8,547 research outputs found
High-order harmonic generation from polyatomic molecules including nuclear motion and a nuclear modes analysis
We present a generic approach for treating the effect of nuclear motion in
the high-order harmonic generation from polyatomic molecules. Our procedure
relies on a separation of nuclear and electron dynamics where we account for
the electronic part using the Lewenstein model and nuclear motion enters as a
nuclear correlation function. We express the nuclear correlation function in
terms of Franck-Condon factors which allows us to decompose nuclear motion into
modes and identify the modes that are dominant in the high-order harmonic
generation process. We show results for the isotopes CH and CD and
thereby provide direct theoretical support for a recent experiment [Baker {\it
et al.}, Science {\bf 312}, 424 (2006)] that uses high-order harmonic
generation to probe the ultra-fast structural nuclear rearrangement of ionized
methane.Comment: 6 pages, 6 figure
Zero-Point cooling and low heating of trapped 111Cd+ ions
We report on ground state laser cooling of single 111Cd+ ions confined in
radio-frequency (Paul) traps. Heating rates of trapped ion motion are measured
for two different trapping geometries and electrode materials, where no effort
was made to shield the electrodes from the atomic Cd source. The low measured
heating rates suggest that trapped 111Cd+ ions may be well-suited for
experiments involving quantum control of atomic motion, including applications
in quantum information science.Comment: 4 pages, 6 figures, Submitted to PR
Manipulating the torsion of molecules by strong laser pulses
A proof-of-principle experiment is reported, where torsional motion of a
molecule, consisting of a pair of phenyl rings, is induced by strong laser
pulses. A nanosecond laser pulse spatially aligns the carbon-carbon bond axis,
connecting the two phenyl rings, allowing a perpendicularly polarized, intense
femtosecond pulse to initiate torsional motion accompanied by an overall
rotation about the fixed axis. The induced motion is monitored by femtosecond
time-resolved Coulomb explosion imaging. Our theoretical analysis accounts for
and generalizes the experimental findings.Comment: 4 pages, 4 figures, submitted to PRL; Major revision of the
presentation of the material; Correction of ion labels in Fig. 2(a
Strong Orientation Effects in Ionization of H by Short, Intense, High-Frequency Light Sources
We present three dimensional time-dependent calculations of ionization of
arbitrarily spatially oriented H by attosecond, intense, high-frequency
laser fields. The ionization probability shows a strong dependence on both the
internuclear distance and the relative orientation between the laser field and
the internuclear axis.Comment: 4 pages, 4 figure
Electronic structure of the ferromagnetic superconductor UCoGe from first principles
The superconductor UCoGe is analyzed with electronic structure calculations
using Linearized Augmented Plane Wave method based on Density Functional
Theory. Ferromagnetic and antiferromagnetic calculations with and without
correlations (via LDA+U) were done. In this compound the Fermi level is
situated in a region where the main contribution to DOS comes from the U-5f
orbital. The magnetic moment is mainly due to the Co-3d orbital with a small
contribution from the U-5f orbital. The possibility of fully non-collinear
magnetism in this compound seems to be ruled out. These results are compared
with the isostructural compound URhGe, in this case the magnetism comes mostly
from the U-5f orbital
Production of Strange Clusters and Strange Matter in Nucleus-Nucleus Collisions at the AGS
Production probabilities for strange clusters and strange matter in Au+Au
collisions at AGS energy are obtained in the thermal fireball model. The only
parameters of the model, the baryon chemical potential and temperature, were
determined from a description of the rather complete set of hadron yields from
Si+nucleus collisions at the AGS. For the production of light nuclear fragments
and strange clusters the results are similar to recent coalescence model
calculations. Strange matter production with baryon number larger than 10 is
predicted to be much smaller than any current experimental sensitivities.Comment: 9 Pages (no figures
Differential atom interferometry beyond the standard quantum limit
We analyze methods to go beyond the standard quantum limit for a class of
atomic interferometers, where the quantity of interest is the difference of
phase shifts obtained by two independent atomic ensembles. An example is given
by an atomic Sagnac interferometer, where for two ensembles propagating in
opposite directions in the interferometer this phase difference encodes the
angular velocity of the experimental setup. We discuss methods of squeezing
separately or jointly observables of the two atomic ensembles, and compare in
detail advantages and drawbacks of such schemes. In particular we show that the
method of joint squeezing may improve the variance by up to a factor of 2. We
take into account fluctuations of the number of atoms in both the preparation
and the measurement stage, and obtain bounds on the difference of the numbers
of atoms in the two ensembles, as well as on the detection efficiency, which
have to be fulfilled in order to surpass the standard quantum limit. Under
realistic conditions, the performance of both schemes can be improved
significantly by reading out the phase difference via a quantum non-demolition
(QND) measurement. Finally, we discuss a scheme using macroscopically entangled
ensembles.Comment: 10 pages, 5 figures; eq. (3) corrected and other minor change
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