Low-temperature quenching of one-dimensional localised Frenkel excitons

We present a theoretical analysis of low-temperature quenching of one-dimensional Frenkel excitons that are localised by moderate on-site (diagonal) uncorrelated disorder. Exciton diffusion is considered as an incoherent hopping over localization segments and is probed by the exciton fluorescence quenching at point traps. The rate equation is used to calculate the temperature dependence of the exciton quenching. The activation temperature of the diffusion is found to be of the order of the width of the exciton absorption band. We demonstrate that the intra-segment scattering is extremely important for the exciton diffusion. We discuss also experimental data on the fast exciton-exciton annihilation in linear molecular aggregates at low temperatures.Comment: 7 pages, 3 figures, accepted to Chem. Phys. Let

Local level statistics for optical and transport properties of disordered systems at finite temperature

It is argued that the (traditional) global level statistics which determines localization and coherent transport properties of disordered systems at zero temperature (e.g. the Anderson model) becomes inappropriate when it comes to incoherent transport. We define local level statistics which proves to be relevant for finite temperature incoherent transport and optics of one-dimensional systems (e.g. molecular aggregates, conjugated polymers, etc.).Comment: 4 pages, 2 figures, reported at EXCON'2006, to appear in the physica status solidi (c

Optical bistability and hysteresis of hybrid metal-semiconductor nano-dimer

Optical response of an artificial composite nano-dimer comprising a semiconductor quantum dot and a metal nanosphere is analyzed theoretically. We show that internal degrees of freedom of the system can manifest bistability and optical hysteresis as functions of the incident field intensity. We argue that these effects can be observed for the real world systems, such as a CdSe quantum dot and an Au nanoparticle hybrids. These properties can be revealed by measuring the optical hysteresis of the Rayleigh scattering. We show also that the total dipole moment of the system can be switched abruptly between its two stable states by small changes in the excitation intensity. The latter promises various applications in the field of all-optical processing at nanoscale, the most underlying of them being the volatile optical memory.Comment: 6 two column pages, 5 figures, to appear in Phys. Rev.

Fermi Bubbles: an Elephant in the Gamma-ray Sky

The Fermi bubbles are one of the most remarkable features in the gamma-ray sky revealed by the Fermi Large Area Telescope (LAT). The nature of the gamma-ray emission and the origin of the bubbles are still open questions. In this note, we will review some basic features of leptonic and hadronic modes of gamma-ray production. At the moment, gamma rays are our best method to study the bubbles, but in order to resolve the origin of the bubbles multi-wavelength and multi-messenger observations will be crucial.Comment: Published in proceedings for RICAP16 conferenc

Selection of dominant multi-exciton transitions in disordered linear J-aggregates

We show that the third-order optical response of disordered linear J-aggregates can be calculated by considering only a limited number of transitions between (multi-) exciton states. We calculate the pump-probe absorption spectrum resulting from the truncated set of transitions and show that, apart from the blue wing of the induced absorption peak, it agrees well with the exact spectrum.Comment: 8 pages, 2 figures, accepted to Journal of Luminescenc

Galactic center gamma-ray excess and the Fermi bubbles

Galactic center (GC) is expected to be the brightest source of possible dark matter (DM) annihilation signal. Excess gamma-ray emission has been detected by several groups. Both DM and more conventional astrophysical explanations of the excess have been proposed. In this report, we discuss possible effects of modeling the Fermi bubbles at low latitudes on the GC excess. We consider a template of the Fermi bubbles at low latitudes derived by assuming that the spectrum between 1 GeV and 10 GeV at low latitudes is the same as at high latitudes. We argue that the presence of the Fermi bubbles near the GC may have a significant influence on the spectrum of the GC excess, especially at energies above 10 GeV.Comment: Proceedings of LaThuile 2017 conferenc