9,702 research outputs found
High-order harmonic generation from polyatomic molecules including nuclear motion and a nuclear modes analysis
We present a generic approach for treating the effect of nuclear motion in
the high-order harmonic generation from polyatomic molecules. Our procedure
relies on a separation of nuclear and electron dynamics where we account for
the electronic part using the Lewenstein model and nuclear motion enters as a
nuclear correlation function. We express the nuclear correlation function in
terms of Franck-Condon factors which allows us to decompose nuclear motion into
modes and identify the modes that are dominant in the high-order harmonic
generation process. We show results for the isotopes CH and CD and
thereby provide direct theoretical support for a recent experiment [Baker {\it
et al.}, Science {\bf 312}, 424 (2006)] that uses high-order harmonic
generation to probe the ultra-fast structural nuclear rearrangement of ionized
methane.Comment: 6 pages, 6 figure
Angular Normal Modes of a Circular Coulomb Cluster
We investigate the angular normal modes for small oscillations about an
equilibrium of a single-component coulomb cluster confined by a radially
symmetric external potential to a circle. The dynamical matrix for this system
is a Laplacian symmetrically circulant matrix and this result leads to an
analytic solution for the eigenfrequencies of the angular normal modes. We also
show the limiting dependence of the largest eigenfrequency for large numbers of
particles
Charge order in Magnetite. An LDA+ study
The electronic structure of the monoclinic structure of FeO is
studied using both the local density approximation (LDA) and the LDA+. The
LDA gives only a small charge disproportionation, thus excluding that the
structural distortion should be sufficient to give a charge order. The LDA+
results in a charge disproportion along the c-axis in good agreement with the
experiment. We also show how the effective can be calculated within the
augmented plane wave methods
High Q Cavity Induced Fluxon Bunching in Inductively Coupled Josephson Junctions
We consider fluxon dynamics in a stack of inductively coupled long Josephson
junctions connected capacitively to a common resonant cavity at one of the
boundaries. We study, through theoretical and numerical analysis, the
possibility for the cavity to induce a transition from the energetically
favored state of spatially separated shuttling fluxons in the different
junctions to a high velocity, high energy state of identical fluxon modes.Comment: 8 pages, 5 figure
Metodenotat om anvendelse af fremsyn i kommunale og regionale udviklings- og planstrategiprocesser
Pyramidal Atoms: Berylliumlike Hollow States
Based on the idea that four excited electrons arrange themselves around the
nucleus in the corners of a pyramid in order to minimize their mutual
repulsion, we present an analytical model of quadruply excited states. The
model shows excellent comparison with ab initio results and provides a clear
physical picture of the intrinsic motion of the four electrons. The model is
used to predict configuration-mixing fractions and spectra of these highly
correlated states.Comment: 4 pages, 2 figure
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