, which is allowed only in the presence of
spin-orbit coupling. By examining the critical behavior of the multipolar
nematic order parameter, we show that it drives the thermal phase transition
near 200 kelvin in CdReO and induces a parity-breaking lattice
distortion as a secondary order.Comment: 9 pages main text, 4 figures, 10 pages supplementary informatio
Field Dependent Phase Diagram of the Quantum Spin Chain (CH3)2NH2CuCl3
Although (CH3)2NH2CuCl3 (MCCL) was first examined in the 1930's [1], there
are open questions regarding the magnetic dimensionality and nature of the
magnetic properties. MCCL is proposed to be a S=1/2 alternating ferromagnetic
antiferromagnetic spin chain alternating along the crystalline a-axis [2,3].
Proposed ferromagnetic (JFM =1.3 meV) and antiferromagnetic (JAFM =1.1 meV)
exchange constants make this system particularly interesting for experimental
study. Because JFM and JAFM are nearly identical, the system should show
competing behavior between S=1/2 (AFM) and S=1(FM) effects. We report low
temperature magnetic field dependent susceptibility, chi(H), and specific heat,
Cp, of MCCL. These provide an initial magnetic-field versus temperature phase
diagram. A zero-field phase transition consistent with long range magnetic
order is observed at T=0.9 K. The transition temperature can be reduced via
application of a magnetic field. We also present comparisons to a FM/AFM dimer
model that accounts for chi(T,H=0) and Cp(H,T).Comment: 2 pages, 1 figure included in text. Submitted to proceedings of 24th
International Conference on Low Temperature Physics, August 200
Static and Dynamic Magnetism in Underdoped Superconductor BaFeCoAs
We report neutron scattering measurements on single crystals of
BaFeCoAs. The magnetic Bragg peak intensity is reduced by
6 % upon cooling through T. The spin dynamics exhibit a gap of 8 meV with
anisotropic three-dimensional (3d) interactions. Below T additional
intensity appears at an energy of 4.5(0.5) meV similar to previous
observations of a spin resonance in other Fe-based superconductors. No further
gapping of the spin excitations is observed below T for energies down to 2
meV. These observations suggest the redistribution of spectral weight from the
magnetic Bragg position to a spin resonance demonstrating the direct
competition between static magnetic order and superconductivity.Comment: 4 pages, 4 figure
Quantum spin correlations in an organometallic alternating sign chain
High resolution inelastic neutron scattering is used to study excitations in
the organometallic magnet DMACuCl. The correct magnetic Hamiltonian
describing this material has been debated for many years. Combined with high
field bulk magnetization and susceptibility studies, the new results imply that
DMACuCl is a realization of the alternating
antiferromagnetic-ferromagnetic (AFM-FM) chain. Coupled-cluster calculations
are used to derive exchange parameters, showing that the AFM and FM
interactions have nearly the same strength. Analysis of the scattering
intensities shows clear evidence for inter-dimer spin correlations, in contrast
to existing results for conventional alternating chains. The results are
discussed in the context of recent ideas concerning quantum entanglement.Comment: 5 pages, 4 figures included in text. Submitted to APS Journal
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