11,052 research outputs found
High-harmonic generation from arbitrarily oriented diatomic molecules including nuclear motion and field-free alignment
We present a theoretical model of high-harmonic generation from diatomic
molecules. The theory includes effects of alignment as well as nuclear motion
and is used to predict results for N, O, H and D. The results
show that the alignment dependence of high-harmonics is governed by the
symmetry of the highest occupied molecular orbital and that the inclusion of
the nuclear motion in the theoretical description generally reduces the
intensity of the harmonic radiation. We compare our model with experimental
results on N and O, and obtain very good agreement.Comment: 12 pages, 8 figures, 2 tables; legends revised on Figs. 1,3,4,6 and
Observation of force-detected nuclear magnetic resonance in a homogeneous field
We report the experimental realization of BOOMERANG (better observation of magnetization, enhanced resolution, and no gradient), a sensitive and general method of magnetic resonance. The prototype millimeter-scale NMR spectrometer shows signal and noise levels in agreement with the design principles. We present H-1 and F-19 NMR in both solid and liquid samples, including time-domain Fourier transform NMR spectroscopy, multiple-pulse echoes, and heteronuclear J spectroscopy. By measuring a H-1-F-19 J coupling, this last experiment accomplishes chemically specific spectroscopy with force-detected NMR. In BOOMERANG, an assembly of permanent magnets provides a homogeneous field throughout the sample, while a harmonically suspended part of the assembly, a detector, is mechanically driven by spin-dependent forces. By placing the sample in a homogeneous field, signal dephasing by diffusion in a field gradient is made negligible, enabling application to liquids, in contrast to other force-detection methods. The design appears readily scalable to µm-scale samples where it should have sensitivity advantages over inductive detection with microcoils and where it holds great promise for application of magnetic resonance in biology, chemistry, physics, and surface science. We briefly discuss extensions of the BOOMERANG method to the µm and nm scales
High-order harmonic generation from polyatomic molecules including nuclear motion and a nuclear modes analysis
We present a generic approach for treating the effect of nuclear motion in
the high-order harmonic generation from polyatomic molecules. Our procedure
relies on a separation of nuclear and electron dynamics where we account for
the electronic part using the Lewenstein model and nuclear motion enters as a
nuclear correlation function. We express the nuclear correlation function in
terms of Franck-Condon factors which allows us to decompose nuclear motion into
modes and identify the modes that are dominant in the high-order harmonic
generation process. We show results for the isotopes CH and CD and
thereby provide direct theoretical support for a recent experiment [Baker {\it
et al.}, Science {\bf 312}, 424 (2006)] that uses high-order harmonic
generation to probe the ultra-fast structural nuclear rearrangement of ionized
methane.Comment: 6 pages, 6 figure
Classification of String-like Solutions in Dilaton Gravity
The static string-like solutions of the Abelian Higgs model coupled to
dilaton gravity are analyzed and compared to the non-dilatonic case. Except for
a special coupling between the Higgs Lagrangian and the dilaton, the solutions
are flux tubes that generate a non-asymptotically flat geometry. Any point in
parameter space corresponds to two branches of solutions with two different
asymptotic behaviors. Unlike the non-dilatonic case, where one branch is always
asymptotically conic, in the present case the asymptotic behavior changes
continuously along each branch.Comment: 15 pages, 6 figures. To be published in Phys. Rev.
Angular Normal Modes of a Circular Coulomb Cluster
We investigate the angular normal modes for small oscillations about an
equilibrium of a single-component coulomb cluster confined by a radially
symmetric external potential to a circle. The dynamical matrix for this system
is a Laplacian symmetrically circulant matrix and this result leads to an
analytic solution for the eigenfrequencies of the angular normal modes. We also
show the limiting dependence of the largest eigenfrequency for large numbers of
particles
Experimental Bell Inequality Violation with an Atom and a Photon
We report the measurement of a Bell inequality violation with a single atom
and a single photon prepared in a probabilistic entangled state. This is the
first demonstration of such a violation with particles of different species.
The entanglement characterization of this hybrid system may also be useful in
quantum information applications.Comment: 4 pages, 2 figure
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